Dynamical charge inhomogeneity and crystal-field fluctuations for 4f ions in high-Tc cuprates

The main relaxation mechanism of crystal-field excitations in rare-earth ions in cuprates is believed to be provided by the fluctuations of crystalline electric field induced by a dynamic charge inhomogeneity generic for the doped cuprates. We address the generalized granular model as one of the model scenario for such an ingomogeneity where the cuprate charge subsystem remind that of Wigner crystal with the melting transition and phonon-like positional excitation modes. Formal description of R-ion relaxation coincides with that of recently suggested magnetoelastic mechanism.Comment: 4 page

Unusual interplay between copper-spin and vortex dynamics in slightly overdoped La{1.83}Sr{0.17}CuO{4}

Our inelastic neutron scattering experiments of the spin excitations in the slightly overdoped La{1.83}Sr{0.17}CuO{4} compound show that, under the application of a magnetic field of 5 Tesla, the low-temperature susceptibility undergoes a weight redistribution centered at the spin-gap energy. Furthermore, by comparing the temperature dependence of the neutron data with ac-susceptibility and magnetization measurements, we conclude that the filling in of the spin gap tracks the irreversibility/melting temperature rather than Tc2, which indicates an unusual interplay between the magnetic vortices and the spin excitations even in the slightly overdoped regime of high-temperature superconductors.Comment: 7 pages, including 5 figure

Incommensurate magnetic ordering in Cu2Te2O5X2Cu_2 Te_2 O_5 X_2 (X=Cl,Br) studied by neutron diffraction

We present the results of the first neutron powder and single crystal diffraction studies of the coupled spin tetrahedra systems {\CuTeX} (X=Cl, Br). Incommensurate antiferromagnetic order with the propagation vectors {\bf{k}_{Cl}}\approx[0.150,0.422,\half], {\bf{k}_{Br}}\approx[0.158,0.354,\half] sets in below $T_{N}$=18 K for X=Cl and 11 K for X=Br. No simple collinear antiferromagnetic or ferromagnetic arrangements of moments within Cu${}^{2+}$ tetrahedra fit these observations. Fitting the diffraction data to more complex but physically reasonable models with multiple helices leads to a moment of 0.67(1)$\mu_B$/Cu${}^{2+}$ at 1.5 K for the Cl-compound. The reason for such a complex ground state may be geometrical frustration of the spins due to the intra- and inter-tetrahedral couplings having similar strengths. The magnetic moment in the Br- compound, calculated assuming it has the same magnetic structure as the Cl compound, is only 0.51(5)$\mu_B$/Cu${}^{2+}$ at 1.5 K. In neither compound has any evidence for a structural transition accompanying the magnetic ordering been found

Influence of higher d-wave gap harmonics on the dynamical magnetic susceptibility of high-temperature superconductors

Using a fermiology approach to the computation of the magnetic susceptibility measured by neutron scattering in hole-doped high-Tc superconductors, we estimate the effects on the incommensurate peaks caused by higher d-wave harmonics of the superconducting order parameter induced by underdoping. The input parameters for the Fermi surface and d-wave gap are taken directly from angle resolved photoemission (ARPES) experiments on Bi{2}Sr{2}CaCu{2}O{8+x} (Bi2212). We find that higher d-wave harmonics lower the momentum dependent spin gap at the incommensurate peaks as measured by the lowest spectral edge of the imaginary part in the frequency dependence of the magnetic susceptibility of Bi2212. This effect is robust whenever the fermiology approach captures the physics of high-Tc superconductors. At energies above the resonance we observe diagonal incommensurate peaks. We show that the crossover from parallel incommensuration below the resonance energy to diagonal incommensuration above it is connected to the values and the degeneracies of the minima of the 2-particle energy continuum.Comment: 13 pages, 7 figure

Direct observation of impurity-induced magnetism in an S = 1/2 antiferromagnetic Heisenberg 2-leg spin ladder

Nuclear magnetic resonance and magnetization measurements were used to probe the magnetic features of single-crystalline Bi(Cu(1-x)Znx)2PO6 with 0<x<0.05 at temperatures between 2.6 K and 300 K. The simple lineshape of the 31P NMR signals of the pristine compound changes considerably for x>0 and we present clear evidence for a temperature dependent variation of the local magnetization close to the Zn sites. The generic nature of this observation is indicated by results of model calculations on appropriate spin systems of limited size employing QMC methods.Comment: 4 pages, 4 figure

Nodal-to-nodeless superconducting order parameter in LaFeAs1−x_{1-x}Px_xO synthesized under high pressure

Similar to chemical doping, pressure produces and stabilizes new phases of known materials, whose properties may differ greatly from those of their standard counterparts. Here, by considering a series of LaFeAs$_{1-x}$P$_x$O iron-pnictides synthesized under high-pressure high-temperature conditions, we investigate the simultaneous effects of pressure and isoelectronic doping in the 1111 family. Results of numerous macro- and microscopic technique measurements, unambiguously show a radically different phase diagram for the pressure-grown materials, characterized by the lack of magnetic order and the persistence of superconductivity across the whole $0.3 \leq x \leq 0.7$ doping range. This unexpected scenario is accompanied by a branching in the electronic properties across $x = 0.5$, involving both the normal and superconducting phases. Most notably, the superconducting order parameter evolves from nodal (for $x < 0.5$) to nodeless (for $x \geq 0.5$), in clear contrast to other 1111 and 122 iron-based materials grown under ambient-pressure conditions.Comment: 9 pages, 7 figures, Suppl. materia

Impact of strong disorder on the static magnetic properties of the spin-chain compound BaCu2SiGeO7

The disordered quasi-1D magnet BaCu2SiGeO7 is considered as one of the best physical realizations of the random Heisenberg chain model, which features an irregular distribution of the exchange parameters and whose ground state is predicted to be the scarcely investigated random-singlet state (RSS). Based on extensive 29Si NMR and magnetization studies of BaCu2SiGeO7, combined with numerical Quantum Monte Carlo simulations, we obtain remarkable quantitative agreement with theoretical predictions of the random Heisenberg chain model and strong indications for the formation of a random-singlet state at low temperatures in this compound. As a local probe, NMR is a well-adapted technique for studying the magnetism of disordered systems. In this case it also reveals an additional local transverse staggered field (LTSF), which affects the low-temperature properties of the RSS. The proposed model Hamiltonian satisfactorily accounts for the temperature dependence of the NMR line shapes.Comment: 10 pages, 7 figure

Structure and superconductivity in the binary Re1−x_{1-x}Mox_x alloys

The binary Re$_{1-x}$Mo$_x$ alloys, known to cover the full range of solid solutions, were successfully synthesized and their crystal structures and physical properties investigated via powder x-ray diffraction, electrical resistivity, magnetic susceptibility, and heat capacity. By varying the Re/Mo ratio we explore the full Re$_{1-x}$Mo$_x$ binary phase diagram, in all its four different solid phases: hcp-Mg ($P6_3/mmc$), $\alpha$-Mn ($I\overline{4}3m$), $\beta$-CrFe ($P4_2/mnm$), and bcc-W ($Im\overline{3}m$), of which the second is non-centrosymmetric with the rest being centrosymmetric. All Re$_{1-x}$Mo$_x$ alloys are superconductors, whose critical temperatures exhibit a peculiar phase diagram, characterized by three different superconducting regions. In most alloys the $T_c$ is almost an order of magnitude higher than in pure Re and Mo. Low-temperature electronic specific-heat data evidence a fully-gapped superconducting state, whose enhanced gap magnitude and specific-heat discontinuity suggest a moderately strong electron-phonon coupling across the series. Considering that several $\alpha$-Mn-type Re$T$ alloys ($T$ = transition metal) show time-reversal symmetry breaking (TRSB) in the superconducting state, while TRS is preserved in the isostructural Mg$_{10}$Ir$_{19}$B$_{16}$ or Nb$_{0.5}$Os$_{0.5}$, the Re$_{1-x}$Mo$_x$ alloys represent another suitable system for studying the interplay of space-inversion, gauge, and time-reversal symmetries in future experiments expected to probe TRSB in the Re$T$ family.Comment: 8 pages, 7 figures, accepted for publication on Physical Review Material