APPLICATION OF MICROCANONICAL TEMPERATURE TO THE SPIN CROSSOVER OF Fe-Co COMPOUNDS

Using the Rugh’s microcanonical approach to temperature we study the classical model of three dimensional spin-crossover of Fe-Co compounds. These compounds are characterized by magnetic ions that can be in a high-spin or low-spin state. We consider the case of diamagnetic low-spin state. The values of the magnetization average, and fraction of high-spin/low-spin are studied over a wide range of values for the system size, temperature, magnetic field, energy difference, nearest neighbor coupling and exchange interaction. We also address the metastability according to the relative values of interaction parameters and the phase diagram of the model. Keywords: phase transition, dynamical temperature, spin crossove

Auxiliary particle theory of threshold singularities in photoemission and X-ray absorption spectra: Test of a conserving T-matrix approximation

We calculate the exponents of the threshold singularities in the photoemission spectrum of a deep core hole and its X-ray absorption spectrum in the framework of a systematic many-body theory of slave bosons and pseudofermions (for the empty and occupied core level). In this representation, photoemission and X-ray absorption can be understood on the same footing; no distinction between orthogonality catastrophe and excitonic effects is necessary. We apply the conserving slave particle T-matrix approximation (CTMA), recently developed to describe both Fermi and non-Fermi liquid behavior systems with strong local correlations, to the X-ray problem as a test case. The numerical results for both photoemission and X-ray absorption are found to be in agreement with the exact infrared powerlaw behavior in the weak as well as in the strong coupling regions. We point out a close relation of the CTMA with the parquet equation approach of Nozi{\`e}res et al.Comment: 10 pages, 9 figures, published versio

Fermi Edge Singularities and Backscattering in a Weakly Interacting 1D Electron Gas

The photon-absorption edge in a weakly interacting one-dimensional electron gas is studied, treating backscattering of conduction electrons from the core hole exactly. Close to threshold, there is a power-law singularity in the absorption, $I(\epsilon) \propto \epsilon^{-\alpha}$, with $\alpha = 3/8 + \delta_+/\pi - \delta_+^2/2\pi^2$ where $\delta_+$ is the forward scattering phase shift of the core hole. In contrast to previous theories, $\alpha$ is finite (and universal) in the limit of weak core hole potential. In the case of weak backscattering $U(2k_F)$, the exponent in the power-law dependence of absorption on energy crosses over to a value $\alpha = \delta_+/\pi - \delta_+^2/2\pi^2$ above an energy scale $\epsilon^* \sim [U(2k_F)]^{1/\gamma}$, where $\gamma$ is a dimensionless measure of the electron-electron interactions.Comment: 8 pages + 1 postscript figure, preprint TPI-MINN-93/40-

Tunneling into a two-dimensional electron system in a strong magnetic field

We investigate the properties of the one-electron Green's function in an interacting two-dimensional electron system in a strong magnetic field, which describes an electron tunneling into such a system. From finite-size diagonalization, we find that its spectral weight is suppressed near zero energy, reaches a maximum at an energy of about $0.2e^{2}/\epsilon l_{c}$, and decays exponentially at higher energies. We propose a theoretical model to account for the low-energy behavior. For the case of Coulomb interactions between the electrons, at even-denominator filling factors such as $\nu=1/2$, we predict that the spectral weight varies as $e^{-\omega_0/|\omega|}$, for $\omega\rightarrow 0$

Flow equation analysis of the anisotropic Kondo model

We use the new method of infinitesimal unitary transformations to calculate zero temperature correlation functions in the strong-coupling phase of the anisotropic Kondo model. We find the dynamics on all energy scales including the crossover behaviour from weak to strong coupling. The integrable structure of the Hamiltonian is not used in our approach. Our method should also be useful in other strong-coupling models since few other analytical methods allow the evaluation of their correlation functions on all energy scales.Comment: 4 pages RevTeX, 2 eps figures include

Fermi edge singularities in X-ray spectra of strongly correlated fermions

We discuss the problem of the X-ray absorption in a system of interacting fermions and, in particular, those features in the X-ray spectra that can be used to discriminate between conventional Fermi-liquids and novel "strange metals". Focusing on the case of purely forward scattering off the core-hole potential, we account for the relevant interactions in the conduction band by means of the bosonization technique. We find that the X-ray Fermi edge singularities can still be present, although modified, even if the density of states vanishes at the Fermi energy, and that, in general, the relationship between the two appears to be quite subtle.Comment: Latex, 16 pages, Princeton preprin

Dynamics of Tunneling Centers in Metallic Systems

Dynamics of tunneling centers (TC) in metallic systems is studied, using the technique of bosonization. The interaction of the TC with the conduction electrons of the metal involves two processes, namely, the screening of the TC by electrons, and the so-called electron assisted tunneling. The presence of the latter process leads to a different form of the renormalized tunneling frequency of the TC, and the tunneling motion is damped with a temperature dependent relaxation rate. As the temperature is lowered, the relaxation rate per temperature shows a steep rise as opposed to that in the absence of electron assisted process. It is expected that this behavior should be observed at very low temperatures in a careful experiment. The present work thus tries to go beyond the existing work on the {\it dynamics} of a two-level system in metals, by treating the electron assisted process.Comment: REVTeX twocolumn format, 5 pages, two PostScript figures available on request. Preprint # : imsc 94/3

Numerical Calculation of the Fidelity for the Kondo and the Friedel-Anderson Impurities

The fidelities of the Kondo and the Friedel-Anderson (FA) impurities are calculated numerically. The ground states of both systems are calculated with the FAIR (Friedel artificially inserted resonance) theory. The ground state in the interacting systems is compared with a nullstate in which the interaction is zero. The different multi-electron states are expressed in terms of Wilson states. The use of N Wilson states simulates the use of a large effective number N_{eff} of states. A plot of ln(F) versus N\proptoln(N_{eff}) reveals whether one has an Anderson orthogonality catastrophe at zero energy. The results are at first glance surprising. The ln(F)-ln(N_{eff}) plot for the Kondo impurity diverges for large N_{eff}. On the other hand, the corresponding plot for the symmetric FA impurity saturates for large N_{eff} when the level spacing at the Fermi level is of the order of the singlet-triplet excitation energy. The behavior of the fidelity allows one to determine the phase shift of the electron states in this regime. PACS: 75.20.Hr, 71.23.An, 71.27.+a, 05.30.-

Fermi-edge singularities in linear and non-linear ultrafast spectroscopy

We discuss Fermi-edge singularity effects on the linear and nonlinear transient response of an electron gas in a doped semiconductor. We use a bosonization scheme to describe the low energy excitations, which allows to compute the time and temperature dependence of the response functions. Coherent control of the energy absorption at resonance is analyzed in the linear regime. It is shown that a phase-shift appears in the coherent control oscillations, which is not present in the excitonic case. The nonlinear response is calculated analytically and used to predict that four wave-mixing experiments would present a Fermi-edge singularity when the exciting energy is varied. A new dephasing mechanism is predicted in doped samples that depends linearly on temperature and is produced by the low-energy bosonic excitations in the conduction band.Comment: long version; 9 pages, 4 figure

Anomalous heavy-fermion and ordered states in the filled skutterudite PrFe4P12

Specific heat and magnetization measurements have been performed on high-quality single crystals of filled-skutterudite PrFe_4P_{12} in order to study the high-field heavy-fermion state (HFS) and low-field ordered state (ODS). From a broad hump observed in C/T vs T in HFS for magnetic fields applied along the direction, the Kondo temperature of ~ 9 K and the existence of ferromagnetic Pr-Pr interactions are deduced. The {141}-Pr nuclear Schottky contribution, which works as a highly-sensitive on-site probe for the Pr magnetic moment, sets an upper bound for the ordered moment as ~ 0.03 \mu_B/Pr-ion. This fact strongly indicates that the primary order parameter in the ODS is nonmagnetic and most probably of quadrupolar origin, combined with other experimental facts. Significantly suppressed heavy-fermion behavior in the ODS suggests a possibility that the quadrupolar degrees of freedom is essential for the heavy quasiparticle band formation in the HFS. Possible crystalline-electric-field level schemes estimated from the anisotropy in the magnetization are consistent with this conjecture.Comment: 7 pages and 7 figures. Accepted for publication in Phys. Rev.