Electronic correlations in double ionization of atoms in pump-probe experiments

The ionization dynamics of a two-electron atom in an attosecond XUV-infrared pump-probe experiment is simulated by solving the time-dependent two-electron Schr\"odinger equation. A dramatic change of the double ionization (DI) yield with variation of the pump-probe delay is reported and the governing role of electron-electron correlations is shown. The results allow for a direct control of the DI yield and of the relative strength of double and single ionization

Towards a theory of attosecond transient recorder

Laser assisted photoemission by a chirped subfemtosecond extreme ultraviolet (XUV) pulse is considered within an exactly solvable quantum-mechanical model. Special emphasis is given to the energy dependence of photoexcitation cross-section. The streaked spectra are analyzed within the classical picture of initial time-momentum distribution r_ini(p,t) of photoelectrons mapped to the final energy scale. The actual time-momentum distribution in the absence of the probe laser field is shown to be a poor choice for r_ini, and a more adequate ansatz is suggested. The semiclassical theory offers a simple practically useful approximation for streaked spectra. Its limitations for sufficiently long chirped XUV pulses are established.Comment: 9 pages 8 figure

Anticorrelation between temperature and fluctuations in moderately damped Josephson junctions

We study the influence of dissipation on the switching current statistics of moderately damped Josephson junctions. Different types of both low- and high- $T_c$ junctions with controlled damping are studied. The damping parameter of the junctions is tuned in a wide range by changing temperature, magnetic field, gate voltage, introducing a ferromagnetic layer or in-situ capacitive shunting. A paradoxical collapse of switching current fluctuations occurs with increasing $T$ in all studied junctions. The phenomenon critically depends on dissipation in the junction and is explained by interplay of two counteracting consequences of thermal fluctuations, which on the one hand assist in premature switching into the resistive state and on the other hand help in retrapping back to the superconducting state. This is one of the rare examples of anticorrelation between temperature and fluctuation amplitude of a physically measurable quantity.Comment: 17 pages, 20 figure

Efficient grid-based method in nonequilibrium Green's function calculations. Application to model atoms and molecules

We propose and apply the finite-element discrete variable representation to express the nonequilibrium Green's function for strongly inhomogeneous quantum systems. This method is highly favorable against a general basis approach with regard to numerical complexity, memory resources, and computation time. Its flexibility also allows for an accurate representation of spatially extended hamiltonians, and thus opens the way towards a direct solution of the two-time Schwinger/Keldysh/Kadanoff-Baym equations on spatial grids, including e.g. the description of highly excited states in atoms. As first benchmarks, we compute and characterize, in Hartree-Fock and second Born approximation, the ground states of the He atom, the H$_2$ molecule and the LiH molecule in one spatial dimension. Thereby, the ground-state/binding energies, densities and bond-lengths are compared with the direct solution of the time-dependent Schr\"odinger equation.Comment: 11 pages, 5 figures, submitted to Physical Review