Landauer Theory, Inelastic Scattering and Electron Transport in Molecular Wires

In this paper we address the topic of inelastic electron scattering in mesoscopic quantum transport. For systems where only elastic scattering is present, Landauer theory provides an adequate description of transport that relates the electronic current to single-particle transmission and reflection probabilities. A formalism proposed recently by Bonca and Trugman facilitates the calculation of the one-electron transmission and reflection probabilities for inelastic processes in mesoscopic conductors connected to one-dimensional ideal leads. Building on their work, we have developed a self-consistent procedure for the evaluation of the non-equilibrium electron distributions in ideal leads connecting such mesoscopic conductors to electron reservoirs at finite temperatures and voltages. We evaluate the net electronic current flowing through the mesoscopic device by utilizing these non-equilibrium distributions. Our approach is a generalization of Landauer theory that takes account of the Pauli exclusion principle for the various competing elastic and inelastic processes while satisfying the requirement of particle conservation. As an application we examine the influence of elastic and inelastic scattering on conduction through a two site molecular wire with longitudinal phonons using the Su-Schrieffer-Heeger model of electron-phonon coupling.Comment: 25 pages, 8 figure

Stationary cantilever vibrations in the oscillating cantilever-driven adiabatic reversals -- magnetic resonance force microscopy technique

We consider theoretically the novel technique in magnetic resonance force microscopy which is called ``oscillating cantilever-driven adiabatic reversals''. We present analytical and numerical analysis for the stationary cantilever vibrations in this technique. For reasonable values of parameters we estimate the resonant frequency shift as 6Hz per the Bohr magneton. We analyze also the regime of small oscillations of the paramagnetic moment near the transversal plane and the frequency shift of the damped cantilever vibrations.Comment: 12 pages RevTex

Spin Relaxation Caused by Thermal Excitations of High Frequency Modes of Cantilever Vibrations

We consider the process of spin relaxation in the oscillating cantilever-driven adiabatic reversals technique in magnetic resonance force microscopy. We simulated the spin relaxation caused by thermal excitations of the high frequency cantilever modes in the region of the Rabi frequency of the spin sub-system. The minimum relaxation time obtained in our simulations is greater but of the same order of magnitude as one measured in recent experiments. We demonstrated that using a cantilever with nonuniform cross-sectional area may significantly increase spin relaxation time.Comment: 12 pages RevTe

Single-Spin Measurement and Decoherence in Magnetic Resonance Force Microscopy

We consider a simple version of a cyclic adiabatic inversion (CAI) technique in magnetic resonance force microscopy (MRFM). We study the problem: What component of the spin is measured in the CAI MRFM? We show that the non-destructive detection of the cantilever vibrations provides a measurement of the spin component along the effective magnetic field. This result is based on numerical simulations of the Hamiltonian dynamics (the Schrodinger equation) and the numerical solution of the master equation.Comment: 5 pages + 5 figures (PNG format

Transient Dynamics in Magnetic Force Microscopy for a Single-Spin Measurement

We analyze a single-spin measurement using a transient process in magnetic force microscopy (MFM) which could increase the maximum operating temperature by a factor of Q (the quality factor of the cantilever) in comparison with the static Stern-Gerlach effect. We obtain an exact solution of the master equation, which confirms this result. We also discuss the conditions required to create a macroscopic Schrodinger cat state in the cantilever.Comment: 22 pages 2 figure

Decoherence in elastic and polaronic transport via discrete quantum states

Here we study the effect of decoherence on elastic and polaronic transport via discrete quantum states. The calculations are performed with the help of nonperturbative computational scheme, based on the Green's function theory within the framework of polaron transformation (GFT-PT), where the many-body electron-phonon interaction problem is mapped exactly into a single-electron multi-channel scattering problem. In particular, the influence of dephasing and relaxation processes on the shape of the electrical current and shot noise curves is discussed in detail under the linear and nonlinear transport conditions.Comment: 11 pages, 3 figure

Theory of Current and Shot Noise Spectroscopy in Single-Molecular Quantum Dots with Phonon Mode

Using the Keldysh nonequilibrium Green function technique, we study the current and shot noise spectroscopy of a single molecular quantum dot coupled to a local phonon mode. It is found that in the presence of electron-phonon coupling, in addition to the resonant peak associated with the single level of the dot, satellite peaks with the separation set by the frequency of phonon mode appear in the differential conductance. In the ``single level'' resonant tunneling region, the differential shot noise power exhibit two split peaks. However, only single peaks show up in the ``phonon assisted'' resonant-tunneling region. An experimental setup to test these predictions is also proposed.Comment: 5 pages, 3 eps figures embedde

Realistic simulations of single-spin nondemolition measurement by magnetic resonance force microscopy

A requirement for many quantum computation schemes is the ability to measure single spins. This paper examines one proposed scheme: magnetic resonance force microscopy, including the effects of thermal noise and back-action from monitoring. We derive a simplified equation using the adiabatic approximation, and produce a stochastic pure state unraveling which is useful for numerical simulations.Comment: 33 pages LaTeX, 9 figure files in EPS format. Submitted to Physical Review

Optical Detection of a Single Nuclear Spin

We propose a method to optically detect the spin state of a 31-P nucleus embedded in a 28-Si matrix. The nuclear-electron hyperfine splitting of the 31-P neutral-donor ground state can be resolved via a direct frequency discrimination measurement of the 31-P bound exciton photoluminescence using single photon detectors. The measurement time is expected to be shorter than the lifetime of the nuclear spin at 4 K and 10 T.Comment: 4 pages, 3 figure

Phonon and plasmon excitation in inelastic electron tunneling spectroscopy of graphite

The inelastic electron tunneling spectrum (IETS)of highly oriented pyrolitic graphite (HOPG) has been measured with scanning tunneling spectroscopy (STS) at 6K. The observed spectral features are in very good agreement with the vibrational density of states (vDOS) of graphite calculated from first principles. We discuss the enhancement of certain phonon modes by phonon-assisted tunneling in STS based on the restrictions imposed by the electronic structure of graphite. We also demonstrate for the first time the local excitation of surface-plasmons in IETS which are detected at an energy of 40 meV.Comment: PRB rapid communication, submitte