115 research outputs found

    Magnetoresistance of Pr1βˆ’x_{1-x}Lax_xOs4_4Sb12_{12}: Disentangling local crystalline-electric-field physics and lattice effects

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    Resistivity measurements were performed on Pr1βˆ’x_{1-x}Lax_xOs4_4Sb12_{12} single crystals at temperatures down to 20 mK and in fields up to 18 T. The results for dilute-Pr samples (x=0.3x=0.3 and 0.67) are consistent with model calculations performed assuming a singlet crystalline-electric-field (CEF) ground state. The residual resistivity of these crystals features a smeared step centered around 9 T, the predicted crossing field for the lowest CEF levels. The CEF contribution to the magnetoresistance has a weaker-than-calculated dependence on the field direction, suggesting that interactions omitted from the CEF model lead to avoided crossing in the effective levels of the Pr3+^{3+} ion. The dome-shaped magnetoresistance observed for x=0x = 0 and 0.05 cannot be reproduced by the CEF model, and likely results from fluctuations in the field-induced antiferroquadrupolar phase

    First and second order magnetic and structural transitions in BaFe2(1βˆ’x)_{2(1-x)}Co2x_{2x}As2_{2}

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    We present here high resolution magnetization measurements on high-quality BaFe2(1βˆ’x)_{2(1-x)}Co2x_{2x}As2_{2}, 0≀\leqx≀\leq0.046 as-grown single crystals. The results confirm the existence of a magnetic tricritical point in the (xx,TT) plane at xtrm^{m}_{tr}β‰ˆ\approx0.022 and reveal the emergence of the heat capacity anomaly associated with the onset of the structural transition at xs^{s}β‰ˆ\approx0.0064. We show that the samples with doping near xtrm^{m}_{tr} do not show superconductivity, but rather superconductivity emerges at a slightly higher cobalt doping, xβ‰ˆ\approx0.0315Comment: 4 pages, 5 figure

    Exotic Kondo-hole band resistivity and magnetoresistance of Ce1βˆ’x_{1-x}Lax_{x}Os4_4Sb12_{12} alloys

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    Electrical resistivity measurements of non-magnetic single-crystalline Ce1βˆ’x_{1-x}Lax_xOs4_4Sb12_{12} alloys, x=0.02x=0.02 and 0.1, are reported for temperatures down to 20 mK and magnetic fields up to 18 T. At the lowest temperatures, the resistivity of Ce0.98_{0.98}La0.02_{0.02}Os4_4Sb12_{12} has a Fermi-liquid-like temperature variation ρ=ρ0+AT2\rho=\rho_0+A T^2, but with negative AA in small fields. The resistivity has an unusually strong magnetic field dependence for a paramagnetic metal. The 20 mK resistivity increases by 75% between H=0 and 4 T and then decreases by 65% between 4 T and 18 T. Similarly, the AA coefficient increases with the field from -77 to 29ΞΌΞ© \mu\OmegacmKβˆ’2^{-2} between H=0 and 7 T and then decreases to 18ΞΌΞ© \mu\OmegacmKβˆ’2^{-2} for 18 T. This nontrivial temperature and field variation is attributed to the existence of a very narrow Kondo-hole band in the hybridization gap, which pins the Fermi energy. Due to disorder the Kondo-hole band has localized states close to the band edges. The resistivity for x=0.1x=0.1 has a qualitatively similar behavior to that of x=0.02x=0.02, but with a larger Kondo-hole band
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