120 research outputs found
High resolution for x-ray spectroscopy studies with highly charged heavy ions at the CRYRING@ESR electron cooler
In this work, we report on the first x-ray spectroscopy study associated with the RR processes for bare lead ions at the electron cooler of the CRYRING@ESR, as storage rings are currently the only facilities routinely delivering hydrogen-like ions at high-Z in large quantities. With ultra-cold electron beam temperatures and near zero electron-ion collision energies, the effective production of characteristic projectile x-rays was well demonstrated at 0 deg and 180 deg observation geometries in our experiment by decelerated 10 MeV/u hydrogen-like lead ions. To reveal the role of radiative feeding transitions in the formation of observed intense Lyman and Balmer lines, an elaborate theoretical model describing the radiative decay dynamics and each (n, l, j)-state population varying over time is put to a test. As a result, the presented rigorous treatment reproduces observed x-ray spectroscopy really well in terms of the RR transitions and characteristic x-ray lines. In addition, we found a strong enhancement for l = n − 1 states in inner shells due to radiative Yrast-cascades from high Rydberg states, that finally contribute strikingly to the observed intensities of characteristic x-ray lines. Further on the current thesis lays the basis for a successful effort to push the experimental resolution of x-ray spectroscopy for L → K ground-state transitions at high-Z of below 80 eV at about 100 keV. This was done in an RR experiment of free electrons into the bound states of initially hydrogen-like uranium ions by adopting low temperature x-ray detectors, namely metallic magnetic calorimeters. Such an experiment allowed us for the first time to resolve the substructure of the Kα2 line and partially the Kα1 line in helium-like uranium ions. The preliminary data again prove the unique potential of the experimental method based on x-ray spectroscopy at the electron cooler of the CRYRING@ESR
Comment on "Atomic Scale Structure and Chemical Composition across Order-Disorder Interfaces"
Interfaces have long been known to be the key to many mechanical and electric
properties. To nickel base superalloys which have perfect creep and fatigue
properties and have been widely used as materials of turbine blades, interfaces
determine the strengthening capacities in high temperature. By means of high
resolution scanning transmission electron microscopy (HRSTEM) and 3D atom probe
(3DAP) tomography, Srinivasan et al. proposed a new point that in nickel base
superalloys there exist two different interfacial widths across the
{\gamma}/{\gamma}' interface, one corresponding to an order-disorder
transition, and the other to the composition transition. We argue about this
conclusion in this comment
Fast Network Community Detection with Profile-Pseudo Likelihood Methods
The stochastic block model is one of the most studied network models for
community detection. It is well-known that most algorithms proposed for fitting
the stochastic block model likelihood function cannot scale to large-scale
networks. One prominent work that overcomes this computational challenge is
Amini et al.(2013), which proposed a fast pseudo-likelihood approach for
fitting stochastic block models to large sparse networks. However, this
approach does not have convergence guarantee, and is not well suited for small-
or medium- scale networks. In this article, we propose a novel likelihood based
approach that decouples row and column labels in the likelihood function, which
enables a fast alternating maximization; the new method is computationally
efficient, performs well for both small and large scale networks, and has
provable convergence guarantee. We show that our method provides strongly
consistent estimates of the communities in a stochastic block model. As
demonstrated in simulation studies, the proposed method outperforms the
pseudo-likelihood approach in terms of both estimation accuracy and computation
efficiency, especially for large sparse networks. We further consider
extensions of our proposed method to handle networks with degree heterogeneity
and bipartite properties
The normal-auxeticity mechanical phase transition in graphene
When a solid object is stretched, in general, it shrinks transversely. However, the abnormal ones are
auxetic, which exhibit lateral expansion, or negative Poisson ratio. While graphene is a paradigm
2D material, surprisingly, graphene converts from normal to auxetic at certain strains. Here, we
show via molecular dynamics simulations that the normal-auxeticity mechanical phase transition
only occurs in uniaxial tension along the armchair direction or the nearest neighbor direction. Such
a characteristic persists at temperatures up to 2400 K. Besides monolayer, bilayer and multi-layer
graphene also possess such a normal-auxeticity transition. This unique property could extend the
applications of graphene to new horizons
Digital photoprogramming of liquid-crystal superstructures featuring intrinsic chiral photoswitches
Dynamic patterning of soft materials in a fully reversible and programmable manner with light enables applications in anti-counterfeiting, displays and labelling technology. However, this is a formidable challenge due to the lack of suitable chiral molecular photoswitches. Here, we report the development of a unique intrinsic chiral photoswitch with broad chirality modulation to achieve digitally controllable, selectable and extractable multiple stable reflection states. An anti-counterfeiting technique, embedded with diverse microstructures, featuring colour-tunability, erasability, reversibility, multi-stability and viewing-angle dependency of pre-recorded patterns, is established with these photoresponsive superstructures. This strategy allows dynamic helical transformation from the molecular and supramolecular to the macroscopic level using light-activated intrinsic chirality, demonstrating the practicality of photoprogramming photonics
High-sensitivity magnetic sensor based on the evanescent scattering by a magnetorheological film
We present a simple concept to implement a magnetic sensor that uses evanescent scattering by a suspended magnetorheological (MR) film above a planar waveguide. The soft MR film embedded with ferromagnetic particles is to induce scattering on the evanescent field of a planar waveguide at a proximity distance. This distance can be controlled precisely by a magnetic field. Consequently, the waveguide output power changes in response to the magnetic intensity. Two sensor prototypes of different film thicknesses were designed and tested showing a trade-off between the sensitivity and dynamic sensing range. A maximum sensitivity of ∼2.62dB/mT was obtained. Compared to optical micro-electromechanical systems, the presented sensors feature a simple design, easy fabrication, low cost, and the potential for large-scale production and miniaturization to be integrated into portable devices
Determination of incommensurate modulated structure in Bi2Sr1.6La0.4CuO6+{\delta} by aberration-corrected transmission electron microscopy
Incommensurate modulated structure (IMS) in Bi2Sr1.6La0.4CuO6+{\delta}
(BSLCO) has been studied by aberration corrected transmission electron
microscopy in combination with high-dimensional (HD) space description. Two
images in the negative Cs imaging (NCSI) and passive Cs imaging (PCSI) modes
were deconvoluted, respectively. Similar results as to IMS have been obtained
from two corresponding projected potential maps (PPMs), but meanwhile the size
of dots representing atoms in the NCSI PPM is found to be smaller than that in
PCSI one. Considering that size is one of influencing factors of precision,
modulation functions for all unoverlapped atoms in BSLCO were determined based
on the PPM obtained from the NCSI image in combination with HD space
description
Magic auxeticity angle of graphene
Solids exhibit transverse shrinkage when they are stretched, except auxetics that abnormally demonstrate lateral expansion instead. Graphene possesses the unique normal-auxeticity (NA) transition when it is stretched along the armchair direction but not along the zigzag direction. Here we report on the anisotropic temperature-dependent NA transitions in strained graphene using molecular dynamics simulations. The critical strain where the NA transition occurs increases with respect to an increase in the tilt angle deviating from armchair direction upon uniaxial loading. The magic angle for the NA transition is 10.9°, beyond which the critical strain is close to fracture strain. In addition, the critical strain decreases with an increasing temperature when the tilt angle is smaller than the NA magic angle. Our results shed lights on the unprecedented nonlinear dimensional response of graphene to the large mechanical loading at various temperatures
- …