Structural Properties of Two-Dimensional Strontium Titanate: A First-Principles Investigation

Motivated by the experimental synthesis of two-dimensional (2D) perovskite materials, we study the stability of 2D SrTiO$_3$ from first principles. We find that the TiO$_6$ octahedral rotations emerge in 2D SrTiO$_3$ with a rotation angle twice that in the 3D bulk. The rotation angle decreases significantly with the film thickness, reflecting the strong interlayer coupling that is absent in the conventional 2D materials. Using the molecular dynamics simulations, the cubic-like phase is found to appear above 1000 K that is much higher than the transition temperature of 3D SrTiO$_3$.Comment: 5 pages, 4 figure

Magnetic field induced effects in the high source-drain bias current of weakly coupled vertical quantum dot molecules

We report on the basic properties of recently observed magnetic field resonance, induced time dependent oscillation, and hysteresis effects in the current flowing through two weakly coupled vertical quantum dots at high source-drain bias (up to a few tens of mV). These effects bare some similarity to those reported in the N=2 spin-blockade regime, usually for weak in-plane magnetic field, of quantum dot molecules and attributed to hyperfine coupling, except here the measurements are conducted outside of the spin-blockade regime and the out-of-plane magnetic field is up to ~6 T.Comment: 3 pages, 3 figures, accepted for publication in Physica E in EP2DS 17 conference proceeding

Determination of effective microscopic models for the frustrated antiferromagnets Cs2_2CuCl4_4 and Cs2_2CuBr4_4 by density functional methods

We investigate the electronic and magnetic properties of the frustrated triangular-lattice antiferromagnets Cs$_2$CuCl$_4$ and Cs$_2$CuBr$_4$ in the framework of density functional theory. Analysis of the exchange couplings J and J' using the available X-ray structural data corroborates the values obtained from experimental results for Cs$_2$CuBr$_4$ but not for Cs$_2$CuCl$_4$. In order to understand this discrepancy, we perform a detailed study of the effect of structural optimization on the exchange couplings of Cs$_2$CuCl$_4$ employing different exchange-correlation functionals. We find that the exchange couplings depend on rather subtle details of the structural optimization and that only when the insulating state (mediated through spin polarization) is present in the structural optimization, we do have good agreement between the calculated and the experimentally determined exchange couplings. Finally, we discuss the effect of interlayer couplings as well as longer-ranged couplings in both systems.Comment: Phys. Rev. B in pres

Two level anti-crossings high up in the single-particle energy spectrum of a quantum dot

We study the evolution with magnetic field of the single-particle energy levels high up in the energy spectrum of one dot as probed by the ground state of the adjacent dot in a weakly coupled vertical quantum dot molecule. We find that the observed spectrum is generally well accounted for by the calculated spectrum for a two-dimensional elliptical parabolic confining potential, except in several regions where two or more single-particle levels approach each other. We focus on two two-level crossing regions which show unexpected anti-crossing behavior and contrasting current dependences. Within a simple coherent level mixing picture, we can model the current carried through the coupled states of the probed dot provided the intrinsic variation with magnetic field of the current through the states (as if they were uncoupled) is accounted for by an appropriate interpolation scheme.Comment: 4 pages, 4 figures, accepted for publication in Physica E in MSS 13 conference proceeding

Spin-accumulation in small ferromagnetic double barrier junctions

The non-equilibrium spin accumulation in ferromagnetic double barrier junctions is shown to govern the transport in small structures. Transport properties of such systems are described by a generalization of the theory of the Coulomb blockade. The spin accumulation enhances the magnetoresistance. The transient non-linear transport properties are predicted to provide a unique experimental evidence of the spin-accumulation in the form of a reversed current on time scales of the order of the spin-flip relaxation time.Comment: 4 pages, 3 figures, to appear in PR

Resistive detection of the Néel temperature of Cr₂O₃ thin films

Although bulk magnetic properties of various antiferromagnets have been vigorously studied since long ago, their properties in the form of thin films, which are more relevant to antiferromagnetic spintronic devices, have not been investigated as much. In this work, we characterized the Néel temperature of Cr₂O₃ thin films by investigating the temperature dependence of the spin Hall magnetoresistance in Cr₂O₃/Pt bilayers. A precise determination of the Néel temperature was made possible by carefully designing the direction of the magnetic anisotropy in Cr₂O₃. The results provide a reliable way to determine the Néel temperature of antiferromagnetic thin films.Tatsuya Iino, Takahiro Moriyama, Hiroyuki Iwaki, Hikaru Aono, Yu Shiratsuchi, and Teruo Ono, Appl. Phys. Lett. 114, 022402 (2019); https://doi.org/10.1063/1.5082220