390 research outputs found
Radiative decay effects influence the local electromagnetic response of the monolayer graphene with surface corrugations in terahertz range
We continue the study of surface corrugations influence on the monolayer
graphene local electromagnetic response in terahertz range we started earlier.
The effects of radiative decay, double-valley structure of charge carriers
spectrum in graphene and the breathing surface curvature form induced synthetic
electric fields are taken into account. To fulfill this program the generalized
nonlinear self-consistent equation is obtained. In case of weak external
alternating electric field for the obtained equation in linear approximation on
the external electric field the exact solution is found. It shows that in this
case we get local dephasing in induced current paths depending on the surface
form . This theoretical result qualitatively explains the corresponding
experiments with local current patterns in graphene without using fully quantum
approach which is necessary for theoretical description of such phenomenon in
graphene nanoribbons. Besides the formulae obtained in the present paper could
become the basis of the new method of the imaging of surface corrugations form
for given picture of local current paths. The obtained results allow to study
mechanical behavior of materials at nanoscale deviates from macroscoping
established concepts and this is of particular importance for graphene
Alternative approach to computing transport coefficients: application to conductivity and Hall coefficient of hydrogenated amorphous silicon
We introduce a theoretical framework for computing transport coefficients for
complex materials. As a first example, we resolve long-standing inconsistencies
between experiment and theory pertaining to the conductivity and Hall mobility
for amorphous silicon and show that the Hall sign anomaly is a consequence of
localized states. Next, we compute the AC conductivity of amorphous
polyanaline. The formalism is applicable to complex materials involving defects
and band-tail states originating from static topological disorder and extended
states. The method may be readily integrated with current \textit{ab initio}
methods.Comment: 4 pages, 2 figures, submitted to Phys. Rev. Let
Comment on `Dynamical properties of small polarons'
We show that the conclusion on the breakdown of the standard small polaron
theory made recently by E.V. deMello and J. Ranninger (Phys. Rev. B 55, 14872
(1997)) is a result of an incorrect interpretation of the electronic and
vibronic energy levels of the two-site Holstein model. The small polaron
theory, when properly applied, agrees well with the numerical results of these
authors. Also we show that their attempt to connect the properties of the
calculated correlation functions with the features of the intersite electron
hopping is unsuccessful.Comment: To appear in Phys. Rev.
A Variational Approach to Nonlocal Exciton-Phonon Coupling
In this paper we apply variational energy band theory to a form of the
Holstein Hamiltonian in which the influence of lattice vibrations (optical
phonons) on both local site energies (local coupling) and transfers of
electronic excitations between neighboring sites (nonlocal coupling) is taken
into account. A flexible spanning set of orthonormal eigenfunctions of the
joint exciton-phonon crystal momentum is used to arrive at a variational
estimate (bound) of the ground state energy for every value of the joint
crystal momentum, yielding a variational estimate of the lowest polaron energy
band across the entire Brillouin zone, as well as the complete set of polaron
Bloch functions associated with this band. The variation is implemented
numerically, avoiding restrictive assumptions that have limited the scope of
previous assaults on the same and similar problems. Polaron energy bands and
the structure of the associated Bloch states are studied at general points in
the three-dimensional parameter space of the model Hamiltonian (electronic
tunneling, local coupling, nonlocal coupling), though our principal emphasis
lay in under-studied area of nonlocal coupling and its interplay with
electronic tunneling; a phase diagram summarizing the latter is presented. The
common notion of a "self-trapping transition" is addressed and generalized.Comment: 33 pages, 11 figure
Disorder-driven superconductor-normal metal phase transition in quasi-one-dimensional organic conductors
Effects of non-magnetic disorder on the critical temperature T_c and on
diamagnetism of quasi-one-dimensional superconductors are reported. The energy
of Josephson-coupling between wires is considered to be random, which is
typical for dirty organic superconductors. We show that this randomness
destroys phase coherence between wires and that T_c vanishes discontinuously at
a critical disorder-strength. The parallel and transverse components of the
penetration-depth are evaluated. They diverge at different critical
temperatures T_c^{(1)} and T_c, which correspond to pair-breaking and
phase-coherence breaking respectively. The interplay between disorder and
quantum phase fluctuations is shown to result in quantum critical behavior at
T=0, which manifests itself as a superconducting-normal metal phase transition
of first-order at a critical disorder strength.Comment: 12 pages, 3 figure
Effects of the electron-phonon coupling near and within the insulating Mott phase
The role of the electron-phonon interaction in the Holstein-Hubbard model is
investigated in the metallic phase close to the Mott transition and in the
insulating Mott phase. The model is studied by means of a variational slave
boson technique. At half-filling, mean-field static quantities are in good
agreement with the results obtained by numerical techniques. By taking into
account gaussian fluctuations, an analytic expression of the spectral density
is derived in the Mott insulating phase showing that an increase of the
electron-phonon coupling leads to a sensitive reduction of the Mott gap through
a reduced effective repulsion. The relation of the results with recent
experimental observations in strongly correlated systems is discussed.Comment: 4 pages, 4 figure
Optical properties of small polarons from dynamical mean-field theory
The optical properties of polarons are studied in the framework of the
Holstein model by applying the dynamical mean-field theory. This approach
allows to enlighten important quantitative and qualitative deviations from the
limiting treatments of small polaron theory, that should be considered when
interpreting experimental data. In the antiadiabatic regime, accounting on the
same footing for a finite phonon frequency and a finite electron bandwidth
allows to address the evolution of the optical absorption away from the
well-understood molecular limit. It is shown that the width of the multiphonon
peaks in the optical spectra depends on the temperature and on the frequency in
a way that contradicts the commonly accepted results, most notably in the
strong coupling case. In the adiabatic regime, on the other hand, the present
method allows to identify a wide range of parameters of experimental interest,
where the electron bandwidth is comparable or larger than the broadening of the
Franck-Condon line, leading to a strong modification of both the position and
the shape of the polaronic absorption. An analytical expression is derived in
the limit of vanishing broadening, which improves over the existing formulas
and whose validity extends to any finite-dimensional lattice. In the same
adiabatic regime, at intermediate values of the interaction strength, the
optical absorption exhibits a characteristic reentrant behavior, with the
emergence of sharp features upon increasing the temperature -- polaron
interband transitions -- which are peculiar of the polaron crossover, and for
which analytical expressions are provided.Comment: 16 pages, 6 figure
Luttinger-liquid-like transport in long InSb nanowires
Long nanowires of degenerate semiconductor InSb in asbestos matrix (wire
diameter is around 50 \AA, length 0.1 - 1 mm) were prepared. Electrical
conduction of these nanowires is studied over a temperature range 1.5 - 350 K.
It is found that a zero-field electrical conduction is a power function of the
temperature with the typical exponent .
Current-voltage characteristics of such nanowires are found to be nonlinear and
at sufficiently low temperatures follows the power law . It
is shown that the electrical conduction of these nanowires cannot be accounted
for in terms of ordinary single-electron theories and exhibits features
expected for impure Luttinger liquid. For a simple approximation of impure LL
as a pure one broken into drops by weak links, the estimated weak-link density
is around per cm.Comment: 5 pages, 2 figure
Polaron and bipolaron transport in a charge segregated state of doped strongly correlated 2D semiconductor
The 2D lattice gas model with competing short and long range interactions is
appliedused for calculation of the incoherent charge transport in the classical
strongly-correlated charge segregated polaronic state. We show, by means of
Monte-Carlo simulations, that at high temperature the transport is dominated by
hopping of the dissociated correlated polarons, where with thetheir mobility is
inversely proportional to the temperature. At the temperatures below the
clustering transition temperature the bipolaron transport becomes dominant. The
energy barrier for the bipolaron hopping is determined by the Coulomb effects
and is found to be lower than the barrier for the single-polaron hopping. This
leads to drastically different temperature dependencies of mobilities for
polarons and bipolarons at low temperatures
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