Energy transfer from intense laser pulse to dielectrics in time-dependent density functional theory

Energy transfer processes from a high-intensity ultrashort laser pulse to electrons in simple dielectrics, silicon, diamond, and $\alpha$-quartz are theoretically investigated by first-principles calculations based on time-dependent density functional theory (TDDFT). Dependences on frequency as well as intensity of the laser pulse are examined in detail, making a comparison with the Keldysh theory. Although the Keldysh theory reliably reproduces the main features of the TDDFT calculation, we find some deviations between results by the two theories. The origin of the differences is examined in detail

Random Wandering Around Homoclinic-like Manifolds in Symplectic Map Chain

We present a method to construct a symplecticity preserving renormalization group map of a chain of weakly nonlinear symplectic maps and obtain a general reduced symplectic map describing its long-time behaviour. It is found that the modulational instability in the reduced map triggers random wandering of orbits around some homoclinic-like manifolds, which is understood as the Bernoulli shifts.Comment: submitted to Prog. Theor. Phy

31P-nuclear magnetic resonance studies of intact plasmodia of Physarum polycephalum

Abstract31P-nuclear magnetic resonance spectra were obtained from intact plasmodial cells of Physarum polycephalum, where cytoplasmic streaming is generated by actin-myosin-ATP interaction. Several peaks were resolved and identified. They included ATP, ADP, orthophosphate and polyphosphates. Peaks for phosphocreatine, phosphoarginine or AMP were not detected. The intracellular pH and concentrations of ATP and free Mg2+ were estimated to be pH 6.9, 0.2–0.5 mM, and about 1 mM, respectively

The folate‐binding module of Thermus thermophilus cobalamin‐dependent methionine synthase displays a distinct variation of the classical TIM barrel: a TIM barrel with a `twist’

Peer Reviewedhttps://deepblue.lib.umich.edu/bitstream/2027.42/141455/1/ayd2kw5140.pd

Interaction of intense ultrashort laser pulses with solid targets: A systematic analysis using first-principles calculations

Intense ultrashort laser pulse irradiation of solid targets was systematically investigated at the first-principles level, both theoretically and computationally. In the method, the propagation of a pulsed light through a thin film is described by a one-dimensional Maxwell's equation, and the microscopic electronic motion at different positions in the film is described by employing first-principles time-dependent density functional theory (TDDFT). The method uses a coarse-graining approximation to couple light propagation and electronic motion, and is termed the multiscale Maxwell-TDDFT method. The reflectance, transmittance, and absorbance of pulsed light incident normally on thin films of 50-200 nm thickness were calculated for materials with different optical properties, such as aluminum (simple metal), graphite (semi-metal), silicon (small-gap dielectric), and quartz (wide-gap dielectric). Optical response transitions were explored as the light intensity shifted from the linear regime, represented by the dielectric function for weak light, to the extremely nonlinear regime, represented by plasma reflection under intense light conditions. Numerous mechanisms that depend on the laser pulse intensity and material type were found to contribute to these changes. These include multiphoton absorption, saturable absorption, sign change of the effective dielectric constant, and transition from quantum occupation to classical Boltzmann distribution. Thus, the calculations provide a unified understanding of the interaction of intense pulsed light with solids, occurring on an extremely short time scale.Comment: 17 pages, 6 figure

The Nature of the Stable Soft X-ray Emissions in Several Types of Active Galactic Nuclei Observed by Suzaku

To constrain the origin of the soft X-ray excess phenomenon seen in many active galactic nuclei, the intensity-correlated spectral analysis, developed by Noda et al. (2011b) for Markarian 509, was applied to wide-band (0.5-45 keV) Suzaku data of five representative objects with relatively weak reflection signature. They are the typical bare-nucleus type 1 Seyfert Fairall 9, the bright and typical type 1.5 Seyfert MCG-2-58-22, 3C382 which is one of the X-ray brightest broad line radio galaxies, the typical Seyfert-like radio loud quasar 4C+74.26, and the X-ray brightest radio quiet quasar MR2251-178. In all of them, soft X-ray intensities in energies below 3 keV were tightly correlated with that in 3-10 keV, but with significant positive offsets. These offsets, when calculated in finer energy bands, define a stable soft component in 0.5-3 keV. In each object, this component successfully explained the soft excess above a power-law fit. These components were interpreted in several alternative ways, including a thermal Comptonization component which is independent of the dominant power-law emission. This interpretation, considered physically most reasonable, is discussed from a viewpoint of Multi-Zone Comptonization, which was proposed for the black hole binary Cygnus X-1 (Makishima et al. 2008).Comment: 18 pages, 12 figures, 7 table