Femtosecond pulses and dynamics of molecular photoexcitation: RbCs example

We investigate the dynamics of molecular photoexcitation by unchirped femtosecond laser pulses using RbCs as a model system. This study is motivated by a goal of optimizing a two-color scheme of transferring vibrationally-excited ultracold molecules to their absolute ground state. In this scheme the molecules are initially produced by photoassociation or magnetoassociation in bound vibrational levels close to the first dissociation threshold. We analyze here the first step of the two-color path as a function of pulse intensity from the low-field to the high-field regime. We use two different approaches, a global one, the 'Wavepacket' method, and a restricted one, the 'Level by Level' method where the number of vibrational levels is limited to a small subset. The comparison between the results of the two approaches allows one to gain qualitative insights into the complex dynamics of the high-field regime. In particular, we emphasize the non-trivial and important role of far-from-resonance levels which are adiabatically excited through 'vertical' transitions with a large Franck-Condon factor. We also point out spectacular excitation blockade due to the presence of a quasi-degenerate level in the lower electronic state. We conclude that selective transfer with femtosecond pulses is possible in the low-field regime only. Finally, we extend our single-pulse analysis and examine population transfer induced by coherent trains of low-intensity femtosecond pulses.Comment: 25 pages, 12 figure

Dusty Cometary Globules in W5

We report the discovery of four dusty cometary tails around low mass stars in two young clusters belonging to the W5 star forming region. Fits to the observed emission profiles from 24 micron observations with the Spitzer Space Telescope give tail lifetimes < 30 Myr, but more likely < 5 Myr. This result suggests that the cometary phase is a short lived phenomenon, occurring after photoevaporation by a nearby O star has removed gas from the outer disk of a young low mass star (see also Balog et al. 2006; Balog et al. 2008).Comment: 11 pages, 3 figures. Accepted for publication to ApJ Letter

A Quantum-Proof Non-Malleable Extractor, With Application to Privacy Amplification against Active Quantum Adversaries

In privacy amplification, two mutually trusted parties aim to amplify the secrecy of an initial shared secret $X$ in order to establish a shared private key $K$ by exchanging messages over an insecure communication channel. If the channel is authenticated the task can be solved in a single round of communication using a strong randomness extractor; choosing a quantum-proof extractor allows one to establish security against quantum adversaries. In the case that the channel is not authenticated, Dodis and Wichs (STOC'09) showed that the problem can be solved in two rounds of communication using a non-malleable extractor, a stronger pseudo-random construction than a strong extractor. We give the first construction of a non-malleable extractor that is secure against quantum adversaries. The extractor is based on a construction by Li (FOCS'12), and is able to extract from source of min-entropy rates larger than $1/2$. Combining this construction with a quantum-proof variant of the reduction of Dodis and Wichs, shown by Cohen and Vidick (unpublished), we obtain the first privacy amplification protocol secure against active quantum adversaries

Efficient exploration of unknown indoor environments using a team of mobile robots

Whenever multiple robots have to solve a common task, they need to coordinate their actions to carry out the task efficiently and to avoid interferences between individual robots. This is especially the case when considering the problem of exploring an unknown environment with a team of mobile robots. To achieve efficient terrain coverage with the sensors of the robots, one first needs to identify unknown areas in the environment. Second, one has to assign target locations to the individual robots so that they gather new and relevant information about the environment with their sensors. This assignment should lead to a distribution of the robots over the environment in a way that they avoid redundant work and do not interfere with each other by, for example, blocking their paths. In this paper, we address the problem of efficiently coordinating a large team of mobile robots. To better distribute the robots over the environment and to avoid redundant work, we take into account the type of place a potential target is located in (e.g., a corridor or a room). This knowledge allows us to improve the distribution of robots over the environment compared to approaches lacking this capability. To autonomously determine the type of a place, we apply a classifier learned using the AdaBoost algorithm. The resulting classifier takes laser range data as input and is able to classify the current location with high accuracy. We additionally use a hidden Markov model to consider the spatial dependencies between nearby locations. Our approach to incorporate the information about the type of places in the assignment process has been implemented and tested in different environments. The experiments illustrate that our system effectively distributes the robots over the environment and allows them to accomplish their mission faster compared to approaches that ignore the place labels

ATLASGAL-selected massive clumps in the inner Galaxy: VI. Kinetic temperature and spatial density measured with formaldehyde

We aim to directly determine the kinetic temperature and spatial density with formaldehyde for the $\sim$100 brightest ATLASGAL-selected clumps at 870 $\mu$m representing various evolutionary stages of high-mass star formation. Ten transitions ($J$ = 3-2 and 4-3) of ortho- and para-H$_2$CO near 211, 218, 225, and 291 GHz were observed with the APEX 12 m telescope. Using non-LTE models with RADEX, we derive the gas kinetic temperature and spatial density using the measured p-H$_2$CO 3$_{21}$-2$_{20}$/3$_{03}$-2$_{02}$, 4$_{22}$-3$_{21}$/4$_{04}$-3$_{03}$, and 4$_{04}$-3$_{03}$/3$_{03}$-2$_{02}$ ratios. The gas kinetic temperatures derived from the p-H$_2$CO 3$_{21}$-2$_{20}$/3$_{03}$-2$_{02}$ and 4$_{22}$-3$_{21}$/4$_{04}$-3$_{03}$ line ratios are high, ranging from 43 to $>$300 K with an unweighted average of 91 $\pm$ 4 K. Deduced $T_{\rm kin}$ values from the $J$ = 3-2 and 4-3 transitions are similar. Spatial densities of the gas derived from the p-H$_2$CO 4$_{04}$-3$_{03}$/3$_{03}$-2$_{02}$ line ratios yield 0.6-8.3 $\times$ 10$^6$ cm$^{-3}$ with an unweighted average of 1.5 ($\pm$0.1) $\times$ 10$^6$ cm$^{-3}$. A comparison of kinetic temperatures derived from p-H$_2$CO, NH$_3$, and the dust emission indicates that p-H$_2$CO traces a distinctly higher temperature than the NH$_3$ (2,2)/(1,1) transitions and the dust, tracing heated gas more directly associated with the star formation process. The H$_2$CO linewidths are found to be correlated with bolometric luminosity and increase with the evolutionary stage of the clumps, which suggests that higher luminosities tend to be associated with a more turbulent molecular medium. It seems that the spatial densities measured with H$_2$CO do not vary significantly with the evolutionary stage of the clumps. However, averaged gas kinetic temperatures derived from H$_2$CO increase with time through the evolution of the clumps.Comment: Accepted for publication in A&

Systematic observation of tunneling field-ionization in highly excited Rb Rydberg atoms

Pulsed field ionization of high-$n$ (90 $\leq n \leq$ 150) manifold states in Rb Rydberg atoms has been investigated in high slew-rate regime. Two peaks in the field ionization spectra were systematically observed for the investigated $n$ region, where the field values at the lower peak do not almost depend on the excitation energy in the manifold, while those at the higher peak increase with increasing excitation energy. The fraction of the higher peak component to the total ionization signals increases with increasing $n$, exceeding 80% at $n$ = 147. Characteristic behavior of the peak component and the comparison with theoretical predictions indicate that the higher peak component is due to the tunneling process. The obtained results show for the first time that the tunneling process plays increasingly the dominant role at such highly excited nonhydrogenic Rydberg atoms.Comment: 8 pages, 5 figure

Decaying shock studies of phase transitions in MgOSiO2 systems: implications for the Super-Earths interiors

We report an experimental study of the phase diagrams of periclase (MgO), enstatite (MgSiO3) and forsterite (Mg2SiO4) at high pressures. We investigated with laser driven decaying shocks the pressure/temperature curves of MgO, MgSiO3 and Mg2SiO4 between 0.2-1.2 TPa, 0.12-0.5 TPa and 0.2-0.85 TPa respectively. A melting signature has been observed in MgO at 0.47 TPa and 9860 K, while no phase changes were observed neither in MgSiO3 nor in Mg2SiO4. An increasing of reflectivity of MgO, MgSiO3 and Mg2SiO4 liquids have been detected at 0.55 TPa -12 760 K, 0.15 TPa - 7540 K, 0.2 TPa - 5800 K, respectively. In contrast to SiO2, melting and metallization of these compounds do not coincide implying the presence of poor electrically conducting liquids close to the melting lines. This has important implications for the generation of dynamos in Super-earths mantles

User Experience Design for E-Voting: How mental models align with security mechanisms

This paper presents a mobile application for vote-casting and vote-verification based on the Selene e-voting protocol and explains how it was developed and implemented using the User Experience Design process. The resulting interface was tested with 38 participants, and user experience data was collected via questionnaires and semi-structured interviews on user experience and perceived security. Results concerning the impact of displaying security mechanisms on UX were presented in a complementary paper. Here we expand on this analysis by studying the mental models revealed during the interviews and compare them with theoretical security notions. Finally, we propose a list of improvements for designs of future voting protocols.Comment: E-Vote-ID 2019 TalTech Proceeding

Ultrathin Oxide Films by Atomic Layer Deposition on Graphene

In this paper, a method is presented to create and characterize mechanically robust, free standing, ultrathin, oxide films with controlled, nanometer-scale thickness using Atomic Layer Deposition (ALD) on graphene. Aluminum oxide films were deposited onto suspended graphene membranes using ALD. Subsequent etching of the graphene left pure aluminum oxide films only a few atoms in thickness. A pressurized blister test was used to determine that these ultrathin films have a Young's modulus of 154 \pm 13 GPa. This Young's modulus is comparable to much thicker alumina ALD films. This behavior indicates that these ultrathin two-dimensional films have excellent mechanical integrity. The films are also impermeable to standard gases suggesting they are pinhole-free. These continuous ultrathin films are expected to enable new applications in fields such as thin film coatings, membranes and flexible electronics.Comment: Nano Letters (just accepted