Structural behavior of uranium dioxide under pressure by LSDA+U calculations

The structural behavior of UO2 under high pressure up to 300GPa has been studied by first-principles calculations with LSDA+U approximation. The results show that a pressure-induced structural transition to the cotunnite-type (orthorhombic Pnma) phase occurs at 38GPa. It agrees well with the experimentally observed ~42 GPa. An isostructural transition following that is also predicted to take place from 80 to 130GPa, which has not yet been observed in experiments. Further high compression beyond 226GPa will result in a metallic and paramagnetic transition. It corresponds to a volume of 90A^3 per cell, in good agreement with a previous theoretical analysis in the reduction of volume required to delocalize 5f states.Comment: 10 pages, 8 figure

Big-Bang Nucleosynthesis with Unstable Gravitino and Upper Bound on the Reheating Temperature

We study the effects of the unstable gravitino on the big-bang nucleosynthesis. If the gravitino mass is smaller than \sim 10 TeV, primordial gravitinos produced after the inflation are likely to decay after the big-bang nucleosynthesis starts, and the light element abundances may be significantly affected by the hadro- and photo-dissociation processes as well as by the p n conversion process. We calculate the light element abundances and derived upper bound on the reheating temperature after the inflation. In our analysis, we calculate the decay parameters of the gravitino (i.e., lifetime and branching ratios) in detail. In addition, we performed a systematic study of the hadron spectrum produced by the gravitino decay, taking account of all the hadrons produced by the decay products of the gravitino (including the daughter superparticles). We discuss the model-dependence of the upper bound on the reheating temperature.Comment: 32 pages, 11 figure

A Start-Timing Detector for the Collider Experiment PHENIX at RHIC-BNL

We describe a start-timing detector for the PHENIX experiment at the relativistic heavy-ion collider RHIC. The role of the detector is to detect a nuclear collision, provide precise time information with an accuracy of 50ps, and determine the collision point along the beam direction with a resolution of a few cm. Technical challenges are that the detector must be operational in a wide particle-multiplicity range in a high radiation environment and a strong magnetic field. We present the performance of the prototype and discuss the final design of the detector.Comment: 12 pages, LaTeX, 9 gif and 4 ps figures. Submitted to NIM

Ab initio investigation on oxygen defect clusters in UO2+x

By first-principles LSDA+U calculations, we revealed that the current physical picture of defective uranium dioxide suggested solely by neutron diffraction analysis is unsatisfactory. An understanding based on quantum theory has been established as a thermodynamical competition among point defects and cuboctahedral cluster, which naturally interprets the puzzled origin of the asymmetric O' and O'' interstitials. It also gives a clear and consistent agreement with most available experimental data. Unfortunately, the observed high occupation of O'' site cannot be accounted for in this picture and is still a challenge for theoretical simulations.Comment: 4 pages, 3 figures, title change