718 research outputs found
Evolution of ferromagnetic circular dichroism coincident with magnetization and anomalous Hall effect in Co-doped rutile TiO2
Magnetic circular dichroism (MCD) of rutile Ti1-xCoxO2-d is systematically
examined with various x and d to reveal a phase diagram for the appearance of
ferromagnetism at higher carrier concentration and Co content. The phase
diagram exactly matches with that determined from anomalous Hall effect (AHE).
The magnetic field dependence of MCD also shows good coincidence with those of
the magnetization and AHE. The coincidence of these independent measurements
strongly suggests single and intrinsic ferromagnetic origin.Comment: 9 pages, 4 figure
Bulk and Surface Magnetization of Co atoms in Rutile Ti_[1-x]Co_xO_[2-delta] Thin Films Revealed by X-Ray Magnetic Circular Dichroism
We have studied magnetism in Ti_[1-x]Co_xO_[2-\delta] thin films with various
x and \delta by soft x-ray magnetic circular dichroism (XMCD) measurements at
the Co L_[2,3] absorption edges. The estimated ferromagnetic moment by XMCD was
0.15-0.24 \mu\beta/Co in the surface, while in the bulk it was 0.82-2.25
\mu\beta/Co, which is in the same range as the saturation magnetization of
1.0-1.5 \mu\beta/Co. Theseresults suggest that the intrinsic origin of the
erromagnetism. The smaller moment of Co atom at surface is an indication of a
magnetically dead layer of a few nm thick at the surface of the thin films.Comment: This Paper is accepted in J. of Phys: Conds. Matte
Magnetic oxide semiconductors
Magnetic oxide semiconductors, oxide semiconductors doped with transition
metal elements, are one of the candidates for a high Curie temperature
ferromagnetic semiconductor that is important to realize semiconductor
spintronics at room temperature. We review in this paper recent progress of
researches on various magnetic oxide semiconductors. The magnetization,
magneto-optical effect, and magneto-transport such as anomalous Hall effect are
examined from viewpoint of feasibility to evaluate the ferromagnetism. The
ferromagnetism of Co-doped TiO2 and transition metal-doped ZnO is discussed.Comment: 26 pages, 5 tables, 6 figure
Ultrafast optical control of magnetization in EuO thin films
All-optical pump-probe detection of magnetization precession has been
performed for ferromagnetic EuO thin films at 10 K. We demonstrate that the
circularly-polarized light can be used to control the magnetization precession
on an ultrafast time scale. This takes place within the 100 fs duration of a
single laser pulse, through combined contribution from two nonthermal
photomagnetic effects, i.e., enhancement of the magnetization and an inverse
Faraday effect. From the magnetic field dependences of the frequency and the
Gilbert damping parameter, the intrinsic Gilbert damping coefficient is
evaluated to be {\alpha} \approx 3\times10^-3.Comment: 5 pages, 3 figures, accepted for publication in Phys. Rev.
Signature of Carrier-Induced Ferromagnetism in Ti_{1-x}Co_{x}O_{2-delta}: Exchange Interaction Between High-Spin Co 2+ and the Ti 3d Conduction Band
X-ray photoemission spectroscopy measurements were performed on thin-film
samples of rutile Ti_{1-x}Co_{x}O_{2-delta} to reveal the electronic structure.
The Co 2p core level spectra indicate that the Co ions take the high-spin Co 2+
configuration, consistent with substitution on the Ti site. The high spin state
and the shift due to the exchange splitting of the conduction band suggest
strong hybridization between carriers in the Ti 3d t2g band and the t2g states
of the high-spin Co 2+. These observations support the argument that room
temperature ferromagnetism in Ti_{1-x}Co_{x}O_{2-delta} is intrinsic.Comment: 4 pages, 5 figures. Accepted for publication in Physical Review
Letter
X-ray Anomalous Scattering of Diluted Magnetic Oxide Semiconductors: Possible Evidence of Lattice Deformation for High Temperature Ferromagnetism
We have examined whether the Co ions crystallographically substitute on the
Ti sites in rutile and anatase Ti_{1-x}_{x}_{2-delta}K_{1-x}_{x}_{2-delta}_2_{1-x}_{x}$O thin films and
obtained direct evidence that the Co ions are indeed substituted on the Zn
sites.Comment: 5 pages, 4 figures, accepted in PR
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