28 research outputs found

    A Review of Research Progress on the Analytical Method of Large-<i>n</i> Detrital Zircon U-Pb Geochronology

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    BACKGROUND: Detrital zircon U-Pb geochronology is an important tool for identifying sedimentary provenance and determining the maximum depositional age. The numbers of grains for detrital zircon provenance investigations using laser-ablation inductively coupled-plasma mass spectrometer (LA-ICP-MS) typically range from 60 to 120. In this range, age components are commonly not identified from the sample aliquot. In order to improve the reliability of provenance investigation, analysis of more grains (n ≥ 300) or even the large-n aliquot with more than 1000 grains (n>1000) are required. The emergence of large-n detrital zircon U-Pb geochronology is challenging the methods of data measurement, reduction and evaluation.OBJECTIVES: To summarize the progress of measurement, data reduction and data evaluation of large-n detrital zircon U-Pb geochronology.METHODS: By summarizing the method innovation of domestic and foreign literature.RESULTS: Firstly, each measurement requires rapid acquisition of U and Pb isotope signals, which can be conducted by improving the transmission efficiency of aerosol. The "flat" signal acquisition time can be shortened or transformed to a "peak" signal mode for rapid measurement. Secondly, large-n data require efficient data reduction protocol or powerful software (e.g. iolite) to improve visualization and reduce the variability between inter-laboratory comparisons. For U-Pb data processing flow, several optimized methods are introduced for fractionation correction and propagating uncertainty. In addition, total integrated counts and linear regression correction are introduced to specially process "peak" signals. Thirdly, the new calculation method of U-Pb and Pb-Pb age discordance, such as using Aitchison concordia distance, makes data filtering more reasonable. Based on recent research progress, the future of automation and standardization of large-n detrital zircon U-Pb geochronology is discussed and advice on the selection of instruments and reduction software is provided.CONCLUSIONS:In the future, the development of large-n detrital zircon U-Pb geochronology has great prospects, and will play a greater role in the study of provenance tracing and stratigraphic dating

    Increasing Nitrogen Losses Due to Changing Food Consumption Patterns in Bayannur City, China

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    Increasing urbanization and affluence have led to changes in food consumption patterns. The application of nitrogen (N) fertilizers ensures food security but also leads to environmental pollution due to N losses, through processes such as acidification, eutrophication, and greenhouse gas emissions. To clarify whether changes in food consumption patterns could increase N losses and to explore sustainable food system pathways, this study integrated the Chinese Food System Dashboard and the Nutrient Flows in Food Chains, Environment and Resources Use model to quantify and compare the link between food consumption and N losses in different agricultural regions using a case study of Bayannur City in the Yellow River Basin from 2000 to 2016. During the study period, Bayannur’s food consumption pattern changed from a “high carbohydrate and pork pattern” to a “high fiber and herbivore pattern”, which represents a shift from low to high N consumption. The per-capita food consumption decreased by 11.55% from 425.41 kg cap−1, whereas the per-capita N losses increased by 12.42% from 35.60 kg N cap−1. The average share of the plant-oriented and animal-oriented food supply in these losses was 53.39% and 46.61%, respectively. There were differences in the food consumption patterns and N losses in Bayannur’s farming, farming–pastoral, and pastoral regions. The changes in N losses were most significant in the pastoral region. The N losses to the environment increased sharply by 112.33% from 22.75 g N cap−1 over the past 16 years. The low level of economic development in Bayannur resulted in a shift in the food consumption pattern to a high N consumption. Four measures to protect food security and reduce the food N cost were proposed: (1) increasing the wheat planting area and maintaining the existing corn one; (2) expanding the scale of high-quality alfalfa planting; (3) enhancing the area of oat grass and wheat replanting; and (4) using modern planting technology

    Altitudinal Difference of Growth–Climate Response Models in the Coniferous Forests of Southeastern Tibetan Plateau, China

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    Characterized as a climatologically sensitive region, the southeastern Tibetan Plateau (STP) is an ideal location for dendrochronological research. Here, five tree-ring width (TRW) chronologies were developed: three for Picea likiangensis along altitudinal gradients from 3600 to 4400 m a.s.l. and two for Sabina saltuaria and Abies squamata from 4200 m a.s.l. Significant differences in the growth rates and age composition of Picea likiangensis were observed at various elevation gradients. The chronology statistics (mean sensitivity, etc.) fluctuated with the elevation gradient. Picea likiangensis showed distinct growth patterns in response to climatic variability along the altitude gradient: the minimum temperature influenced tree growth at lower and middle altitudes, while higher altitudes were affected by precipitation. The radial growth of different tree species growing in the same region is controlled by the same climatic factors. Sabina saltuaria and Abies squamata exhibited similar growth responses to Picea likiangensis. Stand conditions (wind speeds, slope, and elevation) and biotic factors (the depth of root, forest type, tree age, and sensitivity) can partially explain why the ring width–climate relationships change with altitude

    A detailed East Asian monsoon history surrounding the ‘Mystery Interval’ derived from three Chinese speleothem records

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    The ‘Mystery Interval’ (MI, 17.5−14.5 ka) was the first stage of the last deglaciation, a key interval for understanding mechanisms of glacial–interglacial cycles. To elucidate possible causes of the MI, here we present three high-resolution, precisely dated oxygen-isotope records of stalagmites from Qingtian and Hulu Caves in China, reflecting changes in the East Asian summer monsoon (EASM) then. Based on well-established chronologies using precise 230Th dates and annual-band counting results, the two-cave δ18O profiles of ~ 7-yr resolution match well at decadal timescales. Both of the two-cave records document an abrupt weakening (2‰ of δ18O rise within 20 yr) in the EASM at ~ 16.1 ka, coinciding with the transition of the two-phased MI reconstructed from New Mexico's Lake Estancia. Our results indicate that the maximum southward displacement of the Intertropical Convergence Zone and associated southward shift of polar jet stream may generate this two-phase feature of the MI during that time. We also discover a linear relationship among decreasing EASM intensity, rising atmospheric CO2 and weakening Atlantic Meridional Overturning Circulation between the MI and Younger Dryas episodes, suggesting a strong coupling of atmospheric/oceanic circulations in response to the millennial-scale forcing, which in turn regulates global climate changes and carbon cycles

    Strong coupling of Asian Monsoon and Antarctic climates on sub-orbital timescales

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    There is increasing evidence that millennial-scale climate variability played an active role on orbital-scale climate changes, but the mechanism for this remains unclear. A 230Th-dated stalagmite δ18O record between 88 and 22 thousand years (ka) ago from Yongxing Cave in central China characterizes changes in Asian monsoon (AM) strength. After removing the 65°N insolation signal from our record, the δ18O residue is strongly anti-phased with Antarctic temperature variability on sub-orbital timescales during the Marine Isotope Stage (MIS) 3. Furthermore, once the ice volume signal from Antarctic ice core records were removed and extrapolated back to the last two glacial-interglacial cycles, we observe a linear relationship for both short- and long-duration events between Asian and Antarctic climate changes. This provides the robust evidence of a link between northern and southern hemisphere climates that operates through changes in atmospheric circulation. We find that the weakest monsoon closely associated with the warmest Antarctic event always occurred during the Terminations. This finding, along with similar shifts in the opal flux record, suggests that millennial-scale events play a key role in driving the deglaciation through positive feedbacks associated with enhanced upwelling and increasing CO2.Published versio

    Early anthropogenic impacts on the Indian summer monsoon induced by land-use and land-cover changes

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    The impacts of anthropogenic forcing on Indian summer monsoon (ISM) rainfall are obscure, partly due to limited availability of highly resolved hydroclimate proxy records as well as the highly regionalized nature of precipitation. Here, we report an annually-resolved speleothem oxygen isotope record from Xianren Cave, southwestern China, which represents rainfall change over the broad ISM region. We find that the region has endured at least six decadal-scale weak monsoon events in the past three hundred years. One of them, lasting from the early to mid 19th century, shares the similar gradual, persistent trend as the most recent decline in ISM rainfall and both have a magnitude substantially larger than the others dominated by natural variability. This early weak monsoon event occurred during a historical time of intensive deforestation in the region. We conclude that the ISM trend could have been altered by the changes in land-use and land-cover since the early 19th century.Ministry of Education (MOE)National Research Foundation (NRF)Published versionWe are in debt to Dr. Ming Tan who initiated the research in Xianren Cave with a grant from the National Natural Science Foundation of China (NSFC-41272204). This work has been possible thanks to the support by the Earth Observatory of Singapore via its funding from the National Research Foundation Singapore (NRF), the Singapore Ministry of Education (MOE) under the Research Centres of Excellence initiative. X. W. acknowledges the financial support from an MOE Tier 2 grant (MOE2019-T2-1-174) and an NRF grant (NRF2017NRF-NSFC001-047). U-Th dating at the High-Precision Mass Spectrometry and Environment Change Laboratory was supported by grants from the Science Vanguard Research Program of the Ministry of Science and Technology, Taiwan, ROC (109-2123-M-002-001 to C.-C.S.), the Higher Education Sprout Project of the Ministry of Education, Taiwan, ROC (109L901001 to C.-C.S.), and the National Taiwan University (110L8907 to C.-C.S.). K. L. acknowledges the financial support (SKLLQG1815) from State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, China

    Reconciliation of hydroclimate sequences from the Chinese Loess Plateauand low-latitude East Asian Summer Monsoon regions over thepast 14,500 years

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    We discuss replicated stalagmite &delta;18O records with interannual-to-multidecadal resolution from Lianhua Cave on the Chinese Loess Plateau to illustrate the precipitation history of the East Asian Summer Monsoon (EASM) region over the last 14.5 thousand years (ka BP, before 1950 CE, hereafter), and to re-evaluate the inconsistency in the proxy-inferred palaeoclimate time series in northern China. Agreement between the stalagmite &delta;18O from Lianhua and other caves from central-southern China indicates that regional climate changes after the Last Glacial were concurrent across mainland China, indicating that insolation was the primary factor controlling the evolution of the Asian Summer Monsoon (ASM). The stalagmite 18O enrichment of 2.5&permil; in the Younger Dryas and 1.7&permil; during the 8.2-ka BP event in Lianhua were larger than those in caves from central and southern China. The evidence suggests that different meridional responses of weak precipitation conditions in the ASM realm occurred during these two abrupt events, driven by high-latitude forcing in the Northern Hemisphere. The heterogeneous hydroclimate sequences in northern China inferred from different natural archives are most likely attributable to the complexity of the formations and/or some chronological uncertainty.</p
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