Theoretical analysis of spectral gain in a THz quantum cascade laser: prospects for gain at 1 THz

In a recent Letter [Appl. Phys. Lett. 82, 1015 (2003)], Williams et al. reported the development of a terahertz quantum cascade laser operating at 3.4 THz or 14.2 meV. We have calculated and analyzed the gain spectra of the quantum cascade structure described in their work, and in addition to gain at the reported lasing energy of ~= 14 meV, we have discovered substantial gain at a much lower energy of around 5 meV or just over 1 THz. This suggests an avenue for the development of a terahertz laser at this lower energy, or of a two-color terahertz laser.Comment: in press APL, tentative publication date 29 Sep 200

Gain and Loss in Quantum Cascade Lasers

We report gain calculations for a quantum cascade laser using a fully self-consistent quantum mechanical approach based on the theory of nonequilibrium Green functions. Both the absolute value of the gain as well as the spectral position at threshold are in excellent agreement with experimental findings for T=77 K. The gain strongly decreases with temperature.Comment: 7 pages, 3 figures directly include

Positive Correlations in Tunneling through coupled Quantum Dots

Due to the Fermi-Dirac statistics of electrons the temporal correlations of tunneling events in a double barrier setup are typically negative. Here, we investigate the shot noise behavior of a system of two capacitively coupled quantum dot states by means of a Master equation model. In an asymmetric setup positive correlations in the tunneling current can arise due to the bunching of tunneling events. The underlying mechanism will be discussed in detail in terms of the current-current correlation function and the frequency-dependent Fano factor.Comment: HCIS 13 in Moden

Time Dependent Study of Multiple Exciton Generation in Nanocrystal Quantum Dots

We study the exciton dynamics in an optically excited nanocrystal quantum dot. Multiple exciton formation is more efficient in nanocrystal quantum dots compared to bulk semiconductors due to enhanced Coulomb interactions and the absence of conservation of momentum. The formation of multiple excitons is dependent on different excitation parameters and the dissipation. We study this process within a Lindblad quantum rate equation using the full many-particle states. We optically excite the system by creating a single high energy exciton $E_{SX}$ in resonance to a double exciton $E_{DX}$. With Coulomb electron-electron interaction, the population can be transferred from the single exciton to the double exciton state by impact ionisation (inverse Auger process). The ratio between the recombination processes and the absorbed photons provide the yield of the structure. We observe a quantum yield of comparable value to experiment assuming typical experimental conditions for a $4$ nm PbS quantum dot.Comment: 10 pages, 6 figures. Submitted to the conference "Progress in Nonequilibrium Green's Functions VI Proceedings" at Lund University, Sweden, August 17th - 21st, 2015. To be published in the Journal of Physics: Conference Serie

Transport in semiconductor superlattices: from quantum kinetics to terahertz-photon detectors

Semiconductor superlattices are interesting for two distinct reasons: the possibility to design their structure (band-width(s),doping, etc.) gives access to a large parameter space where different physical phenomena can be explored. Secondly, many important device applications have been proposed, and then subsequently successfully fabricated. A number of theoretical approaches has been used to describe their current-voltage characteristics, such as miniband conduction, Wannier-Stark hopping, and sequential tunneling. The choice of a transport model has often been dictated by pragmatic considerations without paying much attention to the strict domains of validity of the chosen model. In the first part of this paper we review recent efforts to map out these boundaries, using a first-principles quantum transport theory, which encompasses the standard models as special cases. In the second part, focusing in the mini-band regime, we analyze a superlattice device as an element in an electric circuit, and show that its performance as a THz-photon detector allows significant optimization, with respect to geometric and parasitic effects, and detection frequency. The key physical mechanism enhancing the responsivity is the excitation of hybrid Bloch-plasma oscillations.Comment: 22 pages, 10 figures, uses lamuphys.sty (included); to appear in the Proceedings of the XVI Sitges Conference, Statistical and Dynamical Aspects of Mesoscopic Systems (Lecture Notes in Physics, Springer

Microscopic modelling of perpendicular electronic transport in doped multiple quantum wells

We present a microscopic calculation of transport in strongly doped superlattices where domain formation is likely to occur. Our theoretical method is based on a current formula involving the spectral functions of the system, and thus allows, in principle, a systematic investigation of various interaction mechanisms. Taking into account impurity scattering and optical phonons we obtain a good quantitative agreement with existing experimental data from Helgesen and Finstad (J. Appl. Phys. 69, 2689, (1991)). Furthermore the calculated spectral functions indicate a significant increase of the average intersubband spacing compared to the bare level differences which might explain the experimental trend.Comment: 10 pages 5 figure

Simulation of Transport and Gain in Quantum Cascade Lasers

Quantum cascade lasers can be modeled within a hierarchy of different approaches: Standard rate equations for the electron densities in the levels, semiclassical Boltzmann equation for the microscopic distribution functions, and quantum kinetics including the coherent evolution between the states. Here we present a quantum transport approach based on nonequilibrium Green functions. This allows for quantitative simulations of the transport and optical gain of the device. The division of the current density in two terms shows that semiclassical transitions are likely to dominate the transport for the prototype device of Sirtori et al. but not for a recent THz-laser with only a few layers per period. The many particle effects are extremely dependent on the design of the heterostructure, and for the case considered here, inclusion of electron-electron interaction at the Hartree Fock level, provides a sizable change in absorption but imparts only a minor shift of the gain peak.Comment: 12 pages, 5 figures included, to appear in in "Advances in Solid State Physics", ed. by B. Kramer (Springer 2003