23 research outputs found

    Hidden Orbital Order in URu2Si2URu_{2}Si_{2}

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    When matter is cooled from high temperatures, collective instabilities develop amongst its constituent particles that lead to new kinds of order. An anomaly in the specific heat is a classic signature of this phenomenon. Usually the associated order is easily identified, but sometimes its nature remains elusive. The heavy fermion metal URu2Si2URu_2Si_2 is one such example, where the order responsible for the sharp specific heat anomaly at T0=17KT_0=17 K has remained unidentified despite more than seventeen years of effort. In URu2Si2URu_{2}Si_{2}, the coexistence of large electron-electron repulsion and antiferromagnetic fluctuations in URu2Si2URu_2Si_2 leads to an almost incompressible heavy electron fluid, where anisotropically paired quasiparticle states are energetically favored. In this paper we use these insights to develop a detailed proposal for the hidden order in URu2Si2URu_2Si_2. We show that incommensurate orbital antiferromagnetism, associated with circulating currents between the uranium ions, can account for the local fields and entropy loss observed at the 17K17 K transition; furthermore we make detailed predictions for neutron scattering measurements

    Magnetic field resonantly enhanced free spins in heavily underdoped YBa2Cu3O6+x

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    Using neutron scattering, we investigate the effect of a magnetic field on the static and dynamic spin response in heavily underdoped superconducting YBa2_{2}Cu3_{3}O6+x_{6+x} (YBCO6+x_{6+x}) with x=0.33 (Tc_{c}=8 K) and 0.35 (Tc_{c}=18 K). In contrast to the heavily doped and superconducting monolayer cuprates, the elastic central peak characterizing static spin correlations does not respond observably to a magnetic field which suppresses superconductivity. Instead, we find a magnetic field induced resonant enhancement of the spin fluctuations. The energy scale of the enhanced fluctuations matches the Zeeman energy within both the normal and vortex phases while the momentum dependence is the same as the zero field bilayer response. The magnitude of the enhancement is very similar in both phases with a fractional intensity change of (I/I0−1)∼0.1(I/I_{0}-1) \sim 0.1. We suggest that the enhancement is not directly correlated with superconductivity but is the result of almost free spins located near hole rich regions.Comment: (8 pages, 5 figures, submitted to Physical Review B

    Magnetic structures of Laves phase superlattices

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    The magnetic structure of Laves phase superlattices of structure [70/30]60, [150/100]50 and [50/70]60 were discussed. It was found that the [50/70]60 sample showed unexpected behavior because the moments aligned largely perpendicular to an applied field. The net moments on the DyFe2 and YFe2 layers were also discussed

    Multiphonon and Single-Particle Excitations in Quantum Crystals

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    Magnetic structures of Laves phase superlattices

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    The magnetic structure of Laves phase superlattices of structure [70/30]60, [150/100]50 and [50/70]60 were discussed. It was found that the [50/70]60 sample showed unexpected behavior because the moments aligned largely perpendicular to an applied field. The net moments on the DyFe2 and YFe2 layers were also discussed

    Evidence for decay of spin-waves above the pseudogap in underdoped YBa2Cu3O6.35

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    The magnetic spectrum at high-energies in heavily underdoped YBa2_{2}Cu3_{3}O6.35_{6.35} (Tc_{c}=18 K) has been determined throughout the Brillouin zone. At low-energy the scattering forms a cone of spin excitations emanating from the antiferromagnetic (0.5, 0.5) wave vector with an acoustic velocity similar to that of insulating cuprates. At high energy transfers, below the maximum energy of 270 meV at (0.5, 0), we observe zone boundary dispersion much larger and spectral weight loss more extensive than in insulating antiferromagnets. Moreover we report phenomena not found in insulators, an overall lowering of the zone-boundary energies and a large damping of ∼\sim 100 meV of the spin excitations at high-energies. The energy above which the damping occurs coincides approximately with the gap determined from transport measurements. We propose that as the energy is raised the spin excitations encounter an extra channel of decay into particle-hole pairs of a continuum that we associate with the pseudogap

    Quantum phase transitions in magnetism and superconductivity: Emergent spin topology seen with neutrons

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    Magnetic spins and charges interact strongly in high-temperature superconductors. New physics emerges as layers of copper oxide are tuned towards the boundary of the superconducting phase. As the pseudogap increases the characteristic spin excitation energy decreases. We show that our well-annealed YBa2Cu3O6+x (YBCO6+x) single crystals are orthorhombic and superconducting but not antiferromagnetically ordered. Near the critical concentration for superconductivity for x = 0.35 the spins fluctuate on two energy scales, one a relaxational spin response at ~2 meV and the other a slow central mode that is resolution-limited in energy (<0.08 meV) but broad in momentum. The gradual formation on cooling of a central mode over a range of momenta suggests that the spin ground state from which coherent superconducting pairing emerges may be quantum disordered. We show that YBCO6.35 adopts a homogeneous state that consists of highly-organized frozen sub-critical three-dimensional spin correlations. The continuous spin evolution indicates that a single quantum state occurs in contrast to claims from site-based probes that lightly doped YBCO undergoes a transition to antiferromagnetic Bragg order followed by a sharp transition to a cluster glass phase. For x = 0.35, where Tc = 18 K is reduced to 1/5 of Tcmax, the spin ground state is reached without a sharp transition and consists of short correlations extending over only 8 Angstrom between cells and 42 Angstrom within the planes. Polarized neutrons show the angular spin distribution to be isotropic unlike the AF insulator. Since moment is conserved we interpret this as evidence for hole-induced spin rotations rather than decay.Comment: Review of spin response in cuprate superconductors YBCO underdoped to suppress Tc based on talk at International Conference on Neutron Scattering, Sydney, Australia, Nov 27-Dec 2, 2005 6 pages 6 figure
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