17,584 research outputs found
Improved cosmological constraints on the curvature and equation of state of dark energy
We apply the Constitution compilation of 397 supernova Ia, the baryon
acoustic oscillation measurements including the parameter, the distance
ratio and the radial data, the five-year Wilkinson microwave anisotropy probe
and the Hubble parameter data to study the geometry of the universe and the
property of dark energy by using the popular Chevallier-Polarski-Linder and
Jassal-Bagla-Padmanabhan parameterizations. We compare the simple
method of joined contour estimation and the Monte Carlo Markov chain method,
and find that it is necessary to make the marginalized analysis on the error
estimation. The probabilities of and in the
Chevallier-Polarski-Linder model are skew distributions, and the marginalized
errors are ,
, , and
. For the Jassal-Bagla-Padmanabhan model, the
marginalized errors are ,
, , and
. The equation of state parameter of dark energy
is negative in the redshift range at more than level.
The flat CDM model is consistent with the current observational data
at the level.Comment: 10 figures, 12 pages, Classical and Quantum Gravity in press; v2 to
match the pulished versio
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Study of quasi-distributed optical fiber methane sensors based on laser absorption spectrometry
The coal industry plays an important role in the economic development of China. With the increase of coal mining year by year, coal mine accidents caused by gas explosion also occur frequently, which poses a serious threat to the life safety of absenteeism and national property safety. Therefore, high-precision methane fiber sensor is of great significance to ensure coal mine safety. This paper mainly introduces two kinds of quasi-distributed gas optical fiber sensing systems based on laser absorption spectroscopy. The gas fiber optic sensor based on absorption spectrum has high measurement accuracy, fast response and long service life. One is quasi-distributed optical fiber sensing system based on spatial division multiplexing (SDM) technology and the other is quasi-distributed optical fiber sensing system based on optical time domain reflection and time division multiplexing(TDM) technology
Oxygen reduction reaction activity in non-precious single-atom (M–N/C ) catalysts-contribution of metal and carbon/nitrogen framework-based sites.
We examine the performance of a number of single-atom M-N/C electrocatalysts with a common structure in order to deconvolute the activity of the framework N/C support from the metal M-N4 sites in M-N/Cs. The formation of the N/C framework with coordinating nitrogen sites is performed using zinc as a templating agent. After the formation of the electrically conducting carbon-nitrogen metal-coordinating network, we (trans)metalate with different metals producing a range of different catalysts (Fe-N/C, Co-N/C, Ni-N/C, Sn-N/C, Sb-N/C, and Bi-N/C) without the formation of any metal particles. In these materials, the structure of the carbon/nitrogen framework remains unchanged-only the coordinated metal is substituted. We assess the performance of the subsequent catalysts in acid, near-neutral, and alkaline environments toward the oxygen reduction reaction (ORR) and ascribe and quantify the performance to a combination of metal site activity and activity of the carbon/nitrogen framework. The ORR activity of the carbon/nitrogen framework is about 1000-fold higher in alkaline than it is in acid, suggesting a change in mechanism. At 0.80 VRHE, only Fe and Co contribute ORR activity significantly beyond that provided by the carbon/nitrogen framework at all pH values studied. In acid and near-neutral pH values (pH 0.3 and 5.2, respectively), Fe shows a 30-fold improvement and Co shows a 5-fold improvement, whereas in alkaline pH (pH 13), both Fe and Co show a 7-fold improvement beyond the baseline framework activity. The site density of the single metal atom sites is estimated using the nitrite adsorption and stripping method. This method allows us to deconvolute the framework sites and metal-based active sites. The framework site density of catalysts is estimated as 7.8 × 1018 sites g-1. The metal M-N4 site densities in Fe-N/C and Co-N/C are 9.4 × 1018 sites-1 and 4.8 × 1018 sites g-1, respectively
Impact of elevated precipitation, nitrogen deposition and warming on soil respiration in a temperate desert
Abstract. Soil respiration (Rs) is the most important source of carbon
dioxide emissions from soil to atmosphere. However, it is unclear what the
interactive response of Rs would be to environmental changes such
as elevated precipitation, nitrogen (N) deposition and warming, especially in
unique temperate desert ecosystems. To investigate this an in situ field
experiment was conducted in the Gurbantunggut Desert, northwest China, from
September 2014 to October 2016. The results showed that precipitation and N
deposition significantly increased Rs, but warming decreased
Rs, except in extreme precipitation events, which was mainly
through its impact on the variation of soil moisture at 5 cm depth. In
addition, the interactive response of Rs to combinations of the
factors was much less than that of any single-factor, and the main response
was a positive effect, except for the response from the interaction of
increased precipitation and high N deposition
(60 kg N ha−1 yr−1). Although Rs was found to show
a unimodal change pattern with the variation of soil moisture, soil
temperature and soil NH4+-N content, and it was significantly
positively correlated to soil dissolved organic carbon (DOC) and pH, a
structural equation model found that soil temperature was the most important
controlling factor. Those results indicated that Rs was mainly
interactively controlled by the soil multi-environmental factors and soil
nutrients, and was very sensitive to elevated precipitation, N deposition and
warming. However, the interactions of multiple factors largely reduced
between-year variation of Rs more than any single-factor,
suggesting that the carbon cycle in temperate deserts could be profoundly
influenced by positive carbon–climate feedback.
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Phase Control of Nonadiabaticity-induced Quantum Chaos in An Optical Lattice
The qualitative nature (i.e. integrable vs. chaotic) of the translational
dynamics of a three-level atom in an optical lattice is shown to be
controllable by varying the relative laser phase of two standing wave lasers.
Control is explained in terms of the nonadiabatic transition between optical
potentials and the corresponding regular to chaotic transition in mixed
classical-quantum dynamics. The results are of interest to both areas of
coherent control and quantum chaos.Comment: 3 figures, 4 pages, to appear in Physical Review Letter
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