Separation of Spin and Charge Quantum Numbers in Strongly Correlated Systems

In this paper we reexamine the problem of the separation of spin and charge degrees of freedom in two dimensional strongly correlated systems. We establish a set of sufficient conditions for the occurence of spin and charge separation. Specifically, we discuss this issue in the context of the Heisenberg model for spin-1/2 on a square lattice with nearest ($J_1$) and next-nearest ($J_2$) neighbor antiferromagnetic couplings. Our formulation makes explicit the existence of a local SU(2) gauge symmetry once the spin-1/2 operators are replaced by bound states of spinons. The mean-field theory for the spinons is solved numerically as a function of the ratio $J_2/J_1$ for the so-called s-RVB Ansatz. A second order phase transition exists into a novel flux state for $J_2/J_1>(J_2/J_1)_{{\rm cr}}$. We identify the range $0<J_2/J_1<(J_2/J_1)_{\rm cr}$ as the s-RVB phase. It is characterized by the existence of a finite gap to the elementary excitations (spinons) and the breakdown of all the continuous gauge symmetries. An effective continuum theory for the spinons and the gauge degrees of freedom is constructed just below the onset of the flux phase. We argue that this effective theory is consistent with the deconfinement of the spinons carrying the fundamental charge of the gauge group. We contrast this result with the study of the one dimensional quantum antiferromagnet within the same approach. We show that in the one dimensional model, the spinons of the gauge picture are always confined and thus cannot be identified with the gapless spin-1/2 excitations of the quantum antiferromagnet Heisenberg model.Comment: 56 pages, RevteX 3.

The mechanism of spin and charge separation in one dimensional quantum antiferromagnets

We reconsider the problem of separation of spin and charge in one dimensional quantum antiferromagnets. We show that spin and charge separation in one dimensional strongly correlated systems cannot be described by the slave boson or fermion representation within any perturbative treatment of the interactions between the slave holons and slave spinons. The constraint of single occupancy must be implemented exactly. As a result the slave fermions and bosons are not part of the physical spectrum. Instead, the excitations which carry the separate spin and charge quantum numbers are solitons. To prove this {\it no-go} result, it is sufficient to study the pure spinon sector in the slave boson representation. We start with a short-range RVB spin liquid mean-field theory for the frustrated antiferromagnetic spin-${1\over2}$ chain. We derive an effective theory for the fluctuations of the Affleck-Marston and Anderson order parameters. We show how to recover the phase diagram as a function of the frustration by treating the fluctuations non-perturbatively.Comment: 53 pages; Revtex 3.

Dispersion of the second-order nonlinear susceptibility in ZnTe, ZnSe, and ZnS

We have measured the absolute values of the second-harmonic generation (SHG) coefficient |d| for the zinc-blende II-VI semiconductors ZnTe, ZnSe, and ZnS at room temperature. The investigated spectral region of the fundamental radiation λF ranges from 520 to 1321 nm using various pulsed laser sources. In the transparent region of the II-VI semiconductors, the SHG coefficient exceeds the values of birefringent materials as ammonium dihydrogen phosphate (ADP) and potassium dihydrogen phosphate (KDP) by one or two orders of magnitudes. Above the E0 band gap a strong dispersion of |d| is observed, showing a maximum for a second-harmonic frequency close to the E1 gap. The experimental results are compared to calculated values using a simple three-band model including spin-orbit splitting. Substantial agreement is found to the experimentally observed dispersion of the second-order nonlinear susceptibility