Sensor Development for Single-Photon Thermoelectric Detectors

As we reported earlier [1], thermoelectric detectors can be competitive as nondispersive energy resolving focal-plane instruments in X-ray/UV spectrum. The first generations of prototype devices demonstrated the viability of detector design and provided good agreement between theoretical expectations and experimental data. These devices exploited sensors made of gold with a small fraction of iron impurity. To get the projected high resolution one needs another type of material, namely, lanthanum-cerium hexaborides. We report on the first experimental tests of the feasibility of lanthanum-cerium films as sensor materials. Progress with thin films of these materials argues for the success of these thermoelectric detectors

Voltage Responses to Optical Pulses of Unbiased Normal and Superconducting Samples

The direct transformation of the energy of an incident high-energy photon into a measurable potential difference within an absorbing metal is investigated. Experimental evidence is presented that the effect arises from the inherent energy dependence of the electronic density of states, rather than from a simple temperature excursion. The similarities between the results on Al and YBa2Cu3O7 samples indicate that the effect is universal in nature. We assert it may be used as the basis of a fast, energy resolving, individual photon detector for the ultraviolet radiation and x-rays

Luminescence spectra and kinetics of disordered solid solutions

We have studied both theoretically and experimentally the luminescence spectra and kinetics of crystalline, disordered solid solutions after pulsed excitation. First, we present the model calculations of the steady-state luminescence band shape caused by recombination of excitons localized in the wells of random potential induced by disorder. Classification of optically active tail states of the main exciton band into two groups is proposed. The majority of the states responsible for the optical absorption corresponds to the group of extended states belonging to the percolation cluster, whereas only a relatively small group of “radiative” states forms the steady-state luminescence band. The continuum percolation theory is applied to distinguish the “radiative” localized states, which are isolated in space and have no ways for nonradiative transitions along the tail states. It is found that the analysis of the exciton-phonon interaction gives the information about the character of the localization of excitons. We have shown that the model used describes quite well the experimental cw spectra of CdS(1−c)Sec and ZnSe(1−c)Tec solid solutions. Further, the experimental results are presented for the temporal evolution of the luminescence band. It is shown that the changes of band shape with time come from the interplay of population dynamics of extended states and spatially isolated “radiative” states. Finally, the measurements of the decay of the spectrally integrated luminescence intensity at long delay times are presented. It is shown that the observed temporal behavior can be described in terms of relaxation of separated pairs followed by subsequent exciton formation and radiative recombination. Electron tunneling processes are supposed to be responsible for the luminescence in the long-time limit at excitation below the exciton mobility edge. At excitation by photons with higher energies the diffusion of electrons can account for the observed behavior of the luminescence