Retrieval of target structure information from laser-induced photoelectrons by few-cycle bicircular laser fields

Citation: Hoang, V. H., Le, V. H., Lin, C. D., & Le, A. T. (2017). Retrieval of target structure information from laser-induced photoelectrons by few-cycle bicircular laser fields. Physical Review A, 95(3), 6. doi:10.1103/PhysRevA.95.031402By analyzing theoretical results from a numerical solution of the time-dependent Schrodinger equation for atoms in few-cycle bicircular laser pulses, we show that high-energy photoelectron momentum spectra can be used to extract accurate elastic scattering differential cross sections of the target ion with free electrons. We find that the retrieval range for a scattering angle with bicircular pulses is wider than with linearly polarized pulses, although the retrieval method has to be modified to account for different returning directions of the electron in the continuum. This result can be used to extend the range of applicability of ultrafast imaging techniques such as laser-induced electron diffraction and for the accurate characterization of laser pulses

Retrieval of interatomic separations of molecules from laser-induced high-order harmonic spectra

We illustrate an iterative method for retrieving the internuclear separations of N$_2$, O$_2$ and CO$_2$ molecules using the high-order harmonics generated from these molecules by intense infrared laser pulses. We show that accurate results can be retrieved with a small set of harmonics and with one or few alignment angles of the molecules. For linear molecules the internuclear separations can also be retrieved from harmonics generated using isotropically distributed molecules. By extracting the transition dipole moment from the high-order harmonic spectra, we further demonstrated that it is preferable to retrieve the interatomic separation iteratively by fitting the extracted dipole moment. Our results show that time-resolved chemical imaging of molecules using infrared laser pulses with femtosecond temporal resolutions is possible.Comment: 14 pages, 9 figure

Theoretical analysis of dynamic chemical imaging with lasers using high-order harmonic generation

We report theoretical investigations of the tomographic procedure suggested by Itatani {\it et al.} [Nature, {\bf 432} 867 (2004)] for reconstructing highest occupied molecular orbitals (HOMO) using high-order harmonic generation (HHG). Using the limited range of harmonics from the plateau region, we found that under the most favorable assumptions, it is still very difficult to obtain accurate HOMO wavefunction, but the symmetry of the HOMO and the internuclear separation between the atoms can be accurately extracted, especially when lasers of longer wavelengths are used to generate the HHG. We also considered the possible removal or relaxation of the approximations used in the tomographic method in actual applications. We suggest that for chemical imaging, in the future it is better to use an iterative method to locate the positions of atoms in the molecule such that the resulting HHG best fits the macroscopic HHG data, rather than by the tomographic method.Comment: 13 pages, 14 figure

Retrieval of material properties of monolayer transition-metal dichalcogenides from magnetoexciton energy spectra

Reduced exciton mass, polarizability, and dielectric constant of the surrounding medium are essential properties for semiconduction materials, and they can be extracted recently from the magnetoexciton energies. However, the acceptable accuracy of the previously suggested method requires very high magnetic intensity. Therefore, in the present paper, we propose an alternative method of extracting these material properties from recently available experimental magnetoexciton s-state energies in monolayer transition-metal dichalcogenides (TMDCs). The method is based on the high sensitivity of exciton energies to the material parameters in the Rytova-Keldysh model. It allows us to vary the considered material parameters to get the best fit of the theoretical calculation to the experimental exciton energies for the $1s$, $2s$, and $3s$ states. This procedure gives values of the exciton reduced mass and 2D polarizability. Then, the experimental magnetoexciton spectra compared to the theoretical calculation gives also the average dielectric constant. Concrete applications are presented only for monolayers WSe$_2$ and WS$_2$ from the recently available experimental data. However, the presented approach is universal and can be applied to other monolayer TMDCs. The mentioned fitting procedure requires a fast and effective method of solving the Schr\"{o}dinger of an exciton in monolayer TMDCs with a magnetic field. Therefore, we also develop such a method in this study for highly accurate magnetoexciton energies.Comment: 8 pages, 4 figures, 4 table

Low dietary intakes of essential nutrients during pregnancy in Vietnam

Inadequate intake of nutrients during pregnancy has been associated with poor pregnancy and infant outcomes; however, evidence remains limited in low-resource settings in Asia. This paper assessed food, macronutrient, and micronutrient intakes among 1944 Vietnamese pregnant women. Dietary information was collected via an interviewer-administered food frequency questionnaire, and nutrient intakes were estimated using the Vietnamese food composition tables. The levels of nutrient intakes were evaluated against the Vietnamese recommended nutrient intakes (RNI) for pregnancy. The diet profiles were reported as means and percentages. The average daily food intakes across socio-demographic factors were compared using ANOVA, with adjustment for multiple comparisons by the Tukey–Kramer test. Rice, fruits, and vegetables were the main food sources consumed. The mean energy intake was 2004 kcal/day with 15.9%, 31.8%, and 52.2% of energy deriving from proteins, fats, and carbohydrates, respectively. Just over half of the women did not meet the RNI for total energy intake. The intakes of essential micronutrients including folate, calcium, iron, and zinc were below the RNI, and almost all pregnant women failed to meet the recommendations for these micronutrients. The associations of maternal age, education, and pre-pregnancy body mass index with nutrient intakes varied across the nutrient subgroups. Targeted programs are needed to improve nutrient intakes in Vietnamese pregnant women

Wigner-Seitz cells in neutron star crust with finite range interactions

The structure of Wigner-Seitz cells in the inner crust of neutron stars is investigated using a microcospic Hartree-Fock-BCS approach with finite range D1S and M3Y-P4 interactions. Large effects on the densities are found compared to previous predictions using Skyrme interactions. Pairing effects are found to be small, and they are attenuated by the use of finite range interactions in the mean field.Comment: 11 pages, 5 figure

Evaluating the impacts of rice-based protection dykes on floodwater dynamics in the vietnamese mekong delta using geographical impact factor (Gif)

This study aims at evaluating the geographical influences of rice-based protection dykes on floodwater regimes along the main rivers, namely the Mekong and the Bassac, in the Vietnamese Mekong Delta (VMD). Specifically, numerous low dykes and high dykes have been constructed particularly in the upper delta’s floodplains to protect the double and triple rice cropping against the annual flooding. For the whole deltaic domain, a 1D-quasi-2D hydrodynamic model setup was used to simulate seventy-two (72) scenarios of dyke construction development in the context of low, medium, and high floods that occurred in the VMD to examine the effects of different flood magnitudes on a certain dyke construction area. Based on the model simulation results, we established an evaluation indicator, the so-called Geographical Impact Factor (GIF), to evaluate the impacts of zone-based dyke compartments on the floodwater regimes along the main rivers for different kinds of floods. Our findings revealed different rates of influences on the floodwater levels along the Mekong and Bassac Rivers under different scenarios of zone-based high-dyke developments. GIF is a useful index for scientists and decision-makers in land use planning, especially in rice intensification, in conjunction with flood management for the VMD and for similar deltas worldwide

Characterization of Single-Shot Attosecond Pulses with Angular Streaking Photoelectron Spectra

Most of the traditional attosecond pulse retrieval algorithms are based on a so-called attosecond streak camera technique, in which the momentum of the electron is shifted by an amount depending on the relative time delay between the attosecond pulse and the streaking infrared pulse. Thus, temporal information of the attosecond pulse is encoded in the amount of momentum shift in the streaked photoelectron momentum spectrogram S(p, τ), where p is the momentum of the electron along the polarization direction and τ is the time delay. An iterative algorithm is then employed to reconstruct the attosecond pulse from the streaking spectrogram. This method, however, cannot be applied to attosecond pulses generated from free-electron x-ray lasers where each single shot is different and stochastic in time. However, using a circularly polarized infrared laser as the streaking field, a two (or three)-dimensional angular streaking electron spectrum can be used to retrieve attosecond pulses for each shot, as well as the time delay with respect to the circularly polarized IR field. Here we show that a retrieval algorithm previously developed for the traditional streaking spectrogram can be modified to efficiently characterize single-shot attosecond pulses. The methods have been applied to retrieve 188 single shots from recent experiments. We analyze the statistical behavior of these 188 pulses in terms of pulse duration, bandwidth, pulse peak energy, and time delay with respect to the IR field. The retrieval algorithm is efficient and can be easily used to characterize a large number of shots in future experiments for attosecond pulses at free-electron x-ray laser facilities

A new kinetic model for biogas production from co-digestion by batch mode

Coming out from the growth kinetics, the Gompertz model has been developed and considered as the best one for simulating the biogas production from anaerobic digestion. However, the model has failed to describe the starting point of the process, and no-sense of lag phase constant has been pointed out. Thus, the goal of this study is to develop a new kinetic model of biogas production with meaningful constants that can alternate the Gompertz model. The kinetic constants of the model were determined by applying the least squares fitting method for experimental data. The experimental data were taken from running seven batch reactors of co-digestion of vegetable, sludge and horse manure under 37oC, pH of 6.7, and total solids of 2.5%. The result of the high coefficient of determination (0.9611-0.9906) demonstrated that the new biogas production kinetic model was feasible to simulate the biogas generation process. This finding has opened a new choice that can deal with simulation of the biogas production. Moreover, co-digestion of vegetable, horse manure, and sludge was also evaluated under strong attention. The biogas potential was in the range of 183-648 Nml/g-VS with the best carbon-to-nitrogen ratio of 16. Vegetable waste played a major role in producing the biogas yield while horse manure and sludge contributed to balancing nutrient of the digestion process. Also, the strong correlation between carbon-to-nitrogen ratio and kinetic constants confirmed that the carbon-to-nitrogen ratio was the key factor that influenced biogas generation

Deep LOFAR observations of the merging galaxy cluster CIZA J2242.8+5301

Previous studies have shown that CIZA J2242.8+5301 (the 'Sausage' cluster, z = 0.192) is a massive merging galaxy cluster that hosts a radio halo and multiple relics. In this paper, we present deep, high-fidelity, low-frequency images made with the LOw-Frequency Array (LOFAR) between 115.5 and 179 MHz. These images, with a noise of 140 μJy beam- 1 and a resolution of θbeam = 7.3 arcsec × 5.3 arcsec, are an order of magnitude more sensitive and five times higher resolution than previous low-frequency images of this cluster. We combined the LOFAR data with the existing Giant Metrewave Radio Telescope (GMRT) (153, 323, 608 MHz) and Westerbork Synthesis Radio Telescope (WSRT) (1.2, 1.4, 1.7, 2.3 GHz) data to study the spectral properties of the radio emission from the cluster. Assuming diffusive shock acceleration (DSA), we found Mach numbers of Mn=2.7{}_{-0.3}^{+0.6} and Ms=1.9_{-0.2}^{+0.3} for the northern and southern shocks. The derived Mach number for the northern shock requires an acceleration efficiency of several percent to accelerate electrons from the thermal pool, which is challenging for DSA. Using the radio data, we characterized the eastern relic as a shock wave propagating outwards with a Mach number of Me=2.4_{-0.3}^{+0.5}, which is in agreement with MeX=2.5{}_{-0.2}^{+0.6} that we derived from Suzaku data. The eastern shock is likely to be associated with the major cluster merger. The radio halo was measured with a flux of 346 ± 64 mJy at 145 MHz. Across the halo, we observed a spectral index that remains approximately constant (α ^{145 MHz-2.3 GHz}_{{across ˜ 1 Mpc}^2}=-1.01± 0.10) after the steepening in the post-shock region of the northern relic. This suggests a generation of post-shock turbulence that re-energies aged electrons