16 research outputs found
Magnetization steps in Zn_(1-x)Mn_xO: Four largest exchange constants and single-ion anisotropy
Magnetization steps (MST's) from Mn pairs in several single crystals of
Zn_(1-x)Mn_xO (0.0056<=x<=0.030, and in one powder (x=0.029), were observed.
The largest two exchange constants, J1/kB=-18.2+/-0.5K and J1'/kB=-24.3+/-0.6K,
were obtained from large peaks in the differential susceptibility, dM/dH,
measured in pulsed magnetic fields, H, up to 500 kOe. These two largest J's are
associated with the two inequivalent classes of nearest neighbors (NN's) in the
wurtzite structure. The 29% difference between J1 and J1' is substantially
larger than 13% in CdS:Mn, and 15% in CdSe:Mn. The pulsed-field data also
indicate that, despite the direct contact between the samples and a
superfluid-helium bath, substantial departures from thermal equilibrium
occurred during the 7.4 ms pulse. The third- and fourth-largest J's were
determined from the magnetization M at 20 mK, measured in dc magnetic fields H
up to 90 kOe. Both field orientations H||c and H||[10-10] were studied. (The
[10-10] direction is perpendicular to the c-axis, [0001].) By definition,
neighbors which are not NN's are distant neighbors (DN's). The largest DN
exchange constant (third-largest overall), has the value J/kB=-0.543+/-0.005K,
and is associated with the DN at r=c. Because this is not the closest DN, this
result implies that the J's do not decrease monotonically with the distance r.
The second-largest DN exchange constant (fourth-largest overall), has the value
J/kB=-0.080 K. It is associated with one of the two classes of neighbors that
have a coordination number z=12, but the evidence is insufficient for a
definite unique choice. The dependence of M on the direction of H gives
D/kB=-0.039+/-0.008K, in fair agreement with -0.031 K from earlier EPR work.Comment: 12 pages, 10 figures. Submitted to PR
Susceptibility Amplitude Ratios Near a Lifshitz Point
The susceptibility amplitude ratio in the neighborhood of a uniaxial Lifshitz
point is calculated at one-loop level using field-theoretic and
-expansion methods. We use the Schwinger parametrization of the
propagator in order to split the quadratic and quartic part of the momenta, as
well as a new special symmetry point suitable for renormalization purposes. For
a cubic lattice (d = 3), we find the result .Comment: 7 pages, late
Magnetization steps in a diluted Heisenberg antiferromagnetic chain: Theory and experiments on TMMC:Cd
A theory for the equilibrium low-temperature magnetization M of a diluted
Heisenberg antiferromagnetic chain is presented. The magnetization curve, M
versus B, is calculated using the exact contributions of finite chains with 1
to 5 spins, and the "rise and ramp approximation" for longer chains. Some
non-equilibrium effects that occur in a rapidly changing B, are also
considered. Specific non-equilibrium models based on earlier treatments of the
phonon bottleneck, and of spin flips associated with cross relaxation and with
level crossings, are discussed. Magnetization data on powders of TMMC diluted
with cadmium [i.e., (CH_3)_4NMn_xCd_(1-x)Cl_3, with 0.16<=x<=0.50 were measured
at 0.55 K in 18 T superconducting magnets. The field B_1 at the first MST from
pairs is used to determine the NN exchange constant, J, which changes from -5.9
K to -6.5 K as x increases from 0.16 to 0.50. The magnetization curves obtained
in the superconducting magnets are compared with simulations based on the
equilibrium theory. Data for the differential susceptibility, dM/dB, were taken
in pulsed magnetic fields (7.4 ms duration) up to 50 T, with the powder samples
in a 1.5 K liquid-helium bath. Non-equilibrium effects, which became more
severe as x decreased, were observed. The non-equilibrium effects are
tentatively interpreted using the "Inadequate Heat Flow Scenario," or to
cross-relaxation, and crossings of energy levels, including those of excited
states.Comment: 16 pages, 14 figure
Specific heat amplitude ratios for anisotropic Lifshitz critical behaviors
We determine the specific heat amplitude ratio near a -axial Lifshitz
point and show its universal character. Using a recent renormalization group
picture along with new field-theoretical -expansion techniques,
we established this amplitude ratio at one-loop order. We estimate the
numerical value of this amplitude ratio for and . The result is in
very good agreement with its experimental measurement on the magnetic material
. It is shown that in the limit it trivially reduces to the
Ising-like amplitude ratio.Comment: 8 pages, RevTex, accepted as a Brief Report in Physical Review
"Quasi two-dimensional" spin distributions in II-VI magnetic semiconductor heterostructures: Clustering and dimensionality
Spin clustering in diluted magnetic semiconductors (DMS) arises from
antiferromagnetic exchange between neighboring magnetic cations and is a strong
function of reduced dimensionality. Epitaxially-grown single monolayers and
abrupt interfaces of DMS are, however, never perfectly two-dimensional (2D) due
to the unavoidable inter-monolayer mixing of atoms during growth. Thus the
magnetization of DMS heterostructures, which is strongly modified by spin
clustering, is intermediate between that of 2D and 3D spin distributions. We
present an exact calculation of spin clustering applicable to arbitrary
distributions of magnetic spins in the growth direction. The results reveal a
surprising insensitivity of the magnetization to the form of the intermixing
profile, and identify important limits on the maximum possible magnetization.
High-field optical studies of heterostructures containing "quasi-2D" spin
distributions are compared with calculation.Comment: 5 pages (RevTeX), 5 embedded EPS figs, published in PRB v61 p1736
(2000
A new picture of the Lifshitz critical behavior
New field theoretic renormalization group methods are developed to describe
in a unified fashion the critical exponents of an m-fold Lifshitz point at the
two-loop order in the anisotropic (m not equal to d) and isotropic (m=d close
to 8) situations. The general theory is illustrated for the N-vector phi^4
model describing a d-dimensional system. A new regularization and
renormalization procedure is presented for both types of Lifshitz behavior. The
anisotropic cases are formulated with two independent renormalization group
transformations. The description of the isotropic behavior requires only one
type of renormalization group transformation. We point out the conceptual
advantages implicit in this picture and show how this framework is related to
other previous renormalization group treatments for the Lifshitz problem. The
Feynman diagrams of arbitrary loop-order can be performed analytically provided
these integrals are considered to be homogeneous functions of the external
momenta scales. The anisotropic universality class (N,d,m) reduces easily to
the Ising-like (N,d) when m=0. We show that the isotropic universality class
(N,m) when m is close to 8 cannot be obtained from the anisotropic one in the
limit d --> m near 8. The exponents for the uniaxial case d=3, N=m=1 are in
good agreement with recent Monte Carlo simulations for the ANNNI model.Comment: 48 pages, no figures, two typos fixe
Magnetic semiconductor quantum wells in high fields to 60 Tesla: Photoluminescence linewidth annealing at magnetization steps
Magnetic semiconductors offer a unique possibility for strongly tuning the intrinsic alloy disorder potential with applied magnetic field. We report the direct observation of a series of step-like reductions in the magnetic alloy disorder potential in single ZnSe/Zn(Cd,Mn)Se quantum wells between O and 60 Tesla. This disorder, measured through the linewidth of low temperature photoluminescence spectra drops abruptly at -19, 36, and 53 Tesla, in concert with observed magnetization steps. Conventional models of alloy disorder (developed for nonmagnetic semiconductors) reproduce the general shape of the data, but markedly underestimate the size of the linewidth reduction
2-(4,5,6,7-tetrafluorobenzimidazol-2-yl)-4,4,5,5-tetramethyl-4,5-dihydro-1H-imidazole-3-oxide-1-oxyl, a hydrogen-bonded organic quasi-1D ferromagnet
The title radical (F4BlmNN) is a stable nitronylnitroxide that forms hydrogen-bonded NH center dot center dot center dot ON chains in the solid state. The chains assemble the F4BlmNN molecules to form stacked contacts between the radical groups, in a geometry that is expected to exhibit ferromagnetic (FM) exchange based on spin polarization (SP) models. The experimental magnetic susceptibility of F4BlmNN confirms the expectation, showing 1-D Heisenberg chain FM exchange behavior over 1.8-300 K with an intrachain exchange constant Of J(chain)/k = +22 K. At lower temperatures, ac magnetic susceptibility and variable field heat capacity measurements show that F4BlmNN acts as a quasi-1-D ferromagnet. The dominant ferromagnetic exchange interaction is attributable to overlap between spin orbitals of molecules within the hydrogen-bonded chains, consistent with the SP model expectations. The chains appear to be antiferromagnetically exchange coupled, giving cusps in the ac susceptibility and zero field heat capacity at lower temperatures. The results indicate that the sample orders magnetically at about 0.7 K. The magnetic heat capacity ordering cusp shifts to lower temperatures as external magnetic field increases, consistent with forming a bulk antiferromagnetic phase below a Neel temperature of T-N(0) = 0.72 K, with a critical field of H-c approximate to 1800 Oe. The interchain exchange is estimated to be zJ/k congruent to (-)0.1 K