47 research outputs found
Phonons and Magnetic Excitations in Mott-Insulator LaTiO
The polarized Raman spectra of stoichiometric LaTiO (T K) were
measured between 6 and 300 K. In contrast to earlier report on half-metallic
LaTiO, neither strong background scattering, nor Fano shape of the
Raman lines was observed. The high frequency phonon line at 655 cm
exhibits anomalous softening below T: a signature for structural
rearrangement. The assignment of the Raman lines was done by comparison to the
calculations of lattice dynamics and the nature of structural changes upon
magnetic ordering are discussed. The broad Raman band, which appears in the
antiferromagnetic phase, is assigned to two-magnon scattering. The estimated
superexchange constant meV is in excellent agreement with the
result of neutron scattering studies.Comment: 4 pages, 5 figure
Self-trapped Exciton and Franck-Condon Spectra Predicted in LaMnO
Because the ground state has cooperative Jahn-Teller order, electronic
excitations in LaMnO are predicted to self-trap by local rearrangement of
the lattice. The optical spectrum should show a Franck-Condon series, that is,
a Gaussian envelope of vibrational sidebands. Existing data are reinterpreted
in this way. The Raman spectrum is predicted to have strong multiphonon
features.Comment: 5 pages with two embedded postscript figure
Calculation of the Coherent Synchrotron Radiation Impedance from a Wiggler
Most studies of Coherent Synchrotron Radiation (CSR) have only considered the
radiation from independent dipole magnets. However, in the damping rings of
future linear colliders, a large fraction of the radiation power will be
emitted in damping wigglers. In this paper, the longitudinal wakefield and
impedance due to CSR in a wiggler are derived in the limit of a large wiggler
parameter . After an appropriate scaling, the results can be expressed in
terms of universal functions, which are independent of . Analytical
asymptotic results are obtained for the wakefield in the limit of large and
small distances, and for the impedance in the limit of small and high
frequencies.Comment: 10 pages, 8 figure
Franck-Condon-Broadened Angle-Resolved Photoemission Spectra Predicted in LaMnO3
The sudden photohole of least energy created in the photoemission process is
a vibrationally excited state of a small polaron. Therefore the photoemission
spectrum in LaMnO3 is predicted to have multiple Franck-Condon vibrational
sidebands. This generates an intrinsic line broadening approximately 0.5 eV.
The photoemission spectral function has two peaks whose central energies
disperse with band width approximately 1.2 eV. Signatures of these phenomena
are predicted to appear in angle-resolved photoemission spectra.Comment: Revtex file 4 pages and 3 figure
Multi-phonon Resonant Raman Scattering Predicted in LaMnO3 from the Franck-Condon Process via Self-Trapped Excitons
Resonant behavior of the Raman process is predicted when the laser frequency
is close to the orbital excitation energy of LaMnO3 at 2 eV. The incident
photon creates a vibrationally excited self-trapped ``orbiton'' state from the
orbitally-ordered Jahn-Teller (JT) ground state. Trapping occurs by local
oxygen rearrangement. Then the Franck-Condon mechanism activates multiphonon
Raman scattering. The amplitude of the -phonon process is first order in the
electron-phonon coupling . The resonance occurs {\it via} a dipole forbidden
to transition. We previously suggested that this transition (also seen
in optical reflectivity) becomes allowed because of asymmetric oxygen
fluctuations. Here we calculate the magnitude of the corresponding matrix
element using local spin-density functional theory. This calculation agrees to
better than a factor of two with our previous value extracted from experiment.
This allows us to calculate the absolute value of the Raman tensor for
multiphonon scattering. Observation of this effect would be a direct
confirmation of the importance of the JT electron-phonon term and the presence
of self-trapped orbital excitons, or ``orbitons''.Comment: 8 pages and 3 embedded figures. The earlier short version is now
replaced by a more complete paper with a slightly different title. This
version includes a caculation by density-functional theory of the dipole
matrix element for exciting the self-trapped orbital exciton which activates
the multiphonon Raman signal
Strain effect on electronic transport and ferromagnetic transition temperature in LaSrMnO thin films
We report on a systematic study of strain effects on the transport properties
and the ferromagnetic transition temperature of high-quality
LaSrMnO thin films epitaxially grown on (100) SrTiO
substrates. Both the magnetization and the resistivity are critically dependent
on the film thickness. is enhanced with decreasing the film thickness
due to the compressive stain produced by lattice mismatch. The resistivity
above 165 K of the films with various thicknesses is consistent with small
polaronic hopping conductivity. The polaronic formation energy is
reduced with the decrease of film thickness. We found that the strain
dependence of mainly results from the strain-induced electron-phonon
coupling. The strain effect on is in good agreement with the
theoretical predictions.Comment: 6 pages and 5 figures, accepted for publication in Phys. Rev.
Electric dipole moments and the search for new physics
Static electric dipole moments of nondegenerate systems probe mass scales for
physics beyond the Standard Model well beyond those reached directly at high
energy colliders. Discrimination between different physics models, however,
requires complementary searches in atomic-molecular-and-optical, nuclear and
particle physics. In this report, we discuss the current status and prospects
in the near future for a compelling suite of such experiments, along with
developments needed in the encompassing theoretical framework.Comment: Contribution to Snowmass 2021; updated with community edits and
endorsement