Revealing the Exciton Fine Structure in PbSe Nanocrystal Quantum Dots

We measure the photoluminescence (PL) lifetime, $\tau$, of excitons in colloidal PbSe nanocrystals (NCs) at low temperatures to 270~mK and in high magnetic fields to 15~T. For all NCs (1.3-2.3~nm radii), $\tau$ increases sharply below 10~K but saturates by 500~mK. In contrast to the usual picture of well-separated ``bright" and ``dark" exciton states (found, e.g., in CdSe NCs), these dynamics fit remarkably well to a system having two exciton states with comparable - but small - oscillator strengths that are separated by only 300-900 $\mu$eV. Importantly, magnetic fields reduce $\tau$ below 10~K, consistent with field-induced mixing between the two states. Magnetic circular dichroism studies reveal exciton g-factors from 2-5, and magneto-PL shows $>$10\% circularly polarized emission.Comment: To appear in Physical Review Letter

Type Ia Supernova Scenarios and the Hubble Sequence

The dependence of the Type Ia supernova (SN Ia) rate on galaxy type is examined for three currently proposed scenarios: merging of a Chandrasekhar--mass CO white dwarf (WD) with a CO WD companion, explosion of a sub--Chandrasekhar mass CO WD induced by accretion of material from a He star companion, and explosion of a sub--Chandrasekhar CO WD in a symbiotic system. The variation of the SNe Ia rate and explosion characteristics with time is derived, and its correlation with parent population age and galaxy redshift is discussed. Among current scenarios, CO + He star systems should be absent from E galaxies. Explosion of CO WDs in symbiotic systems could account for the SNe Ia rate in these galaxies. The same might be true for the CO + CO WD scenario, depending on the value of the common envelope parameter. A testable prediction of the sub--Chandrasekhar WD model is that the average brightness and kinetic energy of the SN Ia events should increase with redshift for a given Hubble type. Also for this scenario, going along the Hubble sequence from E to Sc galaxies SNe Ia events should be brighter on average and should show larger mean velocities of the ejecta. The observational correlations strongly suggest that the characteristics of the SNe Ia explosion are linked to parent population age. The scenario in which WDs with masses below the Chandrasekhar mass explode appears the most promising one to explain the observed variation of the SN Ia rate with galaxy type together with the luminosity--expansion velocity trend.Comment: 16 pages uuencoded compressed Postscript, 2 figures included. ApJ Letters, in pres