7,687 research outputs found
Expansion-limited aggregation of nanoclusters in a single-pulse laser-produced plume
Formation of carbon nanoclusters in a single-laser-pulse created ablation plume was studied both in vacuum and in a noble gas environment at various pressures. The developed theory provides cluster radius dependence on combination of laser parameters, properties of ablated material, and type and pressure of an ambient gas in agreement with experiments. The experiments were performed on carbon nanoclusters formed by laser ablation of graphite targets with 12 picosecond 532 nm laser pulses at MHz-range repetition rate in a broad range of ambient He, Ar, Kr, and Xe gas pressures from 2× 10-2 to 1500 Torr. The experimental results confirmed our theoretical prediction that the average size of the nanoparticles depends weakly on the type of the ambient gas used, and is determined exclusively by the single laser pulse parameters even at the repetition rate as high as 28 MHz with the time gap 36 ns between the pulses. The most important finding relates to the fact that in vacuum the cluster size is mainly determined by hydrodynamic expansion of the plume while in the ambient gas it is controlled by atomic diffusion in the gas. We demonstrate that the ultrashort pulses can be used for production of clusters with the size less than the critical value, which separates the particles with properties drastically different from those of a material in a bulk. The presented results of experiments on formation of carbon nanoclusters are in close agreement with the theoretical scaling. The developed theory is applicable for cluster formation from any monatomic material, such as silicon for example
Cluster formation through the action of a single picosecond laser pulse
We demonstrate experimentally and describe theoretically the formation of carbon nanoclusters created by single picosecond laser pulses. We show that the average size of a nanocluster is determined exclusively by single laser pulse parameters and is independent of the gas fill (He, Ar, Kr, Xe) and pressure in a range from 20mTorr to 200 Torr. Simple kinetic theory allows estimates to be made of the cluster size, which are in qualitative agreement with the experimental data. We conclude that the role of the buffer gas is to induce a transition between thin solid film formation on the substrate and foam formation by diffusing the clusters through the gas, with no significant effect upon the average cluster size
Picosecond high-repetition-rate pulsed laser ablation of dielectrics: the effect of energy accumulation between pulses
We report experiments on the ablation of arsenic trisulphide and silicon using high-repetition-rate (megahertz) trains of picosecond pulses. In the case of arsenic trisulphide, the average single pulse fluence at ablation threshold is found to be >100 times lower when pulses are delivered as a 76-MHz train compared with the case of a solitary pulse. For silicon, however, the threshold for a 4.1-MHz train equals the value for a solitary pulse. A model of irradiation by high-repetition-rate pulse trains demonstrates that for arsenic trisulphide energy accumulates in the target surface from several hundred successive pulses, lowering the ablation threshold and causing a change from the laser-solid to laser-plasma mode as the surface temperature increases
Color-flavor locked strange matter and strangelets at finite temperature
It is possible that a system composed of up, down and strange quarks consists
the true ground state of nuclear matter at high densities and low temperatures.
This exotic plasma, called strange quark matter (SQM), seems to be even more
favorable energetically if quarks are in a superconducting state, the so-called
color-flavor locked state. Here are presented calculations made on the basis of
the MIT bag model considering the influence of finite temperature on the
allowed parameters characterizing the system for stability of bulk SQM (the
so-called stability windows) and also for strangelets, small lumps of SQM, both
in the color-flavor locking scenario. We compare these results with the
unpaired SQM and also briefly discuss some astrophysical implications of them.
Also, the issue of strangelet's electric charge is discussed. The effects of
dynamical screening, though important for non-paired SQM strangelets, are not
relevant when considering pairing among all three flavor and colors of quarks.Comment: 17 pp. 15 figs., to appear in Phys. Rev.
Nonparametric Modeling of Dynamic Functional Connectivity in fMRI Data
Dynamic functional connectivity (FC) has in recent years become a topic of
interest in the neuroimaging community. Several models and methods exist for
both functional magnetic resonance imaging (fMRI) and electroencephalography
(EEG), and the results point towards the conclusion that FC exhibits dynamic
changes. The existing approaches modeling dynamic connectivity have primarily
been based on time-windowing the data and k-means clustering. We propose a
non-parametric generative model for dynamic FC in fMRI that does not rely on
specifying window lengths and number of dynamic states. Rooted in Bayesian
statistical modeling we use the predictive likelihood to investigate if the
model can discriminate between a motor task and rest both within and across
subjects. We further investigate what drives dynamic states using the model on
the entire data collated across subjects and task/rest. We find that the number
of states extracted are driven by subject variability and preprocessing
differences while the individual states are almost purely defined by either
task or rest. This questions how we in general interpret dynamic FC and points
to the need for more research on what drives dynamic FC.Comment: 8 pages, 1 figure. Presented at the Machine Learning and
Interpretation in Neuroimaging Workshop (MLINI-2015), 2015 (arXiv:1605.04435
Collisional transport across the magnetic field in drift-fluid models
Drift ordered fluid models are widely applied in studies of low-frequency
turbulence in the edge and scrape-off layer regions of magnetically confined
plasmas. Here, we show how collisional transport across the magnetic field is
self-consistently incorporated into drift-fluid models without altering the
drift-fluid energy integral. We demonstrate that the inclusion of collisional
transport in drift-fluid models gives rise to diffusion of particle density,
momentum and pressures in drift-fluid turbulence models and thereby obviate the
customary use of artificial diffusion in turbulence simulations. We further
derive a computationally efficient, two-dimensional model which can be time
integrated for several turbulence de-correlation times using only limited
computational resources. The model describes interchange turbulence in a
two-dimensional plane perpendicular to the magnetic field located at the
outboard midplane of a tokamak. The model domain has two regions modeling open
and closed field lines. The model employs a computational expedient model for
collisional transport. Numerical simulations show good agreement between the
full and the simplified model for collisional transport
Manipulating the torsion of molecules by strong laser pulses
A proof-of-principle experiment is reported, where torsional motion of a
molecule, consisting of a pair of phenyl rings, is induced by strong laser
pulses. A nanosecond laser pulse spatially aligns the carbon-carbon bond axis,
connecting the two phenyl rings, allowing a perpendicularly polarized, intense
femtosecond pulse to initiate torsional motion accompanied by an overall
rotation about the fixed axis. The induced motion is monitored by femtosecond
time-resolved Coulomb explosion imaging. Our theoretical analysis accounts for
and generalizes the experimental findings.Comment: 4 pages, 4 figures, submitted to PRL; Major revision of the
presentation of the material; Correction of ion labels in Fig. 2(a
Simulation of transition dynamics to high confinement in fusion plasmas
The transition dynamics from the low (L) to the high (H) confinement mode in
magnetically confined plasmas is investigated using a first-principles
four-field fluid model. Numerical results are in close agreement with
measurements from the Experimental Advanced Superconducting Tokamak - EAST.
Particularly, the slow transition with an intermediate dithering phase is well
reproduced by the numerical solutions. Additionally, the model reproduces the
experimentally determined L-H transition power threshold scaling that the ion
power threshold increases with increasing particle density. The results hold
promise for developing predictive models of the transition, essential for
understanding and optimizing future fusion power reactors
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