NMR and NQR study of pressure-induced superconductivity and the origin of critical-temperature enhancement in the spin-ladder cuprate Sr2_2Ca12_{12}Cu24_{24}O41_{41}

Pressure-induced superconductivity was studied for a spin-ladder cuprate Sr$_2$Ca$_{12}$Cu$_{24}$O$_{41}$ using nuclear magnetic resonance (NMR) under pressures up to the optimal pressure 3.8 GPa. Pressure application leads to a transitional change from a spin-gapped state to a Fermi-liquid state at temperatures higher than $T_c$. The relaxation rate $1/T_1$ shows activated-type behavior at an onset pressure, whereas Korringa-like behavior becomes predominant at the optimal pressure, suggesting that an increase in the density of states (DOS) at the Fermi energy leads to enhancement of $T_c$. Nuclear quadrupole resonance (NQR) spectra suggest that pressure application causes transfer of holes from the chain to the ladder sites. The transfer of holes increases DOS below the optimal pressure. A dome-shaped $T_c$ versus pressure curve arises from naive balance between the transfer of holes and broadening of the band width

Kondo effect in CeXc_{c} (Xc_{c}=S, Se, Te) studied by electrical resistivity under high pressure

We have measured the electrical resistivity of cerium monochalcogenices, CeS, CeSe, and CeTe, under high pressures up to 8 GPa. Pressure dependences of the antiferromagnetic ordering temperature $T_{N}$, crystal field splitting, and the $\ln T$ anomaly of the Kondo effect have been studied to cover the whole region from the magnetic ordering regime at low pressure to the Fermi liquid regime at high pressure. $T_{N}$ initially increases with increasing pressure, and starts to decrease at high pressure as expected from the Doniach's diagram. Simultaneously, the $\ln T$ behavior in the resistivity is enhanced, indicating the enhancement of the Kondo effect by pressure. It is also characteristic in CeX$_{c}$ that the crystal field splitting rapidly decreases at a common rate of $-12.2$ K/GPa. This leads to the increase in the degeneracy of the $f$ state and further enhancement of the Kondo effect. It is shown that the pressure dependent degeneracy of the $f$ state is a key factor to understand the pressure dependence of $T_{N}$, Kondo effect, magnetoresistance, and the peak structure in the temperature dependence of resistivity.Comment: 9 pages, 5 figures, accepted for publication in J. Phys. Soc. Jp

Electrical resistivity and tunneling anomalies in CeCuAs2

The compound CeCuAs2 is found to exhibit negative temperature (T) coefficient of electrical resistivity (rho) under ambient pressure conditions in the entire T-range of investigation (45 mK to 300 K), even in the presence of high magnetic fields. Preliminary tunneling spectroscopic measurements indicate the existence of a psuedo-gap at least at low temperatures, thereby implying that this compound could be classified as a Kondo semi-conductor, though rho(T) interestingly is not found to be of an activated type.Comment: To appear in the proceedings of SCES200

Stoner gap in the superconducting ferromagnet UGe2

We report the temperature ($T$) dependence of ferromagnetic Bragg peak intensities and dc magnetization of the superconducting ferromagnet UGe2 under pressure ($P$). We have found that the low-$T$ behavior of the uniform magnetization can be explained by a conventional Stoner model. A functional analysis of the data produces the following results: The ferromagnetic state below a critical pressure can be understood as the perfectly polarized state, in which heavy quasiparticles occupy only majority spin bands. A Stoner gap $\Delta(P)$ decreases monotonically with increasing pressure and increases linearly with magnetic field. We show that the present analysis based on the Stoner model is justified by a consistency check, i.e., comparison of density of states at the Fermi energy deduced from the analysis with observed electronic specific heat coeffieients. We also argue the influence of the ferromagnetism on the superconductivity.Comment: 5 pages, 4 figures. to be published in Phys. Rev.

The ground state of Sr3Ru2O7 revisited; Fermi liquid close to a ferromagnetic instability

We show that single-crystalline Sr3Ru2O7 grown by a floating-zone technique is an isotropic paramagnet and a quasi-two dimensional metal as spin-triplet superconducting Sr2RuO4 is. The ground state is Fermi liquid with very low residual resistivity (3 micro ohm cm for in-plane currents) and a nearly ferromagnetic metal with the largest Wilson ratio Rw>10 among paramagnets so far. This contrasts with the ferromagnetic order at Tc=104 K reported on single crystals grown by a flux method [Cao et al., Phys. Rev. B 55, R672 (1997)]. We have also found a dramatic changeover from paramagnetism to ferromagnetism under applied pressure. This suggests the existence of a substantial ferromagnetic instability on the verge of a quantum phase transition in the Fermi liquid state.Comment: 5 pages, 4 figures, to be published in Phys. Rev. B : Rapid co