Magnetic Transition Temperature of (La,Sr)MnO3_3

Using the Kondo lattice model with classical spins in infinite dimension, magnetic phase transition in the perovskite-type $3d$ transition-metal oxide (La,Sr)MnO$_3$ is theoretically studied. On the Bethe lattice, the self-consistency equations are solved exactly. Curie temperatures at the region of double-exchange ferromagnetism $0.1 < x < 0.25$ as well as the Neel temperature at $x=0$ are well reproduced quantitatively. Pressure effect on the Curie temperature is also discussed.Comment: 7 pages, 1 PS file with 3 figures appended at the end, LaTe

Phase Diagram of Half Doped Manganites

An analysis of the properties of half-doped manganites is presented. We build up the phase diagram of the system combining a realistic calculation of the electronic properties and a mean field treatment of the temperature effects. The electronic structure of the manganites are described with a double exchange model with cooperative Jahn-Teller phonons and antiferromagnetic coupling between the $Mn$ core spins. At zero temperature a variety of electronic phases as ferromagnetic (FM) charge ordered (CO) orbital ordered (OO), CE-CO-OO and FM metallic, are obtained. By raising the temperature the CE-CO-OO phase becomes paramagnetic (PM), but depending on the electron-phonon coupling and the exchange coupling the transition can be direct or trough intermediate states: a FM disorder metallic, a PM-CO-OO or a FM-CO-OO. We also discus the nature of the high temperature PM phase in the regime of finite electron phonon coupling. In this regime half of the oxygen octahedra surrounding the $Mn$ ions are distorted. In the weak coupling regime the octahedra are slightly deformed and only trap a small amount of electronic charge, rendering the system metallic consequentially. However in the strong coupling regime the octahedra are strongly distorted, the charge is fully localized in polarons and the system is insulator.Comment: 10 pagses, 9 figures include

Superconducting and normal-state interlayer-exchange-coupling in La0.67_{0.67}Sr0.33_{0.33}MnO3{3}-YBa2_{2}Cu3_{3}O7−La_{7}-La_{0.67}SrSr_{0.33}MnO MnO{3}$ epitaxial trilayers

The issue of interlayer exchange coupling in magnetic multilayers with superconducting (SC) spacer is addressed in La$_{0.67}$Sr$_{0.33}$MnO$_{3}$ (LSMO) - YBa$_{2}$Cu$_{3}$O$_{7}$ (YBCO) - La$_{0.67}$Sr$_{0.33}$MnO$_{3}$ (LSMO) epitaxial trilayers through resistivity, ac-susceptibility and magnetization measurements. The ferromagnetic (FM) LSMO layers possessing in-plane magnetization suppress the critical temperature (T$_{c})$ of the c-axis oriented YBCO thin film spacer. The superconducting order, however, survives even in very thin layers (thickness d$_{Y} \sim$ 50 {\AA}, $\sim$ 4 unit cells) at T $<$ 25 K. A predominantly antiferromagnetic (AF) exchange coupling between the moments of the LSMO layers at fields $<$ 200 Oe is seen in the normal as well as the superconducting states of the YBCO spacer. The exchange energy J$_{1}$ ($\sim$ 0.08 erg/cm$^{2}$ at 150 K for d$_{Y}$ = 75 {\AA}) grows on cooling down to T$_{c}$, followed by truncation of this growth on entering the superconducting state. The coupling energy J$_{1}$ at a fixed temperature drops exponentially with the thickness of the YBCO layer. The temperature and d$_{Y}$ dependencies of this primarily non-oscillatory J$_{1}$ are consistent with the coupling theories for systems in which transport is controlled by tunneling. The truncation of the monotonic T dependence of J$_{1}$ below T$_{c}$ suggests inhibition of single electron tunneling across the CuO$_{2}$ planes as the in-plane gap parameter acquires a non-zero value.Comment: Accepted for publication in Phys. Rev.

Electron- and Hole-Doping Effects on AA-site Ordered NdBaMn2_2O6_6

We have investigated electron- and hole-doping effects on $A$-site ordered perovskite manganite NdBaMn$_2$O$_6$, which has the $A$-type (layered) antiferromagnetic (AFM) ground state. Electrons (holes) are introduced by partial substitution of Ba$^{2+}$ (Nd$^{3+}$) with Nd$^{3+}$ (Ba$^{2+}$). Electron-doping generates ferromagnetic (FM) clusters in the $A$-type AFM matrix. With increasing the electron-doping level, the volume fraction of the FM phase or the number of the FM clusters is abruptly increasing. In contrast, the $A$-type AFM phase is robust against the hole-doping, and no FM correlation is observed in the hole-doped NdBaMn$_2$O$_6$.Comment: 8 pages, 5 figures, to be published in Journal of the Physical Society of Japa

Resonant inelastic x-ray scattering study of hole-doped manganites La1-xSrxMnO3 (x=0.2 and 0.4)

Electronic excitations near the Fermi energy in the hole doped manganese oxides (La1-xSrxMnO3, x=0.2 and 0.4) have been elucidated by using the resonant inelastic x-ray scattering (RIXS) method. A doping effect in the strongly correlated electron systems has been observed for the first time. The scattering spectra show that a salient peak appears in low energies indicating the persistence of the Mott gap. At the same time, the energy gap is partly filled by doping holes and the energy of the spectral weight shifts toward lower energies. The excitation spectra show little change in the momentum space as is in undoped LaMnO3, but the scattering intensities in the low energy excitations of x=0.2 are anisotropic as well as temperature dependent, which indicates a reminiscence of the orbital nature

An X-Ray Induced Structural Transition in La_0.875Sr_0.125MnO_3

We report a synchrotron x-ray scattering study of the magnetoresistive manganite La_0.875Sr_0.125MnO_3. At low temperatures, this material undergoes an x-ray induced structural transition at which charge ordering of Mn^3+ and Mn^4+ ions characteristic to the low-temperature state of this compound is destroyed. The transition is persistent but the charge-ordered state can be restored by heating above the charge-ordering transition temperature and subsequently cooling. The charge-ordering diffraction peaks, which are broadened at all temperatures, broaden more upon x-ray irradiation, indicating the finite correlation length of the charge-ordered state. Together with the recent reports on x-ray induced transitions in Pr_(1-x)Ca_xMnO_3, our results demonstrate that the photoinduced structural change is a common property of the charge-ordered perovskite manganites.Comment: 5 pages, 4 embedded EPS figures; significant changes in the data analysis mad

Existence of orbital polarons in ferromagnetic insulating La1−x_{1-x}Srx_xMnO3_{3} (0.11<x<<x<0.14) evidenced by giant phonon softening

We present an inelastic light scattering study of single crystalline (La$_{1-y}$Pr$_y$)$_{1-x}$Sr$_{x}$MnO$_3$ ($0\leq x\leq0.14$,$y=0$ and $x=1/8$,$0\leq y\leq0.5$). A giant softening up to 20 - 30 cm$^{-1}$ of the Mn-O breathing mode has been observed only for the ferromagnetic insulating (FMI) samples ($0.11\leq x \leq 0.14$) upon cooling below the Curie temperature. With increasing Pr-doping the giant softening is gradually suppressed. This is attributed to a coupling of the breathing mode to orbital polarons which are present in the FMI phase.Comment: 4 pages, 5 figure

The Density of States of hole-doped Manganites: A Scanning Tunneling Microscopy/Spectroscopy study

Variable temperature scanning tunneling microscopy/spectroscopy studies on single crystals and epitaxial thin films of hole-doped manganites, which show colossal magnetoresistance, have been done. We have investigated the variation of the density of states, at and near the Fermi energy ($E_f$), as a function of temperature. Simple calculations have been carried out, to find out the effect of temperature on the tunneling spectra and extract the variation of density of states with temperature, from the observed data. We also report here, atomic resolution images, on the single crystals and larger range images showing the growth patterns on thin films. Our investigation shows unambiguously that there is a rapid variation in density of states for temperatures near the Curie temperature ($T_c$). While for temperatures below $T_c$, a finite DOS is observed at $E_f$, for temperatures near $T_c$ a hard gap opens up in the density of states near $E_f$. For temperatures much higher than $T_c$, this gap most likely gives way to a soft gap. The observed hard gap for temperatures near $T_c$, is somewhat higher than the transport gap for all the materials. For different materials, we find that the magnitude of the hard gap decreases as the $T_c$ of the material increases and eventually, for materials with a $T_c$ close to 400 K, the value of the gap approaches zero.Comment: 9 pages RevTeX, 12 postscript figures, 1 table included in text, submitted to Physical Review

Interplay of the CE-type charge ordering and the A-type spin ordering in a half-doped bilayer manganite La{1}Sr{2}Mn{2}O{7}

We demonstrate that the half-doped bilayer manganite La_{1}Sr_{2}Mn_{2}O_{7} exhibits CE-type charge-ordered and spin-ordered states below $T_{N, CO}^A = 210$ K and below $T_{N}^{CE} \sim 145$ K, respectively. However, the volume fraction of the CE-type ordering is relatively small, and the system is dominated by the A-type spin ordering. The coexistence of the two types of ordering is essential to understand its transport properties, and we argue that it can be viewed as an effective phase separation between the metallic $d(x^{2}-y^{2})$ orbital ordering and the charge-localized $d(3x^{2}-r^{2})/d(3y^{2}-r^{2})$ orbital ordering.Comment: 5 pages, 4 figures, submitted to Phys. Rev.

Spin Excitation Spectrum of La1−xAx_{1-x}A_xMnO3_3

As an effective model to describe perovskite-type manganates (La,$A$)MnO$_3$, the double-exchange model on a cubic lattice is investigated. Spin excitation spectrum of the model in the ground state is studied using the spin wave approximation. Spin wave dispersion relation observed in the inelastic neutron scattering experiment of La$_{0.7}$Pb$_{0.3}$MnO$_3$ is reproduced. Effective values for the electron bandwidth as well as Hund's coupling is estimated from the data.Comment: 10 pages LaTeX including 4 PS figure