507 research outputs found
Field-induced staggered magnetic moment in the quasi-two-dimensional organic Mott insulator -(BEDT-TTF)Cu[N(CN)]Cl
We investigated the magnetism under a magnetic field in the
quasi-two-dimensional organic Mott insulator
-(BEDT-TTF)Cu[N(CN)]Cl through magnetization and
C-NMR measurements. We found that in the nominally paramagnetic phase
(i.e., above N\'eel temperature) the field-induced local moments have a
staggered component perpendicular to the applied field. As a result, the
antiferromagnetic transition well defined at a zero field becomes crossover
under a finite field. This unconventional behavior is qualitatively reproduced
by the molecular-field calculation for Hamiltonian including the exchange,
Dzyaloshinsky-Moriya (DM), and Zeeman interactions. This calculation also
explains other unconventional magnetic features in
-(BEDT-TTF)Cu[N(CN)]Cl reported in the literature. The
present results highlight the importance of the DM interaction in field-induced
magnetism in a nominally paramagnetic phase, especially in low-dimensional spin
systems.Comment: 11 pages, 12 figures, selected for Editors' Suggestion
Gain dynamics and ultrafast spectral hole burning in In(Ga)As self-organized quantum dots
Using a femtosecond three-pulse pump-probe technique, we investigated spectral hole-burning and gain recovery dynamics in self-organized In(Ga)As quantum dots. The spectral hole dynamics are qualitatively different from those observed in quantum wells, and allow us to distinguish unambiguously the gain recovery due to intradot relaxation and that due to carrier capture. The gain recovery due to carrier–carrier scattering-dominated intradot relaxation is very fast ( ∼ 130 fs),(∼130fs), indicating that this is not the factor limiting the bandwidth of directly modulated quantum dot lasers. © 2002 American Institute of Physics.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/70041/2/APPLAB-81-4-670-1.pd
Temperature-dependent carrier dynamics in self-assembled InGaAs quantum dots
We measured the transient temperature-dependent carrier population in the confined states of self-assembled In0.4Ga0.6AsIn0.4Ga0.6As quantum dots as well as those of the surrounding wetting layer and barrier region using differential transmission spectroscopy. Results show directly that thermal reemission and nonradiative recombination contribute significantly to the dynamics above 100 K. We offer results of an ensemble Monte Carlo simulation to explain the contribution of these thermally activated processes. © 2002 American Institute of Physics.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/71088/2/APPLAB-80-12-2162-1.pd
Periodic Oscillations of Josephson-Vortex Flow Resistance in Oxygen-Deficient Y1Ba2Cu3Ox
We measured the Josephson vortex flow resistance as a function of magnetic
field applied parallel to the ab-planes using annealed Y1Ba2Cu3Ox intrinsic
Josephson junctions having high anisotropy (around 40) by oxygen content
reduction. Periodic oscillations were observed in magnetic fields above 45-58
kOe, corresponding to dense-dilute boundary for Josephson vortex lattice. The
observed period of oscillations, agrees well with the increase of one fluxon
per two junctions (\textit{=}\textit{/2Ls}), may correspond
to formation of a triangular lattice of Josephson vortices as has been reported
by Ooi et al. for highly anisotropic (larger than 200) Bi-2212 intrinsic
Josephson junctions.Comment: 5 pages, 4 figure
Transport criticality of the first-order Mott transition in a quasi-two-dimensional organic conductor, -(BEDT-TTF)Cu[N(CN)]Cl
An organic Mott insulator, -(BEDT-TTF)Cu[N(CN)]Cl, was
investigated by resistance measurements under continuously controllable He gas
pressure. The first-order Mott transition was demonstrated by observation of
clear jump in the resistance variation against pressure. Its critical endpoint
at 38 K is featured by vanishing of the resistive jump and critical divergence
in pressure derivative of resistance, , which are consistent with the prediction of the dynamical mean field
theory and have phenomenological correspondence with the liquid-gas transition.
The present results provide the experimental basis for physics of the Mott
transition criticality.Comment: 4 pages, 5 figure
Nature of bonding and electronic structure in MgB2, a boron intercalation superconductor
Chemical bonding and electronic structure of MgB2, a boron-based newly
discovered superconductor, is studied using self-consistent band structure
techniques. Analysis of the transformation of the band structure for the
hypothetical series of graphite - primitive graphite - primitive graphite-like
boron - intercalated boron, shows that the band structure of MgB2 is
graphite-like, with pi-bands falling deeper than in ordinary graphite. These
bands possess a typically delocalized and metallic, as opposed to covalent,
character. The in-plane sigma-bands retain their 2D covalent character, but
exhibit a metallic hole-type conductivity. The coexistence of 2D covalent
in-plane and 3D metallic-type interlayer conducting bands is a peculiar feature
of MgB2. We analyze the 2D and 3D features of the band structure of MgB2 and
related compounds, and their contributions to conductivity.Comment: 4 pages in revtex, 3 figures in 4 separate EPS file
Discovery and cardioprotective effects of the first non-peptide agonists of the G protein-coupled prokineticin receptor-1
Prokineticins are angiogenic hormones that activate two G protein-coupled receptors: PKR1 and PKR2. PKR1 has emerged as a critical mediator of cardiovascular homeostasis and cardioprotection. Identification of non-peptide PKR1 agonists that contribute to myocardial repair and collateral vessel growth hold promises for treatment of heart diseases. Through a combination of in silico studies, medicinal chemistry, and pharmacological profiling approaches, we designed, synthesized, and characterized the first PKR1 agonists, demonstrating their cardioprotective activity against myocardial infarction (MI) in mice. Based on high throughput docking protocol, 250,000 compounds were computationally screened for putative PKR1 agonistic activity, using a homology model, and 10 virtual hits were pharmacologically evaluated. One hit internalizes PKR1, increases calcium release and activates ERK and Akt kinases. Among the 30 derivatives of the hit compound, the most potent derivative, IS20, was confirmed for its selectivity and specificity through genetic gain- and loss-of-function of PKR1. Importantly, IS20 prevented cardiac lesion formation and improved cardiac function after MI in mice, promoting proliferation of cardiac progenitor cells and neovasculogenesis. The preclinical investigation of the first PKR1 agonists provides a novel approach to promote cardiac neovasculogenesis after MI
Theory of the beta-type Organic Superconductivity under Uniaxial Compression
We study theoretically the shift of the superconducting transition
temperature (Tc) under uniaxial compression in beta-type organic
superconductors, beta-(BEDT-TTF)2I3 and beta-(BDA-TTP)2X[X=SbF6,AsF6], in order
to clarify the electron correlation, the spin frustration and the effect of
dimerization. The transfer integrals are calculated by the extended Huckel
method assuming the uniaxial strain and the superconducting state mediated by
the spin fluctuation is solved using Eliashberg's equation with the
fluctuation-exchange approximation. The calculation is carried out on both the
dimerized (one-band) and nondimerized (two-band) Hubbard models. We have found
that (i) the behavior of Tc in beta-(BEDT-TTF)2I3 with a stronger dimerization
is well reproduced by the dimer model, while that in weakly dimerized
beta-BDA-TTP salts is rather well reproduced by the two-band model, and (ii)
the competition between the spin frustration and the effect induced by the
fluctuation is important in these materials, which causes nonmonotonic shift of
Tc against uniaxial compression.Comment: 18 pages, 16 figures, 2 tabl
Density and temperature dependence of carrier dynamics in self-organized InGaAs quantum dots
We have used two- and three-pulse femtosecond differential transmission spectroscopy to study the dependence of quantum dot carrier dynamics on temperature. At low temperatures and densities, the rates for relaxation between the quantum dot confined states and for capture from the barrier region into the various dot levels could be directly determined. For electron–hole pairs generated directly in the quantum dot excited state, relaxation is dominated by electron–hole scattering, and occurs on a 5 ps time scale. Capture times from the barrier into the quantum dot are of the order of 2 ps (into the excited state) and 10 ps (into the ground state). The phonon bottleneck was clearly observed in low-density capture experiments, and the conditions for its observation (namely, the suppression of electron–hole scattering for nongeminately captured electrons) were determined. As temperature increases beyond about 100 K, the dynamics become dominated by the re-emission of carriers from the lower dot levels, due to the large density of states in the wetting layer and barrier region. Measurements of the gain dynamics show fast (130 fs) gain recovery due to intradot carrier–carrier scattering, and picosecond-scale capture. Direct measurement of the transparency density versus temperature shows the dramatic effect of carrier re-emission for the quantum dots on thermally activated scattering. The carrier dynamics at elevated temperature are thus strongly dominated by the high density of the high energy continuum states relative to the dot confined levels. Deleterious hot carrier effects can be suppressed in quantum dot lasers by resonant tunnelling injection.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/48924/2/d5_13_003.pd
Comparison of the Fermi-surface topologies of kappa-(BEDT-TTF)_2 Cu(NCS)_2 and its deuterated analogue
We have measured details of the quasi one-dimensional Fermi-surface sections
in the organic superconductor kappa-(BEDT-TTF)_2 Cu(NCS)_2 and its deuterated
analogue using angle-dependent millimetre-wave techniques. There are
significant differences in the corrugations of the Fermi surfaces in the
deuterated and undeuterated salts. We suggest that this is important in
understanding the inverse isotope effect, where the superconducting transition
temperature rises on deuteration. The data support models for superconductivity
which invoke electron-electron interactions depending on the topological
properties of the Fermi surface
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