2 research outputs found
Hall effect in superconducting Fe(Se0.5Te0.5) thin films
The Hall effect is investigated for eight superconducting Fe(Se_0.5_Te_0.5_)
thin films grown on MgO and LaSrAlO_4_ substrates with different transition
temperatures (T_c_). The normal Hall coefficients (R_H_) have positive values
with magnitude of 1 - 1.5 x 10^-3^ cm^3^/C at room temperature for the all
samples. With decreasing temperature, we find two characteristic types of
behavior in R_H_(T) depending on T_c_. For thin films with lower T_c_
(typically T_c_ < 5 K), R_H_ start decreasing approximately below T = 250 K
toward a negative side, some of which shows sign reversal at T = 50 - 60 K, but
turns positive toward T = 0 K. On the other hand for the films with higher T_c_
(typically T_c_ > 9 K), R_ H_ leaves almost unchanged down to T = 100 K, and
then starts decreasing toward a negative side. Around the temperatures when
R_H_ changes its sign from positive to negative, obvious nonlinearity is
observed in the field-dependence of Hall resistance as to keep the low-field
R_H_ positive while the high-field R_H_ negative. Thus the electronic state
just above T_c_ is characterized by n_e_ (electron density) > n_h_ (hole
density) with keeping \mu_e_ < \mu_h_. These results suggest the dominance of
electron density to the hole density is an essential factor for the occurence
of superconductivity in Fe-chalcogenide superconductors.Comment: 11 pages, 4 figures, revised version for Physical Review B. accepted
for publication in Physical Review
Transport and superconducting properties of Fe-based superconductors: SmFeAs(O1-x Fx) versus Fe1+y (Te1-x, Sex)
We present transport and superconducting properties - namely resistivity,
magnetoresistivity, Hall effect, Seebeck effect, thermal conductivity, upper
critical field - of two different families of Fe-based superconductors, which
can be viewed in many respects as end members: SmFeAs(O1-xFx) with the largest
Tc and the largest anisotropy and Fe1+y(Te1-x,Sex), with the largest Hc2, the
lowest Tc and the lowest anisotropy. In the case of the SmFeAs(O1-xFx) series,
we find that a single band description allows to extract an approximated
estimation of band parameters such as carrier density and mobility from
experimental data, although the behaviour of Seebeck effect as a function of
doping demonstrates that a multiband description would be more appropriate. On
the contrary, experimental data of the Fe1+y(Te1-x,Sex) series exhibit a
strongly compensated behaviour, which can be described only within a multiband
model. In the Fe1+y(Te1-x,Sex) series, the role of the excess Fe, tuned by Se
stoichiometry, is found to be twofold: it dopes electrons in the system and it
introduces localized magnetic moments, responsible for Kondo like scattering
and likely pair-breaking of Cooper pairs. Hence, excess Fe plays a crucial role
also in determining superconducting properties such as the Tc and the upper
critical field Bc2. The huge Bc2 values of the Fe1+y(Te1-x,Sex) samples are
described by a dirty limit law, opposed to the clean limit behaviour of the
SmFeAs(O1-xFx) samples. Hence, magnetic scattering by excess Fe seems to drive
the system in the dirty regime, but its detrimental pairbreaking role seems not
to be as severe as predicted by theory. This issue has yet to be clarified,
addressing the more fundamental issue of the interplay between magnetism and
superconductivity