4 research outputs found
Room-temperature exciton-polaritons with two-dimensional WS2
Two-dimensional transition metal dichalcogenides exhibit strong optical
transitions with significant potential for optoelectronic devices. In
particular they are suited for cavity quantum electrodynamics in which strong
coupling leads to polariton formation as a root to realisation of inversionless
lasing, polariton condensationand superfluidity. Demonstrations of such
strongly correlated phenomena to date have often relied on cryogenic
temperatures, high excitation densities and were frequently impaired by strong
material disorder. At room-temperature, experiments approaching the strong
coupling regime with transition metal dichalcogenides have been reported, but
well resolved exciton-polaritons have yet to be achieved. Here we report a
study of monolayer WS coupled to an open Fabry-Perot cavity at
room-temperature, in which polariton eigenstates are unambiguously displayed.
In-situ tunability of the cavity length results in a maximal Rabi splitting of
meV, exceeding the exciton linewidth. Our data
are well described by a transfer matrix model appropriate for the large
linewidth regime. This work provides a platform towards observing strongly
correlated polariton phenomena in compact photonic devices for ambient
temperature applications.Comment: 12 pages, 6 figure
Strong exciton-photon coupling in large area MoSe2 and WSe2 heterostructures fabricated from two-dimensional materials grown by chemical vapor deposition
Two-dimensional semiconducting transition metal dichalcogenides embedded in optical microcavities in the strong exciton-photon coupling regime may lead to promising applications in spin and valley addressable polaritonic logic gates and circuits. One significant obstacle for their realization is the inherent lack of scalability associated with the mechanical exfoliation commonly used for fabrication of two-dimensional materials and their heterostructures. Chemical vapor deposition offers an alternative scalable fabrication method for both monolayer semiconductors and other two-dimensional materials, such as hexagonal boron nitride. Observation of the strong light-matter coupling in chemical vapor grown transition metal dichalcogenides has been demonstrated so far in a handful of experiments with monolayer molybdenum disulfide and tungsten disulfide. Here we instead demonstrate the strong exciton-photon coupling in microcavities composed of large area transition metal dichalcogenide/hexagonal boron nitride heterostructures made from chemical vapor deposition grown molybdenum diselenide and tungsten diselenide encapsulated on one or both sides in continuous few-layer boron nitride films also grown by chemical vapor deposition. These transition metal dichalcogenide/hexagonal boron nitride heterostructures show high optical quality comparable with mechanically exfoliated samples, allowing operation in the strong coupling regime in a wide range of temperatures down to 4 Kelvin in tunable and monolithic microcavities, and demonstrating the possibility to successfully develop large area transition metal dichalcogenide based polariton devices