198 research outputs found
Local atomic structure and discommensurations in the charge density wave of CeTe3
The local structure of CeTe3 in the incommensurate charge density wave
(IC-CDW) state has been obtained using atomic pair distribution function (PDF)
analysis of x-ray diffraction data. Local atomic distortions in the Te-nets due
to the CDW are larger than observed crystallographically, resulting in distinct
short and long Te-Te bonds. Observation of different distortion amplitudes in
the local and average structures are explained by the discommensurated nature
of the CDW since the PDF is sensitive to the local displacements within the
commensurate regions whereas the crystallographic result averages over many
discommensurated domains. The result is supported by STM data. This is the
first quantitative local structural study within the commensurate domains in an
IC-CDW system.Comment: 4 pages, 4 figure
Direct observation of micron-scale ordered structure in a two-dimensional electron system
We have applied a novel scanned probe method to directly resolve the interior
structure of a GaAs/AlGaAs two-dimensional electron system in a tunneling
geometry. We find that the application of a perpendicular magnetic field can
induce surprising density modulations that are not static as a function of the
field. Near six and four filled Landau levels, stripe-like structures emerge
with a characteristic wave length ~2 microns. Present theories do not account
for ordered density modulations on this length scale.Comment: 5 pages, 4 figures. To appear in Phys. Rev.
Scanning-probe spectroscopy of semiconductor donor molecules
Semiconductor devices continue to press into the nanoscale regime, and new
applications have emerged for which the quantum properties of dopant atoms act
as the functional part of the device, underscoring the necessity to probe the
quantum structure of small numbers of dopant atoms in semiconductors[1-3].
Although dopant properties are well-understood with respect to bulk
semiconductors, new questions arise in nanosystems. For example, the quantum
energy levels of dopants will be affected by the proximity of nanometer-scale
electrodes. Moreover, because shallow donors and acceptors are analogous to
hydrogen atoms, experiments on small numbers of dopants have the potential to
be a testing ground for fundamental questions of atomic and molecular physics,
such as the maximum negative ionization of a molecule with a given number of
positive ions[4,5]. Electron tunneling spectroscopy through isolated dopants
has been observed in transport studies[6,7]. In addition, Geim and coworkers
identified resonances due to two closely spaced donors, effectively forming
donor molecules[8]. Here we present capacitance spectroscopy measurements of
silicon donors in a gallium-arsenide heterostructure using a scanning probe
technique[9,10]. In contrast to the work of Geim et al., our data show
discernible peaks attributed to successive electrons entering the molecules.
Hence this work represents the first addition spectrum measurement of dopant
molecules. More generally, to the best of our knowledge, this study is the
first example of single-electron capacitance spectroscopy performed directly
with a scanning probe tip[9].Comment: In press, Nature Physics. Original manuscript posted here; 16 pages,
3 figures, 5 supplementary figure
Chaos in Andreev Billiards
A new type of classical billiard - the Andreev billiard - is investigated
using the tangent map technique. Andreev billiards consist of a normal region
surrounded by a superconducting region. In contrast with previously studied
billiards, Andreev billiards are integrable in zero magnetic field, {\it
regardless of their shape}. A magnetic field renders chaotic motion in a
generically shaped billiard, which is demonstrated for the Bunimovich stadium
by examination of both Poincar\'e sections and Lyapunov exponents. The issue of
the feasibility of certain experimental realizations is addressed.Comment: ReVTeX3.0, 4 pages, 3 figures appended as postscript file (uuencoded
with uufiles
Modeling Subsurface Charge Accumulation Images of a Quantum Hall Liquid
Subsurface Charge Accumulation imaging is a cryogenic scanning probe
technique that has recently been used to spatially probe incompressible strips
formed in a two-dimensional electron system (2DES) at high magnetic fields. In
this paper, we present detailed numerical modeling of these data. At a basic
level, the method produces results that agree well with the predictions of
models based on simple circuit elements. Moreover, the modeling method is
sufficiently advanced to simulate the spatially resolved measurements. By
comparing directly the simulations to the experimentally measured data, we can
extract quantitatively local electronic features of the 2DES. In particular, we
deduce the electron density of states inside the incompressible strips and
electrical resistance across them.Comment: 11 pages, 3 figure
Modifying the surface electronic properties of YBa2Cu3O7-delta with cryogenic scanning probe microscopy
We report the results of a cryogenic study of the modification of
YBa2Cu3O7-delta surface electronic properties with the probe of a scanning
tunneling microscope (STM). A negative voltage applied to the sample during STM
tunneling is found to modify locally the conductance of the native degraded
surface layer. When the degraded layer is removed by etching, the effect
disappears. An additional surface effect is identified using Scanning Kelvin
Probe Microscopy in combination with STM. We observe reversible surface
charging for both etched and unetched samples, indicating the presence of a
defect layer even on a surface never exposed to air.Comment: 6 pages, 4 figures. To appear in Superconductor Science and
Technolog
Anisotropy and periodicity in the density distribution of electrons in a quantum-well
We use low temperature near-field optical spectroscopy to image the electron
density distribution in the plane of a high mobility GaAs quantum well. We find
that the electrons are not randomly distributed in the plane, but rather form
narrow stripes (width smaller than 150 nm) of higher electron density. The
stripes are oriented along the [1-10 ] crystal direction, and are arranged in a
quasi-periodic structure. We show that elongated structural mounds, which are
intrinsic to molecular beam epitaxy, are responsible for the creation of this
electron density texture.Comment: 10 pages, 3 figure
High accuracy FIONA–AFM hybrid imaging
Multi-protein complexes are ubiquitous and play essential roles in many biological mechanisms. Single molecule imaging techniques such as electron microscopy (EM) and atomic force microscopy (AFM) are powerful methods for characterizing the structural properties of multi-protein and multi-protein–DNA complexes. However, a significant limitation to these techniques is the ability to distinguish different proteins from one another. Here, we combine high resolution fluorescence microscopy and AFM (FIONA–AFM) to allow the identification of different proteins in such complexes. Using quantum dots as fiducial markers in addition to fluorescently labeled proteins, we are able to align fluorescence and AFM information to ≥8 nm accuracy. This accuracy is sufficient to identify individual fluorescently labeled proteins in most multi-protein complexes. We investigate the limitations of localization precision and accuracy in fluorescence and AFM images separately and their effects on the overall registration accuracy of FIONA–AFM hybrid images. This combination of the two orthogonal techniques (FIONA and AFM) opens a wide spectrum of possible applications to the study of protein interactions, because AFM can yield high resolution (5–10 nm) information about the conformational properties of multi-protein complexes and the fluorescence can indicate spatial relationships of the proteins in the complexes
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