183 research outputs found
Pressure-induced enhancement of superconductivity and superconducting-superconducting transition in CaC
We measured the electrical resistivity, , of superconducting
CaC at ambient and high pressure up to 16 GPa. For 8 GPa, we found
a large increase of with pressure from 11.5 up to 15.1 K. At 8 GPa,
drops and levels off at 5 K above 10 GPa. Correspondingly, the residual
increases by 200 times and the behavior
becomes flat. The recovery of the pristine behavior after depressurization is
suggestive of a phase transition at 8 GPa between two superconducting phases
with good and bad metallic properties, the latter with a lower and more
static disorder
Structural distortions and model Hamiltonian parameters: from LSDA to a tight-binding description of LaMnO_3
The physics of manganites is often described within an effective two-band
tight-binding (TB) model for the Mn e_g electrons, which apart from the kinetic
energy includes also a local "Hund's rule" coupling to the t_{2g} core spin and
a local coupling to the Jahn-Teller (JT) distortion of the oxygen octahedra. We
test the validity of this model by comparing the energy dispersion calculated
for the TB model with the full Kohn-Sham band-structure calculated within the
local spin-density approximation (LSDA) to density functional theory. We
analyze the effect of magnetic order, JT distortions, and "GdFeO_3-type"
tilt-rotations of the oxygen octahedra. We show that the hopping amplitudes are
independent of magnetic order and JT distortions, and that both effects can be
described with a consistent set of model parameters if hopping between both
nearest and next-nearest neighbors is taken into account. We determine a full
set of model parameters from the density functional theory calculations, and we
show that both JT distortions and Hund's rule coupling are required to obtain
an insulating ground state within LSDA. Furthermore, our calculations show that
the "GdFeO_3-type" rotations of the oxygen octahedra lead to a substantial
reduction of the hopping amplitudes but to no significant deviation from the
simple TB model.Comment: replaced with final (published) version with improved presentatio
Unquenched large orbital magnetic moment in NiO
Magnetic properties of NiO are investigated by incorporating the spin-orbit
interaction in the LSDA+U scheme. It is found that the large part of orbital
moment remains unquenched in NiO. The orbital moment contributes about mu_L =
0.29 mu_B to the total magnetic moment of M = 1.93 mu_B, as leads to the
orbital-to-spin angular momentum ratio of L/S = 0.36. The theoretical values
are in good agreement with recent magnetic X-ray scattering measurements.Comment: 4 pages, 2 figure
Pressure induced transition from a spin glass to an itinerant ferromagnet in half doped manganite Ln0.5Ba0.5MnO3 (Ln=Sm and Nd) with quenched disorder
The effect of quenched disorder on the multiphase competition has been
investigated by examining the pressure phase diagram of half doped manganite
Ln0.5B0.5MnO3 (Ln = Sm and Nd) with A-site disorders. Sm0.5Ba0.5MnO3, a spin
glass insulator at ambient pressure, switches to a ferromagnetic metal with
increasing pressure, followed by a rapid increase of the ferromagnetic
transition temperature Tc. The rapid increase of Tc was confirmed also for
Nd0.5Ba0.5MnO3. These observations indicate that the unusual suppression of the
multicritical phase boundary in the A-site disordered system, previously
observed as a function of the averaged A-site ionic radius, is essentially
controlled by the pressure and hence the band width. The effect of quenched
disorder is therefore much enhanced with approaching the multicritical region.Comment: 4 pages including 3 figure
Electronic Structure, Local Moments and Transport in Fe_2VAl
Local spin density approximation calculations are used to elucidate
electronic and magnetic properties of Heusler structure Fe_2VAl. The compound
is found to be a low carrier density semimetal. The Fermi surface has small
hole pockets derived from a triply degenerate Fe derived state at Gamma
compensated by an V derived electron pocket at the X point. The ideal compound
is found to be stable against ferromagnetism. Fe impurities on V sites,
however, behave as local moments. Because of the separation of the hole and
electron pockets the RKKY interaction between such local moments should be
rapidly oscillating on the scale of its decay, leading to the likelihood of
spin-glass behavior for moderate concentrations of Fe on V sites. These
features are discussed in relation to experimental observations of an unusual
insulating state in this compound.Comment: 16 pages, RevTeX, 5 figure
The Magnetic Phase Diagram and the Pressure and Field Dependence of the Fermi Surface in UGe
The ac susceptibility and de Haas-van Alphen (dHvA) effect in UGe are
measured at pressures {\it P} up to 17.7 kbar for the magnetic field {\it B}
parallel to the {\it a} axis, which is the easy axis of magnetization. Two
anomalies are observed at {\it B}({\it P}) and {\it B}({\it P}) ({\it
B} {\it B} at any {\it P}), and the {\it P}-{\it B} phase diagram
is presented. The Fermi surface and quasiparticle mass are found to vary
smoothly with pressure up to 17.7 kbar unless the phase boundary {\it
B}({\it P}) is crossed. The observed dHvA frequencies may be grouped into
three according to their pressure dependences, which are largely positive,
nearly constant or negative. It is suggested that the quasiparticle mass
moderately increases as the boundary {\it B}({\it P}) is approached. DHvA
effect measurements are also performed across the boundary at 16.8 kbar.Comment: to be published in Phys. Rev.
- …