Nonlinear optical response in doped conjugated polymers

Exciton effects on conjugated polymers are investigated in soliton lattice states. We use the Su-Schrieffer-Heeger model with long-range Coulomb interactions. The Hartree-Fock (HF) approximation and the single-excitation configuration- interaction (single-CI) method are used to obtain optical absorption spectra. The third-harmonic generation (THG) at off-resonant frequencies is calculated as functions of the soliton concentration and the chain length of the polymer. The magnitude of the THG at the 10 percent doping increases by the factor about 10^2 from that of the neutral system. This is owing to the accumulation of the oscillator strengths at the lowest exciton with increasing the soliton concentration. The increase by the order two is common for several choices of Coulomb interaction strengths.Comment: Accepted for publication in J. Phys.: Condens. Matte

Origin of intrinsic dark count in superconducting nanowire single-photon detectors

The origin of the decoherence in superconducting nanowire single-photon detectors, the so-called dark count, was investigated. We measured the direct-current characteristics and bias-current dependencies of the dark count rate in a wide range of temperatures from 0.5 K to 4 K, and analyzed the results by theoretical models of thermal fluctuations of vortices. Our results indicate that the current-assisted unbinding of vortex-antivortex pairs is the dominant origin of the dark count.Comment: 10 pages, 2 figure

Multi-Modes Phonon Softening in Two-Dimensional Electron-Lattice System

Phonon dispersion in a two-dimensional electron-lattice system described by a two-dimensional square-lattice version of Su-Schrieffer-Heeger's model and having the half-filled electronic band is studied theoretically at temperatures higher than the mean field critical temperature of the Peierls transition. When the temperature is lowered from the higher region down to the critical one, softening of multi phonon modes which have wave vectors equal to the nesting vector \vv{Q}=(\pi/a,\pi/a) with $a$ the lattice constant or parallel to \vv{Q} is observed. Although both of the transverse and longitudinal modes are softened at the critical temperature in the case of the wave vector equal to \vv{Q}, only the transverse modes are softened for other wave vectors parallel to \vv{Q}. This behavior is consistent with the Peierls distortions at lower temperatures.Comment: 10 pages, 5 Figure

Detection-dependent six-photon NOON state interference

NOON state interference (NOON-SI) is a powerful tool to improve the phase sensing precision, and can play an important role in quantum sensing and quantum imaging. However, most of the previous NOON-SI experiments only investigated the center part of the interference pattern, while the full range of the NOON-SI pattern has not yet been well explored.In this Letter, we experimentally and theoretically demonstrate up to six-photon NOON-SI and study the properties of the interference patterns over the full range.The multi-photons were generated at a wavelength of 1584 nm from a PPKTP crystal in a parametric down conversion process.It was found that the shape, the coherence time and the visibility of the interference patterns were strongly dependent on the detection schemes.This experiment can be used for applications which are based on the envelope of the NOON-SI pattern, such as quantum spectroscopy and quantum metrology.Comment: 5 pages, 3 figure