2 research outputs found
Evidence for two distinct scales of current flow in polycrystalline Sm and Nd iron oxypnictides
Early studies have found quasi-reversible magnetization curves in
polycrystalline bulk rare-earth iron oxypnictides that suggest either
wide-spread obstacles to intergranular current or very weak vortex pinning. In
the present study of polycrystalline samarium and neodymium rare-earth iron
oxypnictide samples made by high pressure synthesis, the hysteretic
magnetization is significantly enhanced. Magneto optical imaging and study of
the field dependence of the remanent magnetization as a function of particle
size both show that global currents over the whole sample do exist but that the
intergranular and intragranular current densities have distinctively different
temperature dependences and differ in magnitude by about 1000. Assuming that
the highest current density loops are restricted to circulation only within
grains leads to values of ~5 MA/cm2 at 5 K and self field, while whole-sample
current densities, though two orders of magnitude lower are 1000-10000 A/cm2,
some two orders of magnitude higher than in random polycrystalline cuprates. We
cannot yet be certain whether this large difference in global and intragrain
current density is intrinsic to the oxypnictides or due to extrinsic barriers
to current flow, because the samples contain significant second phase, some of
which wets the grain boundaries and produces evidences of SNS proximity effect
in the whole sample critical current.Comment: 28 pages, 14 figure
Evidence for Supercurrent Connectivity in Conglomerate Particles in NdFeAsO1-d
Here we use global and local magnetometry and Hall probe imaging to
investigate the electromagnetic connectivity of the superconducting current
path in the oxygen-deficient fluorine-free Nd-based oxypnictides. High
resolution transmission electron microscopy and scanning electron microscopy
show strongly-layered crystallites, evidence for a ~ 5nm amorphous oxide around
individual particles, and second phase neodymium oxide which may be responsible
for the large paramagnetic background at high field and at high temperatures.
From global magnetometry and electrical transport measurements it is clear
that there is a small supercurrent flowing on macroscopic sample dimensions
(mm), with a lower bound for the average (over this length scale) critical
current density of the order of 103 A/cm2. From magnetometry of powder samples
and local Hall probe imaging of a single large conglomerate particle ~120
microns it is clear that on smaller scales, there is better current
connectivity with a critical current density of the order of 5 x 104 A/cm2. We
find enhanced flux creep around the second peak anomaly in the magnetisation
curve and an irreversibility line significantly below Hc2(T) as determined by
ac calorimetry.Comment: 11 pages, 4 figure