4,511 research outputs found
Magnetic ground state of pyrochlore oxides close to metal-insulator boundary probed by muon spin rotation
Magnetism of ruthernium pyrochlore oxides A2Ru2O7 (A = Hg, Cd, Ca), whose
electronic properties within a localized ion picture are characterized by
non-degenerate t2g orbitals (Ru5+, 4d3) and thereby subject to geometrical
frustration, has been investigated by muon spin rotation/relaxation (muSR)
technique. The A cation (mostly divalent) was varied to examine the effect of
covalency (Hg > Cd > Ca) on their electronic property. In a sample with A = Hg
that exhibits a clear metal-insulator (MI) transition below >> 100 K (which is
associated with a weak structural transition), a nearly commensurate magnetic
order is observed to develop in accordance with the MI transition. Meanwhile,
in the case of A = Cd where the MI transition is suppressed to the level of
small anomaly in the resistivity, the local field distribution probed by muon
indicates emergence of a certain magnetic inhomogeneity below {\guillemotright}
30 K. Moreover, in Ca2Ru2O7 that remains metallic, we find a highly
inhomogeneous local magnetism below >>25 K that comes from randomly oriented Ru
moments and thus described as a "frozen spin liquid" state. The systematic
trend of increasing randomness and itinerant character with decreasing
covalency suggests close relationship between these two characters. As a
reference for the effect of orbital degeneracy and associated Jahn-Teller
instability, we examine a tetravalent ruthernium pyrochlore, Tl2Ru2O7 (Ru4+,
4d4), where the result of muSR indicates a non-magnetic ground state that is
consistent with the formation of the Haldane chains suggested by neutron
diffraction experiment.Comment: 12 pages, 13 figure
Incommensurate spin correlations induced by magnetic Fe ions substituted into overdoped Bi1.75Pb0.35Sr1.90CuO6+z
Spin correlations in the overdoped region of Bi1.75Pb0.35Sr1.90CuO6+z have
been explored with Fe-doped single crystals characterized by neutron
scattering, muon-spin-rotation (muSR) spectroscopy, and magnetic susceptibility
measurements. Static incommensurate spin correlations induced by the Fe spins
are revealed by elastic neutron scattering. The resultant incommensurability
delta is unexpectedly large (~0.2 r.l.u.), as compared with delta ~ 1/8 in
overdoped superconductor La2-xSrxCuO4. Intriguingly, the large delta in this
overdoped region is close to the hole concentration p. This result is
reminiscent of the delta ~ p trend observed in underdoped La2-xSrxCuO4;
however, it is inconsistent with the saturation of delta in the latter compound
in the overdoped regime. While our findings in Fe-doped
Bi1.75Pb0.35Sr1.90CuO6+z support the commonality of incommensurate spin
correlations in high-Tc cuprate superconductors, they also suggest that the
magnetic response might be dominated by a distinct mechanism in the overdoped
region.Comment: 4 pages, 5 figures. Revision in introduction, discussion, and
conclusion
Insular superconductivity in Co-doped iron pnictide CaFeCoAsF
The presence of macroscopic phase separation between the superconducting and
magnetic phases in \cfcaf is demonstrated by muon spin rotation (muSR)
measurements conducted across their phase boundaries (x=0.05-0.15). The
magnetic phase tends to retain the high transition temperature (T_m > T_c),
while Co-doping induces strong randomness. The volumetric fraction of
superconducting phase is nearly proportional to the Co content with
constant superfluid density. These observations suggest the formation of
superconducting "islands" (or domains) associated with Co ions in the
FeAs layers, indicating a very short coherence length.Comment: 5 pages, 5 figure
Two dimensionality in quasi one-dimensional cobalt oxides
By means of muon spin rotation and relaxation (SR) techniques, we have
investigated the magnetism of quasi one-dimensional (1D) cobalt oxides
CoO (=Ca, Sr and Ba, =1, 2, 3, 5 and
), in which the 1D CoO chain is surrounded by six equally spaced
chains forming a triangular lattice in the -plane, using polycrystalline
samples, from room temperature down to 1.8 K. For the compounds with =1 - 5,
transverse field SR experiments showed the existence of a magnetic
transition below 100 K. The onset temperature of the transition () was found to decrease with ; from 100 K for =1 to 60 K for
=5. A damped muon spin oscillation was observed only in the sample with
=1 (CaCoO), whereas only a fast relaxation obtained even at 1.8
K in the other three samples. In combination with the results of susceptibility
measurements, this indicates that a two-dimensional short-range
antiferromagnetic (AF) order appears below for all
compounds with =1 - 5; but quasi-static long-range AF order formed only in
CaCoO, below 25 K. For BaCoO (=), as decreased
from 300 K, 1D ferromagnetic (F) order appeared below 53 K, and a sharp 2D AF
transition occurred at 15 K.Comment: 12 pages, 14 figures, and 2 table
Contrasting Pressure Effects in Sr2VFeAsO3 and Sr2ScFePO3
We report the resistivity measurements under pressure of two Fe-based
superconductors with a thick perovskite oxide layer, Sr2VFeAsO3 and Sr2ScFePO3.
The superconducting transition temperature Tc of Sr2VFeAsO3 markedly increases
with increasing pressure. Its onset value, which was Tc{onset}=36.4 K at
ambient pressure, increases to Tc{onset}=46.0 K at ~4 GPa, ensuring the
potential of the "21113" system as a high-Tc material. However, the
superconductivity of Sr2ScFePO3 is strongly suppressed under pressure. The
Tc{onset} of ~16 K decreases to ~5 K at ~4 GPa, and the zero-resistance state
is almost lost. We discuss the factor that induces this contrasting pressure
effect.Comment: 5 pages, 4 figures, to be published in J. Phys. Soc. Jpn. No.12
(2009
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