6,272 research outputs found
One-Electron Ionization of Multielectron Systems in Strong Nonresonant Laser Fields
We present a novel approach to calculating strong field ionization dynamics
of multielectron molecular targets. Adopting a multielectron wavefunction
ansatz based on field-free ab initio neutral and ionic multielectron states, a
set of coupled time-dependent single-particle Schroedinger equations describing
the neutral amplitude and continuum electron are constructed. These equations,
amenable to direct numerical solution or further analytical treatment, allow
one to study multielectron effects during strong field ionization, recollision,
and high harmonic generation. We apply the method to strong field ionization of
CO_2, and suggest the importance of intermediate core excitation to explain
previous failure of analytical models to reproduce experimental ionization
yields for this molecule.Comment: 25 pages, 6 figure
Ultralong-Range Rydberg Molecules in a Divalent-Atomic System
We report the creation of ultralong-range Sr molecules comprising one
ground-state atom and one atom in a Rydberg state
for ranging from 29 to 36. Molecules are created in a trapped ultracold
atomic gas using two-photon excitation near resonant with the
intermediate state, and their formation is detected through ground-state atom
loss from the trap. The observed molecular binding energies are fit with the
aid of first-order perturbation theory that utilizes a Fermi pseudopotential
with effective -wave and -wave scattering lengths to describe the
interaction between an excited Rydberg electron and a ground-state Sr atom.Comment: 5 pages, 2 figure
Lifetimes of ultralong-range strontium Rydberg molecules in a dense BEC
The lifetimes and decay channels of ultralong-range Rydberg molecules created
in a dense BEC are examined by monitoring the time evolution of the Rydberg
population using field ionization. Studies of molecules with values of
principal quantum number, , in the range to that contain tens
to hundreds of ground state atoms within the Rydberg electron orbit show that
their presence leads to marked changes in the field ionization characteristics.
The Rydberg molecules have lifetimes of s, their destruction
being attributed to two main processes: formation of Sr ions through
associative ionization, and dissociation induced through -changing
collisions. The observed loss rates are consistent with a reaction model that
emphasizes the interaction between the Rydberg core ion and its nearest
neighbor ground-state atom. The measured lifetimes place strict limits on the
time scales over which studies involving Rydberg species in cold, dense atomic
gases can be undertaken and limit the coherence times for such measurements.Comment: 9 pages, 8 figure
A study of packaging and shipping procedures for small electroexplosive devices Final report, May 1, 1966 - Aug. 1, 1967
Packaging, shipping, and shielding procedures for electroexplosive device
Lung metastasectomy for colorectal cancer: The impression of benefit from uncontrolled studies was not supported in a randomized controlled trial
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