15 research outputs found
A Large Blue Shift of the Biexciton State in Tellurium Doped CdSe Colloidal Quantum Dots
The exciton-exciton interaction energy of Tellurium doped CdSe colloidal
quantum dots is experimentally investigated. The dots exhibit a strong Coulomb
repulsion between the two excitons, which results in a huge measured biexciton
blue shift of up to 300 meV. Such a strong Coulomb repulsion implies a very
narrow hole wave function localized around the defect, which is manifested by a
large Stokes shift. Moreover, we show that the biexciton blue shift increases
linearly with the Stokes shift. This result is highly relevant for the use of
colloidal QDs as optical gain media, where a large biexciton blue shift is
required to obtain gain in the single exciton regime.Comment: 9 pages, 4 figure