Magnetic shape-memory effect in SrRuO3_3

Like most perovskites, SrRuO$_3$ exhibits structural phase transitions associated with rotations of the RuO$_6$ octahedra. The application of moderate magnetic fields in the ferromagnetically ordered state allows one to fully control these structural distortions, although the ferromagnetic order occurs at six times lower temperature than the structural distortion. Our neutron diffraction and macroscopic measurements unambiguously show that magnetic fields rearrange structural domains, and that for the field along a cubic [110]$_c$ direction a fully detwinned crystal is obtained. Subsequent heating above the Curie temperature causes a magnetic shape-memory effect, where the initial structural domains recover

Low-energy excitations in the magnetized state of the bond-alternating quantum S=1 chain system NTENP

High intensity inelastic neutron scattering experiments on the S=1 quasi-one-dimensional bond-alternating antiferromagnet Ni(C9D24N4)(NO2)ClO4 (NTENP) are performed in magnetic fields of up to 14.8~T. Excitation in the high field magnetized quantum spin solid (ordered) phase are investigated. In addition to the previously observed coherent long-lived gap excitation [M. Hagiwara et al., Phys. Rev. Lett 94, 177202 (2005)], a broad continuum is detected at lower energies. This observation is consistent with recent numerical studies, and helps explain the suppression of the lowest-energy gap mode in the magnetized state of NTENP. Yet another new feature of the excitation spectrum is found at slightly higher energies, and appears to be some kind of multi-magnon state.Comment: 5 pages, 4 fugure

Fractional spinon excitations in the quantum Heisenberg antiferromagnetic chain

Assemblies of interacting quantum particles often surprise us with properties that are difficult to predict. One of the simplest quantum many-body systems is the spin 1/2 Heisenberg antiferromagnetic chain, a linear array of interacting magnetic moments. Its exact ground state is a macroscopic singlet entangling all spins in the chain. Its elementary excitations, called spinons, are fractional spin 1/2 quasiparticles; they are created and detected in pairs by neutron scattering. Theoretical predictions show that two-spinon states exhaust only 71% of the spectral weight while higher-order spinon states, yet to be experimentally located, are predicted to participate in the remaining. Here, by accurate absolute normalization of our inelastic neutron scattering data on a compound realizing the model, we account for the full spectral weight to within 99(8)%. Our data thus establish and quantify the existence of higher-order spinon states. The observation that within error bars, the entire weight is confined within the boundaries of the two-spinon continuum, and that the lineshape resembles a rescaled two-spinon one, allow us to develop a simple physical picture for understanding multi-spinon excitations.Comment: 22 pages, 4 figures, Supplementary material

Spin gaps and magnetic structure of NaxCoO2

We present two experiments that provide information on spin anisotropy and the magnetic structure of NaxCoO2. First, we report low-energy neutron inelastic scattering measurements of the zone-center magnetic excitations in the magnetically ordered phase of Na0.75CoO2. The energy spectra suggest the existence of two gaps, and are very well fitted by a spin-wave model with both in-plane and out-of-plane anisotropy terms. The gap energies decrease with increasing temperature and both gaps are found to have closed when the temperature exceeds the magnetic ordering temperature T_m~22 K. Secondly, we present neutron diffraction studies of Na0.85CoO2 with a magnetic field applied approximately parallel to the c axis. For fields in excess of ~8T a magnetic Bragg peak was observed at the (0,0,3) position in reciprocal space. We interpret this as a spin-flop transition of the A-type antiferromagnetic structure, and we show that the spin-flop field is consistent with the size of the anisotropy gap.Comment: 9 pages, 7 figure

Spin Susceptibility of the Topological Superconductor UPt3 from Polarized Neutron Diffraction

Experiment and theory indicate that UPt3 is a topological superconductor in an odd-parity state, based in part from temperature independence of the NMR Knight shift. However, quasiparticle spin-flip scattering near a surface, where the Knight shift is measured, might be responsible. We use polarized neutron scattering to measure the bulk susceptibility with H||c, finding consistency with the Knight shift but inconsistent with theory for this field orientation. We infer that neither spin susceptibility nor Knight shift are a reliable indication of odd-parity