Local measures of fluctuations in inhomogeneous liquids: Statistical mechanics and illustrative applications

We show in detail how three one-body fluctuation profiles, namely the local compressibility, the local thermal susceptibility, and the reduced density, can be obtained from a statistical mechanical many-body description of classical particle-based systems. We present several different and equivalent routes to the definition of each fluctuation profile, facilitating their explicit numerical calculation in inhomogeneous equilibrium systems. This underlying framework is used for the derivation of further properties such as hard wall contact theorems and novel types of inhomogeneous one-body Ornstein-Zernike equations. The practical accessibility of all three fluctuation profiles is exemplified by grand canonical Monte Carlo simulations that we present for hard sphere, Gaussian core and Lennard-Jones fluids in confinement.Comment: 17 pages, 8 figure

Enhanced colloidal transport in twisted magnetic patterns

Bilayers of two-dimensional materials twisted at specific angles can exhibit exceptional properties such as the occurrence of unconventional superconductivity in twisted graphene. We demonstrate here that novel phenomena in twisted materials emerges also in particle-based classical systems. We study the transport of magnetic colloidal particles driven by a drift force and located between two twisted periodic magnetic patterns with either hexagonal or square symmetry. The magnetic potential generated by patterns twisted at specific magic angles develops flat channels, which increase the mobility of the colloidal particles compared to that in single patterns. We characterize the effect of the temperature and that of the magnitude of the drift force on the colloidal mobility. The transport is more enhanced in square than in hexagonal twisted patterns. Our work extends twistronics to classical soft matter systems with potential applications to lab-on-a-chip devices

Colloidal transport in twisted lattices of optical tweezers

We simulate the transport of colloidal particles driven by a static and homogeneous drift force, and subject to the optical potential created by two lattices of optical tweezers. The lattices of optical tweezers are parallel to each other, shifted, and rotated by a twist angle. Due to a negative interference between the potential of the two lattices, flat channels appear in the total optical potential. At specific twist angles, known as magic-angles, the flat channels percolate the entire system and the colloidal particles can then be transported using a weak external drift force. We characterize the transport in both square and hexagonal lattices of twisted optical tweezer