The effect of magnetic dipolar interactions on the interchain spin wave dispersion in CsNiF_3

Inelastic neutron scattering measurements were performed on the ferromagnetic chain system CsNiF_3 in the collinear antiferromagnetic ordered state below T_N = 2.67K. The measured spin wave dispersion was found to be in good agreement with linear spin wave theory including dipolar interactions. The additional dipole tensor in the Hamiltonian was essential to explain some striking phenomena in the measured spin wave spectrum: a peculiar feature of the dispersion relation is a jump at the zone center, caused by strong dipolar interactions in this system. The interchain exchange coupling constant and the planar anisotropy energy were determined within the present model to be J'/k_B = -0.0247(12)K and A/k_B = 3.3(1)K. This gives a ratio J/J' \approx 500, using the previously determined intrachain coupling constant J/k_B = 11.8$. The small exchange energy J' is of the same order as the dipolar energy, which implies a strong competition between the both interactions.Comment: 18 pages, TeX type, 7 Postscript figures included. To be published in Phys. Rev.

Pure hydrogen low-temperature plasma exposure of HOPG and graphene: Graphane formation?

Single- and multilayer graphene and highly ordered pyrolytic graphite (HOPG) were exposed to a pure hydrogen low-temperature plasma (LTP). Characterizations include various experimental techniques such as photoelectron spectroscopy, Raman spectroscopy and scanning probe microscopy. Our photoemission measurement shows that hydrogen LTP exposed HOPG has a diamond-like valence-band structure, which suggests double-sided hydrogenation. With the scanning tunneling microscopy technique, various atomic-scale charge-density patterns were observed, which may be associated with different C-H conformers. Hydrogen-LTP-exposed graphene on SiO₂ has a Raman spectrum in which the D peak to G peak ratio is over 4, associated with hydrogenation on both sides. A very low defect density was observed in the scanning probe microscopy measurements, which enables a reverse transformation to graphene. Hydrogen-LTP-exposed HOPG possesses a high thermal stability, and therefore, this transformation requires annealing at over 1000 °C

Constraints on the density dependence of the symmetry energy

Collisions involving 112Sn and 124Sn nuclei have been simulated with the improved Quantum Molecular Dynamics transport model. The results of the calculations reproduce isospin diffusion data from two different observables and the ratios of neutron and proton spectra. By comparing these data to calculations performed over a range of symmetry energies at saturation density and different representations of the density dependence of the symmetry energy, constraints on the density dependence of the symmetry energy at sub-normal density are obtained. Results from present work are compared to constraints put forward in other recent analysis.Comment: 8 pages, 4 figures,accepted for publication in Phy. Rev. Let

Teleportation: from probability distributions to quantum states

The role of the off-diagonal density matrix elements of the entangled pair is investigated in quantum teleportation of a qbit. The dependence between them and the off-diagonal elements of the teleported density matrix is shown to be linear. In this way the ideal quantum teleportation is related to an entirely classical communication protocol: the one-time pad cypher. The latter can be regarded as the classical counterpart of Bennett's quantum teleportation scheme. The quantum-to-classical transition is demonstrated on the statistics of a gedankenexperiment.Comment: 11 pages, 1 figure, accepted for publication in J. Phys. A (Math. Gen.

Reaction of selected carbohydrate aldehydes with benzylmagnesium halides: benzyl versus o-tolyl rearrangement

The Grignard reaction of 2,3-O-isopropylidene-alpha-D-lyxo-pentodialdo-1,4-furanoside and benzylmagnesium chloride (or bromide) afforded a non-separable mixture of diastereomeric benzyl carbinols and diastereomeric o-tolyl carbinols. The latter resulted from an unexpected benzyl to o-tolyl rearrangement. The proportion of benzyl versus o-tolyl derivatives depended on the reaction conditions. Benzylmagnesium chloride afforded predominantly o-tolyl carbinols while the application of benzylmagnesium bromide led preferably to the o-tolyl carbinols only when used in excess or at higher temperatures. The structures of the benzyl and o-tolyl derivatives were confirmed unambiguously by NMR spectral data and X-ray crystallographic analysis of their 5-ketone analogues obtained by oxidation of the corresponding mixture of diastereomeric carbinols. A possible mechanism for the Grignard reaction leading to the benzyl -> o-tolyl rearrangement is also proposed

Device-spectroscopy of magnetic field effects in a polyfluorene organic light-emitting diode

We perform charge-induced absorption and electroluminescence spectroscopy in a polyfluorene organic magnetoresistive device. Our experiments allow us to measure the singlet exciton, triplet exciton and polaron densities in a live device under an applied magnetic field, and to distinguish between three different models that were proposed to explain organic magnetoresistance. These models are based on different spin-dependent interactions, namely exciton formation, triplet exciton-polaron quenching and bipolaron formation. We show that the singlet exciton, triplet exciton and polaron densities and conductivity all increase with increasing magnetic field. Our data are inconsistent with the exciton formation and triplet-exciton polaron quenching models.Comment: 4 pages, two figure

On The Evolution of Magnetic White Dwarfs

We present the first radiation magnetohydrodynamics simulations of the atmosphere of white dwarf stars. We demonstrate that convective energy transfer is seriously impeded by magnetic fields when the plasma-beta parameter, the thermal to magnetic pressure ratio, becomes smaller than unity. The critical field strength that inhibits convection in the photosphere of white dwarfs is in the range B = 1-50 kG, which is much smaller than the typical 1-1000 MG field strengths observed in magnetic white dwarfs, implying that these objects have radiative atmospheres. We have then employed evolutionary models to study the cooling process of high-field magnetic white dwarfs, where convection is entirely suppressed during the full evolution (B > 10 MG). We find that the inhibition of convection has no effect on cooling rates until the effective temperature (Teff) reaches a value of around 5500 K. In this regime, the standard convective sequences start to deviate from the ones without convection owing to the convective coupling between the outer layers and the degenerate reservoir of thermal energy. Since no magnetic white dwarfs are currently known at the low temperatures where this coupling significantly changes the evolution, effects of magnetism on cooling rates are not expected to be observed. This result contrasts with a recent suggestion that magnetic white dwarfs with Teff < 10,000 K cool significantly slower than non-magnetic degenerates.Comment: 11 pages, 12 figures, accepted for publication in the Astrophysical Journa