Stability of Bose Einstein condensates of hot magnons in YIG

We investigate the stability of the recently discovered room temperature Bose-Einstein condensate (BEC) of magnons in Ytrrium Iron Garnet (YIG) films. We show that magnon-magnon interactions depend strongly on the external field orientation, and that the BEC in current experiments is actually metastable - it only survives because of finite size effects, and because the BEC density is very low. On the other hand a strong field applied perpendicular to the sample plane leads to a repulsive magnon-magnon interaction; we predict that a high-density magnon BEC can then be formed in this perpendicular field geometry.Comment: Submitted to Physical Review Letter

Ab Initio Calculation of Impurity Effects in Copper Oxide Materials

We describe a method for calculating, within density functional theory, the electronic structure associated with typical defects which substitute for Cu in the CuO2 planes of high-Tc superconducting materials. The focus is primarily on Bi2Sr2CaCu2O8, the material on which most STM measurements of impurity resonances in the superconducting state have been performed. The magnitudes of the effective potentials found for Zn, Ni and vacancies on the in-plane Cu sites in this host material are remarkably consistent with phenomenological fits of potential scattering models to STM resonance energies. The effective potential ranges are quite short, of order 1 A with weak long range tails, in contrast to some current models of extended potentials which attempt to fit STM data. For the case of Zn and Cu vacancies, the effective potentials are strongly repulsive, and states on the impurity site near the Fermi level are simply removed. The local density of states (LDOS) just above the impurity is nevertheless found to be a maximum in the case of Zn and a local minimum in case of the vacancy, in agreement with experiment. The Zn and Cu vacancy patterns are explained as due to the long-range tails of the effective impurity potential at the sample surface. The case of Ni is richer due to the Ni atom's strong hybridization with states near the Fermi level; in particular, the short range part of the potential is attractive, and the LDOS is found to vary rapidly with distance from the surface and from the impurity site. We propose that the current controversy surrounding the observed STM patterns can be resolved by properly accounting for the effective impurity potentials and wave-functions near the cuprate surface. Other aspects of the impurity states for all three species are discussed.Comment: 37 pp. pdf including figures, submitted to Phys. Rev.

Long-term, continuous air quality monitoring in a cross-sectional study of three UK non-domestic buildings

Long-term, continuous air quality monitoring has been carried out alongside seasonal passive sampling within a case study a hospital, school and office building, representing a cross-section of the UK non-domestic sector. This approach aimed at adopting state of the art sensor technology to provide a greater understanding of the variations in indoor air quality over time and how these variations relate to both building operation and occupant behavior. The results highlight how the relationship between indoor and outdoor air evolves considerably on both short and long-term basis, with varying behaviors then seen across different sources of pollutants. The mechanically ventilated hospital and school buildings demonstrate the effectiveness of particulate filters, with very low internal concentrations of PM2.5. However, high ventilation rates, combined with the absence of any filtration of NO2, resulted in the hospital having the highest indoor concentrations of NO2 and the highest associated indoor-outdoor ratio. Morning and evening traffic related peaks in NO2 can be observed indoors, with their penetration dependent upon the delivered ventilation rates. This demonstrates the impact of adopting high ventilation rates during peak traffic, and the consequences of CO2 based demand-controlled ventilation systems in polluted urban areas without full filtration. The naturally ventilated office then demonstrates significant seasonal variations, with increased ventilation openings resulting in indoor NO2 concentrations in the summer exceeding those in the winter, despite significant reductions in ambient levels. Conversely, concentrations of indoor pollutants are seen to reduce with increasing ventilation rates, demonstrating the complex balance between the dilution of indoor pollutants and penetration of outdoor sources. Despite significant reductions from the winter to the summer (21.6–11.2 μg/m3), all formaldehyde measurements in the naturally ventilated office exceeded guideline values, indicating improved guidance and product labelling schemes may be required to achieve these guideline concentrations and reduce associated health risks

Quantum Thermoactivation of Nanoscale Magnets

The integral relaxation time describing the thermoactivated escape of a uniaxial quantum spin system interacting with a boson bath is calculated analytically in the whole temperature range. For temperatures T much less than the barrier height \Delta U, the level quantization near the top of the barrier and the strong frequency dependence of the one-boson transition probability can lead to the regularly spaced deep minima of the thermoactivation rate as a function of the magnetic field applied along the z axis.Comment: 4 pages, no figures, rejected from Phys. Rev. Let

An alternate model for magnetization plateaus in the molecular magnet V_15

Starting from an antiferromagnetic Heisenberg Hamiltonian for the fifteen spin-1/2 ions in V_15, we construct an effective spin Hamiltonian involving eight low-lying states (spin-1/2 and spin-3/2) coupled to a phonon bath. We numerically solve the time-dependent Schrodinger equation of this system, and obtain the magnetization as a function of temperature in a time-dependent magnetic field. The magnetization exhibits unusual patterns of hysteresis and plateaus as the field sweep rate and temperature are varied. The observed plateaus are not due to quantum tunneling but are a result of thermal averaging. Our results are in good agreement with recent experimental observations.Comment: Revtex, 4 pages, 5 eps figure

Quantum Relaxation of Magnetisation in Magnetic Particles

At temperatures below the magnetic anisotropy energy, monodomain magnetic systems (small particles, nanomagnetic devices, etc.) must relax quantum mechanically. This quantum relaxation must be mediated by the coupling to both nuclear spins and phonons (and electrons if either particle or substrate is conducting. We analyze the effect of each of these couplings, and then combine them. Conducting systems can be modelled by a "giant Kondo" Hamiltonian, with nuclear spins added in as well. At low temperatures, even microscopic particles on a conducting substrate (containing only $10-50$ spins) will have their magnetisation frozen over millenia by a combination of electronic dissipation and the "degeneracy blocking" caused by nuclear spins. Raising the temperature leads to a sudden unblocking of the spin dynamics at a well defined temperature. Insulating systems are quite different. The relaxation is strongly enhanced by the coupling to nuclear spins. At short times the magnetisation of an ensemble of particles relaxes logarithmically in time, after an initial very fast decay; this relaxation proceeds entirely via the nuclear spins. At longer times phonons take over, but the decay rate is still governed by the temperature-dependent nuclear bias field acting on the particles - decay may be exponential or power-law depending on the temperature. The most surprising feature of the results is the pivotal role played by the nuclear spins. The results are relevant to any experiments on magnetic particles in which interparticle dipolar interactions are unimportant. They are also relevant to future magnetic device technology.Comment: 30 pages, RevTex, e:mail , Submitted to J.Low Temp.Phys. on 1 Nov. 199

Thermally assisted domain walls quantum tunneling at the high temperature range

A theoretical and numerical investigations of the quantum tunneling of the domain walls in ferromagnets and weak ferromagnets was performed taking into account the interaction between walls and thermal excitations of a crystal. The numerical method for calculations of the probability of a thermally stimulated quantum depinning as the function of temperature at the wide temperature range has been evolved.Comment: 5 pages, 3 figure

Quantum Dynamics of a Bose Superfluid Vortex

We derive a fully quantum-mechanical equation of motion for a vortex in a 2-dimensional Bose superfluid, in the temperature regime where the normal fluid density $\rho_n(T)$ is small. The coupling between the vortex "zero mode" and the quasiparticles has no term linear in the quasiparticle variables -- the lowest-order coupling is quadratic. We find that as a function of the dimensionless frequency $\tilde \Omega = \hbar \Omega/k_BT$, the standard Hall-Vinen/Iordanskii equations are valid when $\tilde \Omega \ll 1$ (the "classical regime"), but elsewhere, the equations of motion become highly retarded, with significant experimental implications when $\tilde \Omega \gtrsim 1$.Comment: 12 pages (4 pages + supp info), 2 figures, accepted to PR

Suppression of tunneling by interference in half-integer--spin particles

Within a wide class of ferromagnetic and antiferromagnetic systems, quantum tunneling of magnetization direction is spin-parity dependent: it vanishes for magnetic particles with half-integer spin, but is allowed for integer spin. A coherent-state path integral calculation shows that this topological effect results from interference between tunneling paths.Comment: 14 pages (RevTeX), 2 postscript figures available upon reques