73 research outputs found
Inherent-opening-controlled pattern formation in carbon nanotube arrays
We have introduced inherent openings into densely packed carbon nanotube arrays to study self-organized pattern formation when the arrays undergo a wetting–dewetting treatment from nanotube tips. These inherent openings, made of circular or elongated hollows in nanotube mats, serve as dewetting centres, from where liquid recedes from. As the dewetting centres initiate dry zones and the dry zones expand, surrounding nanotubes are pulled away from the dewetting centres by liquid surface tension. Among short nanotubes, the self-organized patterns are consistent with the shape of the inherent openings, i.e. slender openings lead to elongated trench-like structures, and circular holes result in relatively round nest-like arrangements. Nanotubes in a relatively high mat are more connected, like in an elastic body, than those in a short mat. Small cracks often initialize themselves in a relatively high mat, along two or more adjacent round openings; each of the cracks evolves into a trench as liquid dries up. Self-organized pattern control with inherent openings needs to initiate the dewetting process above the nanotube tips. If there is no liquid on top, inherent openings barely enlarge themselves after the wetting–dewetting treatment
Determining Pair Interactions from Structural Correlations
We examine metastable configurations of a two-dimensional system of
interacting particles on a quenched random potential landscape and ask how the
configurational pair correlation function is related to the particle
interactions and the statistical properties of the potential landscape.
Understanding this relation facilitates quantitative studies of magnetic flux
line interactions in type II superconductors, using structural information
available from Lorentz microscope images or Bitter decorations.
Previous work by some of us supported the conjecture that the relationship
between pair correlations and interactions in pinned flux line ensembles is
analogous to the corresponding relationship in the theory of simple liquids.
The present paper aims at a more thorough understanding of this relation. We
report the results of numerical simulations and present a theory for the low
density behavior of the pair correlation function which agrees well with our
simulations and captures features observed in experiments. In particular, we
find that the resulting description goes beyond the conjectured classical
liquid type relation and we remark on the differences.Comment: 7 pages, 6 figures. See also http://rainbow.uchicago.edu/~grier
A Focused Laser Beam: A Useful and Versatile Tool for 1D Nanomaterials Research: A Review
10.1016/j.jmst.2014.12.006Journal of Materials Science and Technology316616-62
Upcycling fish scales through heating for steganography and Rhodamine B adsorption application
Abstract With increasing population and limited resources, a potential route for improving sustainability is increased reuse of waste materials. By re-looking at wastes, interesting properties and multifunctionalities can be discovered in materials previously explored. Despite years of research on bio-compatible fish scales, there is limited study on the fluorescence property of this abundant waste material. Controlled denaturation of collagen and introduction of defects can serve as a means to transform the fluorescence property of these fish scale wastes while providing more adsorption sites for pollutant removal, turning multifunctional fish scales into a natural steganographic material for transmitting text and images at both the macroscopic and microscopic levels and effectively removing Rhodamine B pollutants (91 % removal) within a short contact time (10 minutes). Our work offers a glimpse into the realm of engineering defects-induced fluorescence in natural material with potential as bio-compatible fluorescence probes while encouraging multidimensional applicability to be established in otherwise overlooked waste resources
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