18,010 research outputs found
Magnetic spin moment reduction in photoexcited ferromagnets through exchange interaction quenching: Beyond the rigid band approximation
The exchange interaction among electrons is one of the most fundamental
quantum mechanical interactions in nature and underlies any magnetic phenomena
from ferromagnetic ordering to magnetic storage. The current technology is
built upon a thermal or magnetic field, but a frontier is emerging to directly
control magnetism using ultrashort laser pulses. However, little is known about
the fate of the exchange interaction. Here we report unambiguously that
photoexcitation is capable of quenching the exchange interaction in all three
ferromagnetic metals. The entire process starts with a small number of
photoexcited electrons which build up a new and self-destructive potential that
collapses the system into a new state with a reduced exchange splitting. The
spin moment reduction follows a Bloch-like law as , where is
the absorbed photon energy and is a scaling exponent. A good agreement
is found between the experimental and our theoretical results. Our findings may
have a broader implication for dynamic electron correlation effects in
laser-excited iron-based superconductors, iron borate, rare-earth
orthoferrites, hematites and rare-earth transition metal alloys.Comment: 16 pages, 3 figures, one supplementary material fil
Generating high-order optical and spin harmonics from ferromagnetic monolayers
High-order harmonic generation (HHG) in solids has entered a new phase of
intensive research, with envisioned band-structure mapping on an ultrashort
time scale. This partly benefits from a flurry of new HHG materials discovered,
but so far has missed an important group. HHG in magnetic materials should have
profound impact on future magnetic storage technology advances. Here we
introduce and demonstrate HHG in ferromagnetic monolayers. We find that HHG
carries spin information and sensitively depends on the relativistic spin-orbit
coupling; and if they are dispersed into the crystal momentum space,
harmonics originating from real transitions can be -resolved and carry
the band structure information. Geometrically, the HHG signal is sensitive to
spatial orientations of monolayers. Different from the optical counterpart, the
spin HHG, though probably weak, only appears at even orders, a consequence of
SU(2) symmetry. Our findings open an unexplored frontier -- magneto-high-order
harmonic generation.Comment: 19 pages, 4 figure
Structural phase control of (LaNdSr)CuO thin films by epitaxial growth technique
Epitaxial growth of (LaNdSr)CuO thin films was
studied by pulsed-laser deposition technique on three different substrates,
SrTiO (100), LaSrAlO (001), and YAlO (001). The
(Nd,Sr,Ce)CuO-type structure appears at the initial growth stage on
SrTiO (100) when the film is deposited under the growth conditions
optimized for (La,Sr)CuO. This (Nd,Sr,Ce)CuO-type structure can
be eliminated by increasing the substrate temperature and the laser repetition
frequency. Films on LaSrAlO (001) maintain a LaCuO-type structure
as bulk samples, but those on YAlO (001) show phase separation into
LaCuO- and NdCuO-type structures. Such complicated results are
explained in terms of the competition between lattice misfit and thermodynamic
conditions. Interestingly the films with LaCuO-type structure prepared
on SrTiO and LaSrAlO show different surface structures and transport
properties. The results indicate the possibility of controlling charge stripes
of (LaNdSr)CuO as was demonstrated in
(La,Ba)CuO thin films by Sato et al. (Phys. Rev. B {\bf 62}, R799
(2000)).Comment: 5 pages, 6 EPS figure, accepted for publication in Phys. Rev.
Extended calculations of energy levels, radiative properties, , hyperfine interaction constants, and Land\'e -factors for nitrogen-like \mbox{Ge XXVI}
Employing two state-of-the-art methods, multiconfiguration
Dirac--Hartree--Fock and second-order many-body perturbation theory, highly
accurate calculations are performed for the lowest 272 fine-structure levels
arising from the , , , ~(), (), and ()
configurations in nitrogen-like Ge XXVI. Complete and consistent atomic data,
including excitation energies, lifetimes, wavelengths, hyperfine structures,
Land\'e -factors, and E1, E2, M1, M2 line strengths, oscillator
strengths, and transition rates among these 272 levels are provided.
Comparisons are made between the present two data sets, as well as with other
available experimental and theoretical values. The present data are accurate
enough for identification and deblending of emission lines involving the
levels, and are also useful for modeling and diagnosing fusion plasmas
Hole Doping Dependence of the Coherence Length in Thin Films
By measuring the field and temperature dependence of magnetization on
systematically doped thin films, the critical current
density and the collective pinning energy are determined in
single vortex creep regime. Together with the published data of superfluid
density, condensation energy and anisotropy, for the first time we derive the
doping dependence of the coherence length or vortex core size in wide doping
regime directly from the low temperature data. It is found that the coherence
length drops in the underdoped region and increases in the overdoped side with
the increase of hole concentration. The result in underdoped region clearly
deviates from what expected by the pre-formed pairing model if one simply
associates the pseudogap with the upper-critical field.Comment: 4 pages, 4 figure
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