Following microscopic motion in a two dimensional glass-forming binary fluid

The dynamics of a binary mixture of large and small discs are studied at temperatures approaching the glass transition using an analysis based on the topology of the Voronoi polygon surrounding each atom. At higher temperatures we find that dynamics is dominated by fluid-like motion that involves particles entering and exiting the nearest-neighbour shells of nearby particles. As the temperature is lowered, the rate of topological moves decreases and motion becomes localised to regions of mixed pentagons and heptagons. In addition we find that in the low temperature state particles may translate significant distances without undergoing changes in their nearest neig hbour shell. These results have implications for dynamical heterogeneities in glass forming liquids.Comment: 12 pages, 7 figure

Aging dynamics in reentrant ferromagnet: Cu0.2_{0.2}Co0.8_{0.8}Cl2_{2}-FeCl3_{3} graphite bi-intercalation compound

Aging dynamics of a reentrant ferromagnet Cu$_{0.2}$Co$_{0.8}$Cl$_{2}$-FeCl$_{3}$ graphite bi-intercalation compound has been studied using AC and DC magnetic susceptibility. This compound undergoes successive transitions at the transition temperatures $T_{c}$ ($= 9.7$ K) and $T_{RSG}$ ($= 3.5$ K). The relaxation rate $S(t)$ exhibits a characteristic peak at $t_{cr}$ close to a wait time $t_{w}$ below $T_{c}$, indicating that the aging phenomena occur in both the reentrant spin glass (RSG) phase below $T_{RSG}$ and the ferromagnetic (FM) phase between $T_{RSG}$ and $T_{c}$. The relaxation rate $S(t)$ ($=\text{d}\chi_{ZFC}(t)/\text{d}\ln t$) in the FM phase exhibits two peaks around $t_{w}$ and a time much shorter than $t_{w}$ under the positive $T$-shift aging, indicating a partial rejuvenation of domains. The aging state in the FM phase is fragile against a weak magnetic-field perturbation. The time ($t$) dependence of $\chi_{ZFC}(t)$ around $t \approx t_{cr}$ is well approximated by a stretched exponential relaxation: $\chi_{ZFC}(t) \approx \exp[-(t/\tau)^{1-n}]$. The exponent $n$ depends on $t_{w}$, $T$, and $H$. The relaxation time $\tau$ ($\approx t_{cr}$) exhibits a local maximum around 5 K, reflecting a chaotic nature of the FM phase. It drastically increases with decreasing temperature below $T_{RSG}$.Comment: 16 pages,16 figures, submitted to Physical Review

Expansion of the Gibbs potential for quantum many-body systems: General formalism with applications to the spin glass and the weakly non-ideal Bose gas

For general quantum systems the power expansion of the Gibbs potential and consequently the power expansion of the self energy is derived in terms of the interaction strength. Employing a generalization of the projector technique a compact representation of the general terms of the expansion results. The general aspects of the approach are discussed with special emphasis on the effects characteristic for quantum systems. The expansion is systematic and leads directly to contributions beyond mean-field of all thermodynamic quantities. These features are explicitly demonstrated and illustrated for two non-trivial systems, the infinite range quantum spin glass and the weakly interacting Bose gas. The Onsager terms of both systems are calculated, which represent the first beyond mean-field contributions. For the spin glass new TAP-like equations are presented and discussed in the paramagnetic region. The investigation of the Bose gas leads to a beyond mean-field thermodynamic description. At the Bose-Einstein condensation temperature complete agreement is found with the results presented recently by alternative techniques.Comment: 17 pages, 0 figures; revised version accepted by Phys Rev

Dynamical Replica Theory for Disordered Spin Systems

We present a new method to solve the dynamics of disordered spin systems on finite time-scales. It involves a closed driven diffusion equation for the joint spin-field distribution, with time-dependent coefficients described by a dynamical replica theory which, in the case of detailed balance, incorporates equilibrium replica theory as a stationary state. The theory is exact in various limits. We apply our theory to both the symmetric- and the non-symmetric Sherrington-Kirkpatrick spin-glass, and show that it describes the (numerical) experiments very well.Comment: 7 pages RevTex, 4 figures, for PR

Local field distributions in spin glasses

Numerical results for the local field distributions of a family of Ising spin-glass models are presented. In particular, the Edwards-Anderson model in dimensions two, three, and four is considered, as well as spin glasses with long-range power-law-modulated interactions that interpolate between a nearest-neighbour Edwards-Anderson system in one dimension and the infinite-range Sherrington-Kirkpatrick model. Remarkably, the local field distributions only depend weakly on the range of the interactions and the dimensionality, and show strong similarities except for near zero local field.Comment: 17 pages, 34 eps-figs included, extensive updates and new results, as to appear in JPA, find related articles at http://www.physics.emory.edu/faculty/boettche

Quantum description of spherical spins

The spherical model for spins describes ferromagnetic phase transitions well, but it fails at low temperatures. A quantum version of the spherical model is proposed. It does not induce qualitative changes near the phase transition. However, it produces a physical low temperature behavior. The entropy is non-negative. Model parameters can be adapted to the description of real quantum spins. Several applications are discussed. Zero-temperature quantum phase transitions are analyzed for a ferromagnet and a spin glass in a transversal field. Their crossover exponents are presented.Comment: 4 pages postscript. Revised version, to appear in Phys. Rev. Let

The 3-SAT problem with large number of clauses in ∞\infty-replica symmetry breaking scheme

In this paper we analyze the structure of the UNSAT-phase of the overconstrained 3-SAT model by studying the low temperature phase of the associated disordered spin model. We derive the $\infty$ Replica Symmetry Broken equations for a general class of disordered spin models which includes the Sherrington - Kirkpatrick model, the Ising $p$-spin model as well as the overconstrained 3-SAT model as particular cases. We have numerically solved the $\infty$ Replica Symmetry Broken equations using a pseudo-spectral code down to and including zero temperature. We find that the UNSAT-phase of the overconstrained 3-SAT model is of the $\infty$-RSB kind: in order to get a stable solution the replica symmetry has to be broken in a continuous way, similarly to the SK model in external magnetic field.Comment: 19 pages, 7 figures; some section improved; iopart styl

No spin glass phase in ferromagnetic random-field random-temperature scalar Ginzburg-Landau model

Krzakala, Ricci-Tersenghi and Zdeborova have shown recently that the random field Ising model with non-negative interactions and arbitrary external magnetic field on an arbitrary lattice does not have a static spin glass phase. In this paper we generalize the proof to a soft scalar spin version of the Ising model: the Ginzburg-Landau model with random magnetic field and random temperature-parameter. We do so by proving that the spin glass susceptibility cannot diverge unless the ferromagnetic susceptibility does.Comment: 9 page

Numerical Results for Ground States of Mean-Field Spin Glasses at low Connectivities

An extensive list of results for the ground state properties of spin glasses on random graphs is presented. These results provide a timely benchmark for currently developing theoretical techniques based on replica symmetry breaking that are being tested on mean-field models at low connectivity. Comparison with existing replica results for such models verifies the strength of those techniques. Yet, we find that spin glasses on fixed-connectivity graphs (Bethe lattices) exhibit a richer phenomenology than has been anticipated by theory. Our data prove to be sufficiently accurate to speculate about some exact results.Comment: 4 pages, RevTex4, 5 ps-figures included, related papers available at http://www.physics.emory.edu/faculty/boettcher

Solution of the local field equations for self-generated glasses

We present a self-consistent local approach to self generated glassiness which is based on the concept of the dynamical mean field theory to many body systems. Using a replica approach to self generated glassiness, we map the problem onto an effective local problem which can be solved exactly. Applying the approach to the Brazovskii-model, relevant to a large class of systems with frustrated micro-phase separation, we are able to solve the self-consistent local theory without using additional approximations. We demonstrate that a glassy state found earlier in this model is generic and does not arise from the use of perturbative approximations. In addition we demonstrate that the glassy state depends strongly on the strength of the frustrated phase separation in that model.Comment: 11 pages, 3 figure