1,031 research outputs found
Pattern formation aspects of electrically charged tri-stable media with implications to bulk heterojunction in organic photovoltaics
A common thread in designing electrochemically-based renewable energy devices
comprises materials that exploit nano-scale morphologies, e.g.,
supercapacitors, batteries, fuel cells, and bulk heterojunction organic
photovoltaics. In these devices, however, Coulomb forces often influence the
fine nano-details of the morphological structure of active layers leading to a
notorious decrease in performance. By focusing on bulk heterojunction organic
photovoltaics as a case model, a self-consistent mean-field framework that
combines binary (bi-stable) and ternary (tri-stable) morphologies with
electrokinetics is presented and analyzed, i.e., undertaking the coupling
between the spatiotemporal evolution of the material and charge dynamics along
with charge transfer at the device electrodes. Particularly, it is shown that
tri-stable composition may stabilize stripe morphology that is ideal bulk
heterojuction. Moreover, since the results rely on generic principles they are
expected to be applicable to a broad range of electrically charged
amphiphilic-type mixtures, such as emulsions, polyelectrolytes, and ionic
liquids.Comment: 8 pages, 4 figure
Magnetization steps in Zn_(1-x)Mn_xO: Four largest exchange constants and single-ion anisotropy
Magnetization steps (MST's) from Mn pairs in several single crystals of
Zn_(1-x)Mn_xO (0.0056<=x<=0.030, and in one powder (x=0.029), were observed.
The largest two exchange constants, J1/kB=-18.2+/-0.5K and J1'/kB=-24.3+/-0.6K,
were obtained from large peaks in the differential susceptibility, dM/dH,
measured in pulsed magnetic fields, H, up to 500 kOe. These two largest J's are
associated with the two inequivalent classes of nearest neighbors (NN's) in the
wurtzite structure. The 29% difference between J1 and J1' is substantially
larger than 13% in CdS:Mn, and 15% in CdSe:Mn. The pulsed-field data also
indicate that, despite the direct contact between the samples and a
superfluid-helium bath, substantial departures from thermal equilibrium
occurred during the 7.4 ms pulse. The third- and fourth-largest J's were
determined from the magnetization M at 20 mK, measured in dc magnetic fields H
up to 90 kOe. Both field orientations H||c and H||[10-10] were studied. (The
[10-10] direction is perpendicular to the c-axis, [0001].) By definition,
neighbors which are not NN's are distant neighbors (DN's). The largest DN
exchange constant (third-largest overall), has the value J/kB=-0.543+/-0.005K,
and is associated with the DN at r=c. Because this is not the closest DN, this
result implies that the J's do not decrease monotonically with the distance r.
The second-largest DN exchange constant (fourth-largest overall), has the value
J/kB=-0.080 K. It is associated with one of the two classes of neighbors that
have a coordination number z=12, but the evidence is insufficient for a
definite unique choice. The dependence of M on the direction of H gives
D/kB=-0.039+/-0.008K, in fair agreement with -0.031 K from earlier EPR work.Comment: 12 pages, 10 figures. Submitted to PR
Single atom quantum walk with 1D optical superlattices
A proposal for the implementation of quantum walks using cold atom technology
is presented. It consists of one atom trapped in time varying optical
superlattices. The required elements are presented in detail including the
preparation procedure, the manipulation required for the quantum walk evolution
and the final measurement. These procedures can be, in principle, implemented
with present technology.Comment: 6 pages, 7 figure
The Single-Particle Structure of Neutron-Rich Nuclei of Astrophysical Interest at the Ornl Hribf
The rapid nuetron-capture process (r process) produces roughly half of the
elements heavier than iron. The path and abundances produced are uncertain,
however, because of the lack of nuclear strucure information on important
neutron-rich nuclei. We are studying nuclei on or near the r-process path via
single-nucleon transfer reactions on neutron-rich radioactive beams at ORNL's
Holifield Radioactive Ion Beam Facility (HRIBF). Owing to the difficulties in
studying these reactions in inverse kinematics, a variety of experimental
approaches are being developed. We present the experimental methods and initial
results.Comment: Proceedings of the Third International Conference on Fission and
Properties of Neutron-Rich Nucle
miR-16 family induces cell cycle arrest by regulating multiple cell cycle genes
MicroRNAs (miRNAs) are a class of small regulatory RNAs that are thought to be involved in diverse biological processes by regulating gene expression. Numerous miRNAs have been identified in various species, and many more miRNAs remain to be detected. Generally, hundreds of mRNAs have been predicted to be potential targets of one miRNA, so it is a great challenge to identify the genuine miRNA targets. Here, we generated the cell lines depleted of Drosha protein and screened dozens of transcripts (including Cyclin D1) regulated potentially by miRNA-mediated RNA silencing pathway. On the basis of miRNA expressing library, we established a miRNA targets reverse screening method by using luciferase reporter assay. By this method, we found that the expression of Cyclin D1 (CCND1) was regulated by miR-16 family directly, and miR-16 induced G1 arrest in A549 cells partially by CCND1. Furthermore, several other cell cycle genes were revealed to be regulated by miR-16 family, including Cyclin D3 (CCND3), Cyclin E1 (CCNE1) and CDK6. Taken together, our data suggests that miR-16 family triggers an accumulation of cells in G0/G1 by silencing multiple cell cycle genes simultaneously, rather than the individual target
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