Magnetic Field Dependence and Efimov Resonance Broadening in Ultracold Three-Body Recombination

We derive an analytic formula which describes the final bound state dependence in ultracold three-body recombination. Using an energy-dependent loss parameter, the recently observed broad resonance in an ultracold gas of $^{6}$Li atoms [T. B. Ottenstein {\it et al.}, Phys. Rev. Lett. 101, 203202 (2008)l J. H. Huckans {\it et al.}, Phys. Rev. Lett. 102, 165302 (2009)] is described quantitatively. We also provide an analytic and approximation for the three-body recombination rate which encapsulates the underlying physics of the universal three-body recombination process.Comment: 4 pages, 4 figure

Comparison of Absorption, Fluorescence, and Polarization Spectroscopy of Atomic Rubidium

An ongoing spectroscopic investigation of atomic rubidium utilizes a two-photon, single-laser excitation process. Transitions accessible with our tunable laser include 5P1/2 (F ′ ) ← 5S1/2 (F) and 5P3/2 (F ′ ) ← 5S1/2 (F). The laser is split into a pump and probe beam to allow for Doppler-free measurements of transitions between hyperfine levels. The pump and probe beams are overlapped in a counter-propagating geometry and the laser frequency scans over a transition. Absorption, fluorescence and polarization spectroscopy techniques are applied to this basic experimental setup. The temperature of the vapor cell and the power of the pump and probe beams have been varied to explore line broadening effects and signal-to-noise of each technique. This humble setup will hopefully grow into a more robust experimental arrangement in which double resonance, two-laser excitations are used to explore hyperfine state changing collisions between rubidium atoms and noble gas atoms. Rb-noble gas collisions can transfer population between hyperfine levels, such as 5P3/2 (F ′ = 3) Collision ←− 5P3/2 (F ′ = 2), and the probe beam couples 7S1/2 (F ′′ = 2) ← 5P3/2 (F ′ = 3). Polarization spectroscopy signal depends on the rate of population transfer due to the collision as well as maintaining the orientation created by the pump laser. Fluorescence spectroscopy relies only on transfer of population due to the collision. Comparison of these techniques yields information regarding the change of the magnetic sublevels, mF , during hyperfine state changing collisions

Three-body rf association of Efimov trimers

We present a theoretical analysis of rf association of Efimov trimers in a 2-component Bose gas with short-range interactions. Using the adiabatic hyperspherical Green's function formalism to solve the quantum 3-body problem, we obtain universal expressions for 3-body rf association rates as a function of the s-wave scattering length $a$. We find that the association rates scale as $a^{-2}$ in the limit of large $a$, and diverge as $a^3 a_{ad}^{3}$ whenever an Efimov state crosses the atom-dimer threshold (where $a_{ad}$ stands for the atom-dimer scattering length). Our calculations show that trimer formation rates as large as $\sim10^{-21}$ cm$^6$/s can be achieved with rf Rabi frequencies of order 1 MHz, suggesting that direct rf association is a powerful tool of making and probing few-body quantum states in ultracold atomic gases.Comment: 4 pages, 2 figure

Global Analysis of Data on the Spin-orbit-coupled A1Σ+ and b3Πu States of Cs2

We present experimentally derived potential curves and spin-orbit interaction functions for the strongly perturbed A1+ u and b3u states of the cesium dimer. The results are based on data from several sources. Laser-induced fluorescence Fourier transform spectroscopy (LIF FTS) was used some time ago in the Laboratoire Aim´e Cotton primarily to study the X1+ g state. More recent work at Tsinghua University provides information from moderate resolution spectroscopy on the lowest levels of the b3± 0u states as well as additional high resolution data. From Innsbruck University, we have precision data obtained with cold Cs2 molecules. Recent data from Temple University was obtained using the optical-optical double resonance polarization spectroscopy technique, and finally, a group at the University of Latvia has added additional LIF FTS data. In the Hamiltonian matrix, we have used analytic potentials (the Expanded Morse Oscillator form) with both finite-difference (FD) coupled-channels and discrete variable representation (DVR) calculations of the term values. Fitted diagonal and off-diagonal spin-orbit functions are obtained and compared with ab initio results from Temple and Moscow State universities

Ultracold giant polyatomic Rydberg molecules: coherent control of molecular orientation

We predict the existence of a class of ultracold giant molecules formed from trapped ultracold Rydberg atoms and polar molecules. The interaction which leads to the formation of such molecules is the anisotropic charge-dipole interaction ($a/R^2$). We show that prominent candidate molecules such as KRb and deuterated hydroxyl (OD) should bind to Rydberg rubidium atoms, with energies $E_b\simeq 5-25$ GHz at distances $R\simeq 0.1-1 \ \mu$m. These molecules form in double wells, mimicking chiral molecules, with each well containing a particular dipole orientation. We prepare a set of correlated dressed electron-dipole eigenstates which are used in a resonant Raman scheme to coherently control the dipole orientation and to create cat-like entangled states of the polar molecule.Comment: 4 pages, 4 figure