9 research outputs found

    Broken Kramers' degeneracy in altermagnetic MnTe

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    Altermagnetism is a newly identified fundamental class of magnetism with vanishing net magnetization and time-reversal symmetry broken electronic structure. Probing the unusual electronic structure with nonrelativistic spin splitting would be a direct experimental verification of altermagnetic phase. By combining high-quality film growth and in situin~situ angle-resolved photoemission spectroscopy, we report the electronic structure of an altermagnetic candidate, α\alpha-MnTe. Temperature dependent study reveals the lifting of Kramers{\textquoteright} degeneracy accompanied by a magnetic phase transition at TN=267 KT_N=267\text{ K} with spin splitting of up to 370 meV370\text{ meV}, providing direct spectroscopic evidence for altermagnetism in MnTe

    Spontaneous breaking of mirror symmetry beyond critical doping in Pb-Bi2212

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    Identifying ordered phases and their underlying symmetries is the first and most important step toward understanding the mechanism of high-temperature superconductivity; critical behaviors of ordered phases are expected to be correlated with superconductivity. Efforts to find such ordered phases have been focused on symmetry breaking in the pseudogap region while the Fermi liquid-like metal region beyond the so-called critical doping pcp_{c} has been regarded as a trivial disordered state. Here, we used rotational anisotropy second harmonic generation and uncovered a broken mirror symmetry in the Fermi liquid-like phase in (Bi,Pb)2_{2}Sr2_{2}CaCu2_{2}O8+δ_{8+\delta} with p=0.205>pcp = 0.205 > p_{c}. By tracking the temperature evolution of the symmetry-breaking response, we verify an order parameter-like behavior with the onset temperature TupT_{up} at which the strange metal to Fermi liquid-like-metal crossover takes place. Complementary angle-resolved photoemission study showed that the quasiparticle coherence between CuO2\mathrm{CuO_{2}} bilayers is enhanced in proportion to the symmetry-breaking response as a function of temperature, indicating that the change in metallicity and symmetry breaking are linked. These observations contradict the conventional quantum disordered scenario for over-critical-doped cuprates and provide new insight into the nature of the quantum critical point in cuprates.Comment: 8 pages, 4 figure

    Free Space Detection Using Camera-LiDAR Fusion in a Bird’s Eye View Plane

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    Although numerous road segmentation studies have utilized vision data, obtaining robust classification is still challenging due to vision sensor noise and target object deformation. Long-distance images are still problematic because of blur and low resolution, and these features make distinguishing roads from objects difficult. This study utilizes light detection and ranging (LiDAR), which generates information that camera images lack, such as distance, height, and intensity, as a reliable supplement to address this problem. In contrast to conventional approaches, additional domain transformation to a bird’s eye view space is executed to obtain long-range data with resolutions comparable to those of short-range data. This study proposes a convolutional neural network architecture that processes data transformed to a bird’s eye view plane. The network’s pathways are split into two parts to resolve calibration errors in the transformed image and point cloud. The network, which has modules that operate sequentially at various scaled dilated convolution rates, is designed to quickly and accurately handle a wide range of data. Comprehensive empirical studies using the Karlsruhe Institute of Technology and Toyota Technological Institute’s (KITTI’s) road detection benchmarks demonstrate that this study’s approach takes advantage of camera and LiDAR information, achieving robust road detection with short runtimes. Our result ranks 22nd in the KITTI’s leaderboard and shows real-time performance

    Comparative study of upconverting nanoparticles with various crystal structures, core/shell structures, and surface characteristics

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    Upconverting nanoparticles (UCNPs) have been studied as novel bioimaging probes owing to the absence of autofluorescence and excellent photostability. For practical applications, biocompatible UCNPs with high upconversion efficiency, bright luminescence, and good colloidal stability are desirable. Herein, we report a quantitative and systematic study on the upconversion luminescence from a set of NaYF4:Yb3+,Er3+-based nanopartides by varying crystal structures, core/shell structures, and surface ligands. Upconversion luminescent properties in colloidal solution and at the single-particle level were examined. Hexagonal-phase core/shell UCNPs exhibited the most intense luminescence among various structures, while the excellent photostability was observed in all different types of UCNPs. To optimize the biomedical imaging capability of UCNPs, various surface coating strategies were tested. By quantitative spectroscopic measurements of surface-modified UCNPs in water, it was suggested that encapsulation with polyethylene glycol (PEG)-phospholipid was found to be effective in retaining both upconversion luminescence intensity and dispersibility in aqueous environment. Finally, UCNPs with different crystal structures were applied and compared in live cells.

    Comparative Study of Upconverting Nanoparticles with Various Crystal Structures, Core/Shell Structures, and Surface Characteristics

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    Upconverting nanoparticles (UCNPs) have been studied as novel bioimaging probes owing to the absence of autofluorescence and excellent photostability. For practical applications, biocompatible UCNPs with high upconversion efficiency, bright luminescence, and good colloidal stability are desirable. Herein, we report a quantitative and systematic study on the upconversion luminescence from a set of NaYF4:Yb3+,Er3+- based nanoparticles by varying crystal structures, core/shell structures, and surface ligands. Upconversion luminescent properties in colloidal solution and at the single-particle level were examined. Hexagonal-phase core/shell UCNPs exhibited the most intense luminescence among various structures, while the excellent photostability was observed in all different types of UCNPs. To optimize the biomedical imaging capability of UCNPs, various surface coating strategies were tested. By quantitative spectroscopic measurements of surface-modified UCNPs in water, it was suggested that encapsulation with polyethylene glycol (PEG)-phospholipid was found to be effective in retaining both upconversion luminescence intensity and dispersibility in aqueous environment. Finally, UCNPs with different crystal structures were applied and compared in live cells.130321sciescopu

    Strain-controlled evolution of electronic structure indicating topological phase transition in the quasi-one-dimensional superconductor TaSe3

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    © 2022 American Physical Society.We report the signature of a strain-controlled topological phase transition in the electronic structure of a quasi-one-dimensional superconductor TaSe3. Using angle-resolved photoemission spectroscopy and first-principles calculation, TaSe3 is identified to be in a weak topological insulator phase which has topologically nontrivial surface states only at the allowed planes. Under uniaxial tensile strain, a Dirac point and the topological surface state emerge on the originally forbidden (101¯) plane, which demonstrates the transition to a strong topological insulator phase. Our results accomplish the experimental realization of possible topological insulating phases in TaSe3 and highlight the possibility of coupling the superconductivity with two distinct topological insulating phases in a controllable manner.11Nsciescopu

    Theranostic Probe Based on Lanthanide-Doped Nanoparticles for Simultaneous In Vivo Dual-Modal Imaging and Photodynamic Therapy

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    Dual-modal in vivo tumor imaging and photodynamic therapy using hexagonal NaYF4:Yb,Er/NaGdF4 core-shell upconverting nanoparticles combined with a photosensitizer, chlorin e6, is reported. Tumors can be clearly observed not only in the upconversion luminescence image but also in the magnetic resonance image. In vivo photodynamic therapy by systemic administration is demonstrated under 980 nm irradiation.

    Comparative Study of Upconverting Nanoparticles with Various Crystal Structures, Core/Shell Structures, and Surface Characteristics

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    Upconverting nanoparticles (UCNPs) have been studied as novel bioimaging probes owing to the absence of autofluorescence and excellent photostability. For practical applications, biocompatible UCNPs with high upconversion efficiency, bright luminescence, and good colloidal stability are desirable. Herein, we report a quantitative and systematic study on the upconversion luminescence from a set of NaYF<sub>4</sub>:Yb<sup>3+</sup>,Er<sup>3+</sup>-based nanoparticles by varying crystal structures, core/shell structures, and surface ligands. Upconversion luminescent properties in colloidal solution and at the single-particle level were examined. Hexagonal-phase core/shell UCNPs exhibited the most intense luminescence among various structures, while the excellent photostability was observed in all different types of UCNPs. To optimize the biomedical imaging capability of UCNPs, various surface coating strategies were tested. By quantitative spectroscopic measurements of surface-modified UCNPs in water, it was suggested that encapsulation with polyethylene glycol (PEG)-phospholipid was found to be effective in retaining both upconversion luminescence intensity and dispersibility in aqueous environment. Finally, UCNPs with different crystal structures were applied and compared in live cells

    Comparative Study of Upconverting Nanoparticles with Various Crystal Structures, Core/Shell Structures, and Surface Characteristics

    Full text link
    Upconverting nanoparticles (UCNPs) have been studied as novel bioimaging probes owing to the absence of autofluorescence and excellent photostability. For practical applications, biocompatible UCNPs with high upconversion efficiency, bright luminescence, and good colloidal stability are desirable. Herein, we report a quantitative and systematic study on the upconversion luminescence from a set of NaYF4:Yb3+,Er3+-based nanopartides by varying crystal structures, core/shell structures, and surface ligands. Upconversion luminescent properties in colloidal solution and at the single-particle level were examined. Hexagonal-phase core/shell UCNPs exhibited the most intense luminescence among various structures, while the excellent photostability was observed in all different types of UCNPs. To optimize the biomedical imaging capability of UCNPs, various surface coating strategies were tested. By quantitative spectroscopic measurements of surface-modified UCNPs in water, it was suggested that encapsulation with polyethylene glycol (PEG)-phospholipid was found to be effective in retaining both upconversion luminescence intensity and dispersibility in aqueous environment. Finally, UCNPs with different crystal structures were applied and compared in live cells.N
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