549 research outputs found
Doping evolution of the electronic specific heat coefficient in slightly-doped La2-xSrxCuO4 single crystals
Detailed doping dependence of the electronic specific heat coefficient gamma
is studied for La2-xSrxCuO4 (LSCO) single crystals in the slightly-doped
regime. We find that gamma systematically increases with doping, and
furthermore, even for the samples in the antiferromagnetic (AF) regime, gamma
already acquires finite value and grows with x. This suggests that finite
electronic density of states (DOS) is created in the AF regime where the
transport shows strong localization at low temperatures, and this means the
system is not a real insulator with a clear gap even though it still keeps long
range AF order.Comment: 4 pages, 4 figures, accepted for publication in Journal of Physics:
Conference Series (LT25 proceeding
Thermal Conductivity of Pr_{1.3-x}La_{0.7}Ce_xCuO_4 Single Crystals and Signatures of Stripes in an Electron-Doped Cuprate
It was recently demonstrated that the anisotropic phonon heat transport
behavior is a good probe of the stripe formation in La_{2-x}Sr_xCuO_4 (LSCO)
[X. F. Sun {\it et al.}, Phys. Rev. B {\bf 67}, 104503 (2003)]. Using this
probe, we examined an electron-doped cuprate Pr_{1.3-x}La_{0.7}Ce_xCuO_4
(PLCCO) and found that essentially the same features as those in LSCO are
observed. Moreover, the in-plane resistivity \rho_{ab} of lightly-doped PLCCO
shows metallic behavior (d\rho_{ab}/dT > 0) in the N\'eel ordered state with a
mobility comparable to that in LSCO. It is discussed that these peculiar
properties in common with LSCO signify the existence of stripes in
electron-doped cuprates.Comment: 4 pages, 4 figures, revised version accepted for publication in Phys.
Rev. Let
Doping dependence of charge-transfer excitations in La_{2-x}Sr_xCuO_4
We report a resonant inelastic x-ray scattering (RIXS) study of the doping
dependence of charge-transfer excitations in . The mome
ntum dependence of these charge excitations are studied over the whole
Brillouin zone in underdoped (x=0.05) and optimally doped (x=0.17) samples, and
compared with that of the undoped (x=0) sample. We observe a large change in
the RIXS spectra between the x=0 and x=0.17 sample, while the RIXS spectra of
the x=0.05 sample are similar to that of the x=0 sample. The most prominent
effect of doped-holes on the charge excitation spectra is the appearance of a
continuum of intensity, which exhibits a strong momentum-dependence below 2 eV.
For the x=0.17 sample, some of the spectral weight from the lowest-lying
charge-transfer excitation of the undoped compound is transferred to the
continuum intensity below the gap, in agreement with earlier optical studies.
However, the higher energy charge-transfer excitation carries significant
spectral weight even for the x=0.17 sample. The doping dependence of the
dispersion of this charge-transfer excitation is also discussed and compared
with recent theoretical calculations.Comment: 7 pages, 6 figures, to appear in Phys. Rev.
Large magneto-thermal effect and the spin-phonon coupling in a parent insulating cuprate Pr_{1.3}La_{0.7}CuO_4
The magnetic-field (H) dependence of the thermal conductivity \kappa of
Pr_{1.3}La_{0.7}CuO_4 is found to show a pronounced minimum for in-plane fields
at low temperature, which is best attributed to the scattering of phonons by
free spins that are seen by a Schottky-type specific heat and a Curie-Weiss
susceptibility. Besides pointing to a strong spin-phonon coupling in cuprates,
the present result demonstrates that the H-dependence of the phonon heat
transport should not be naively neglected when discussing the \kappa(H)
behavior of cuprates, since the Schottky anomaly is ubiquitously found in
cuprates at any doping.Comment: 6 pages, 4 figures, accepted for publication in Phys. Rev.
"Spin-Flop" Transition and Anisotropic Magnetoresistance in Pr_{1.3-x}La_{0.7}Ce_{x}CuO_{4}: Unexpectedly Strong Spin-Charge Coupling in Electron-Doped Cuprates
We use transport and neutron-scattering measurements to show that a
magnetic-field-induced transition from noncollinear to collinear spin
arrangement in adjacent CuO_{2} planes of lightly electron-doped
Pr_{1.3-x}La_{0.7}Ce_{x}CuO_{4} (x=0.01) crystals affects significantly both
the in-plane and out-of-plane resistivity. In the high-field collinear state,
the magnetoresistance (MR) does not saturate, but exhibits an intriguing
four-fold-symmetric angular dependence, oscillating from being positive at
B//[100] to being negative at B//[110]. The observed MR of more than 30% at low
temperatures induced by a modest modification of the spin structure indicates
an unexpectedly strong spin-charge coupling in electron-doped cuprates.Comment: 4 pages, 5 figures, accepted for publication in Phys. Rev. Let
Microscopic analysis of the chemical reaction between Fe(Te,Se) thin films and underlying CaF
To understand the chemical reaction at the interface of materials, we
performed a transmission electron microscopy (TEM) observation in four types of
Fe(Te,Se) superconducting thin films prepared on different types of substrates:
CaF2 substrate, CaF2 substrate with a CaF2 buffer layer, CaF2 substrate with a
FeSe buffer layer, and a LaAlO3 substrate with a CaF2 buffer layer. Based on
the energy-dispersive X-ray spectrometer (EDX) analysis, we found possible
interdiffusion between fluorine and selenium that has a strong influence on the
superconductivity in Fe(Te,Se) films. The chemical interdiffusion also plays a
significant role in the variation of the lattice parameters. The lattice
parameters of the Fe(Te,Se) thin films are primarily determined by the chemical
substitution of anions, and the lattice mismatch only plays a secondary role.Comment: 30 pages, 9 figur
Electronic inhomogeneity and competing phases in electron-doped superconducting Pr0.88LaCe0.12CuO4
We use neutron scattering to demonstrate that electron-doped superconducting
Pr0.88LaCe0.12CuO4 in the underdoped regime is electronically phase separated
in the ground state, showing the coexistence of a superconducting phase with a
three-dimensional antiferromagnetically ordered phase and a
quasi-two-dimensional spin density wave modulation. The Neel temperature of
both antiferromagnetic phases decreases linearly with increasing
superconducting transition temperature (Tc) and vanishes when optimal
superconductivity is achieved. These results indicate that the electron-doped
copper oxides are close to a quantum critical point, where the delicate
energetic balance between different competing states leads to microscopic
heterogeneity.Comment: 14 pages, 4 figures, accepted to Phys. Rev. B as a rapid
communicatio
Zn-impurity effects on quasi-particle scattering in La2-xSrxCuO4 studied by angle-resolved photoemission spectroscopy
Angle-resolved photoemission measurements were performed on Zn-doped
La2-xSrxCuO4 (LSCO) to investigate the effects of Zn impurities on the low
energy electronic structure. The Zn-impurity-induced increase in the
quasi-particle (QP) width in momentum distribution curves (MDC) is
approximately isotropic on the entire Fermi surface and energy-independent near
the Fermi level (EF). The increase in the MDC width is consistent with the
increase in the residual resistivity due to the Zn impurities if we assume the
carrier number to be 1-x for x=0.17 and the Zn impurity to be a potential
scatterer close to the unitarity limit. For x=0.03, the residual resistivity is
found to be higher than that expected from the MDC width, and the effects of
antifferomagnetic fluctuations induced around the Zn impurities are discussed.
The leading edges of the spectra near (pi,0) for x=0.17 are shifted toward
higher energies relative to EF with Zn substitution, indicating a reduction of
the superconducting gap.Comment: 7 pages, 7 figure
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