All-optical measurement of the hot electron sheath driving laser ion acceleration from thin foils

We present experimental results from an all-optical diagnostic method to directly measure the evolution of the hot-electron distribution driving the acceleration of ions from thin foils using high-intensity lasers. Central parameters of laser ion acceleration such as the hot-electron density, the temperature distribution and the conversion efficiency from laser pulse energy into hot electrons become comprehensively accessible with this technique.Deutsche Forschungsgemeinschaft (DFG) (contract number TR18)Germany. Bundesministerium für Bildung und Forschung (contract number 03ZIK445)Germany. Bundesministerium für Bildung und Forschung (contract number 03ZIK052

Measurement of Magnetic-Field Structures in a Laser-Wakefield Accelerator

Experimental measurements of magnetic fields generated in the cavity of a self-injecting laser-wakefield accelerator are presented. Faraday rotation is used to determine the existence of multi-megagauss fields, constrained to a transverse dimension comparable to the plasma wavelength and several plasma wavelengths longitudinally. The fields are generated rapidly and move with the driving laser. In our experiment, the appearance of the magnetic fields is correlated to the production of relativistic electrons, indicating that they are inherently tied to the growth and wavebreaking of the nonlinear plasma wave. This evolution is confirmed by numerical simulations, showing that these measurements provide insight into the wakefield evolution with high spatial and temporal resolution

Peptide Mass Spectra from Micrometer-Thick Ice Films Produced with Femtosecond Pulses

We present a cryogenic mass spectrometry protocol with the capability to detect peptides in the attomole dilution range from ice films. Our approach employs femtosecond laser pulses and implements neither substrate modification nor proton donor agents in the aqueous solution, known to facilitate analyte detection in mass spectrometry. In a systematic study, we investigated the impact of temperature, substrate composition, and irradiation wavelength (513 and 1026 nm) on the bradykinin signal onset. Our findings show that substrate choice and irradiation wavelength have a minor impact on signal intensity once the preparation protocol is optimized. However, if the temperature is increased from −140 to 0 °C, which is accompanied by ice film thinning, a somehow complex picture of analyte desorption and ionization is recognizable, which has not been described in the literature yet. Under cryogenic conditions (−140 °C), obtaining a signal is only possible from isolated sweet spots across the film. If the thin ice film is between −100 and −70 °C of temperature, these sweet spots appear more frequently. Ice sublimation triggered by temperatures above −70 °C leads to an intense and robust signal onset that could be maintained for several hours. In addition to the above findings, we notice that a vibrant fragmentation pattern produced is strikingly similar with both wavelengths. Our findings suggest that while following an optimized protocol, femtosecond mass spectrometry has excellent potential to analyze small organic molecules and peptides with a mass range of up to 2.5 kDa in aqueous solution without any matrix, as employed in matrix-assisted laser desorption/ionization (MALDI) or any substrate surface modification, found in surface-assisted laser desorption/ionization (SALDI)

The reflectivity of relativistic ultra-thin electron layers

The coherent reflectivity of a dense, relativistic, ultra-thin electron layer is derived analytically for an obliquely incident probe beam. Results are obtained by two-fold Lorentz transformation. For the analytical treatment, a plane uniform electron layer is considered. All electrons move with uniform velocity under an angle to the normal direction of the plane; such electron motion corresponds to laser acceleration by direct action of the laser fields, as it is described in a companion paper. Electron density is chosen high enough to ensure that many electrons reside in a volume \lambda_R^3, where \lambda_R is the wavelength of the reflected light in the rest frame of the layer. Under these conditions, the probe light is back-scattered coherently and is directed close to the layer normal rather than the direction of electron velocity. An important consequence is that the Doppler shift is governed by \gamma_x=(1-(V_x/c)^2)^{-1/2} derived from the electron velocity component V_x in normal direction rather than the full \gamma-factor of the layer electrons.Comment: 7 pages, 4 figures, submitted to the special issue "Fundamental Physics with Ultra-High Fields" in The European Physical Journal

Intense high-quality medical proton beams via laser fields

During the past decade, the interaction of high-intensity lasers with solid targets has attracted much interest, regarding its potential in accelerating charged particles. In spite of tremendous progress in laser-plasma based acceleration, it is still not clear which particle beam quality will be accessible within the upcoming multi petawatt (1 PW = 10$^{15}$ W) laser generation. Here, we show with simulations based on the coupled relativistic equations of motion that protons stemming from laser-plasma processes can be efficiently post-accelerated using crossed laser beams focused to spot radii of a few laser wavelengths. We demonstrate that the crossed beams produce monoenergetic accelerated protons with kinetic energies $> 200$ MeV, small energy spreads ($\approx$ 1$$) and high densities as required for hadron cancer therapy. To our knowledge, this is the first scheme allowing for this important application based on an all-optical set-up.Comment: 14 pages, 3 figures, 1 tabl

Nuclear dynamics of singlet exciton fission: a direct observation in pentacene single crystals

Singlet exciton fission (SEF) is a key process in the development of efficient opto-electronic devices. An aspect that is rarely probed directly, and yet has a tremendous impact on SEF properties, is the nuclear structure and dynamics involved in this process. Here we directly observe the nuclear dynamics accompanying the SEF process in single crystal pentacene using femtosecond electron diffraction. The data reveal coherent atomic motions at 1 THz, incoherent motions, and an anisotropic lattice distortion representing the polaronic character of the triplet excitons. Combining molecular dynamics simulations, time-dependent density functional theory and experimental structure factor analysis, the coherent motions are identified as collective sliding motions of the pentacene molecules along their long axis. Such motions modify the excitonic coupling between adjacent molecules. Our findings reveal that long-range motions play a decisive part in the disintegration of the electronically correlated triplet pairs, and shed light on why SEF occurs on ultrafast timescales

Particle physics with a laser-driven positronium atom

A detailed quantum-electrodynamic calculation of muon pair creation in laser-driven electron-positron collisions is presented. The colliding particles stem from a positronium atom exposed to a superintense laser wave of linear polarization, which allows for high luminosity. The threshold laser intensity of this high-energy reaction amounts to a few 10^22 W/cm^2 in the near-infrared frequency range. The muons produced form an ultrarelativistic, strongly collimated beam, which is explicable in terms of a classical simple-man's model. Our results indicate that the process can be observed at high positronium densities with the help of present-day laser technology.Comment: 4 pages, 3 figure

Spectral shaping of laser generated proton beams

The rapid progress in the field of laser particle acceleration has stimulated a debate about the promising perspectives of laser based ion beam sources. For a long time, the beams produced exhibited quasi-thermal spectra. Recent proof-of-principle experiments demonstrated that ion beams with narrow energy distribution can be generated from special target geometries. However, the achieved spectra were strongly limited in terms of monochromacity and reproducibility. We show that microstructured targets can be used to reliably produce protons with monoenergetic spectra above 2 MeV with less than 10% energy spread. Detailed investigations of the effects of laser ablation on the target resulted in a significant improvement of the reproducibility. Based on statistical analysis, we derive a scaling law between proton peak position and laser energy, underlining the suitability of this method for future applications. Both the quality of the spectra and the scaling law are well reproduced by numerical simulations

Nuclear Inelastic X-Ray Scattering of FeO to 48 GPa

The partial density of vibrational states has been measured for Fe in compressed FeO (w\"ustite) using nuclear resonant inelastic x-ray scattering. Substantial changes have been observed in the overall shape of the density of states close to the magnetic transiton around 20 GPa from the paramagnetic (low pressure) to the antiferromagnetic (high pressure) state. Our data indicate a substantial softening of the aggregate sound velocities far below the transition, starting between 5 and 10 GPa. This is consistent with recent radial x-ray diffraction measurements of the elastic constants in FeO. The results indicate that strong magnetoelastic coupling in FeO is the driving force behind the changes in the phonon spectrum of FeO.Comment: 4 pages, 4 figure

Lattice dynamics and correlated atomic motion from the atomic pair distribution function

The mean-square relative displacements (MSRD) of atomic pair motions in crystals are studied as a function of pair distance and temperature using the atomic pair distribution function (PDF). The effects of the lattice vibrations on the PDF peak widths are modelled using both a multi-parameter Born von-Karman (BvK) force model and a single-parameter Debye model. These results are compared to experimentally determined PDFs. We find that the near-neighbor atomic motions are strongly correlated, and that the extent of this correlation depends both on the interatomic interactions and crystal structure. These results suggest that proper account of the lattice vibrational effects on the PDF peak width is important in extracting information on static disorder in a disordered system such as an alloy. Good agreement is obtained between the BvK model calculations of PDF peak widths and the experimentally determined peak widths. The Debye model successfully explains the average, though not detailed, natures of the MSRD of atomic pair motion with just one parameter. Also the temperature dependence of the Debye model largely agrees with the BvK model predictions. Therefore, the Debye model provides a simple description of the effects of lattice vibrations on the PDF peak widths.Comment: 9 pages, 11 figure