86 research outputs found

    Energy levels and lifetimes of Nd IV, Pm IV, Sm IV, and Eu IV

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    To address the shortage of experimental data for electron spectra of triply-ionized rare earth elements we have calculated energy levels and lifetimes of 4f{n+1} and 4f{n}5d configurations of Nd IV (n=2), Pm IV (n=3), Sm IV (n=4), and Eu IV (n=5) using Hartree-Fock and configuration interaction methods. To control the accuracy of our calculations we also performed similar calculations for Pr III, Nd III and Sm III, for which experimental data are available. The results are important, in particular, for physics of magnetic garnets.Comment: 4 pages 1 tabl

    Off-Diagonal Hyperfine Interaction and Parity Non-conservation in Cesium

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    We have performed relativistic many-body calculations of the hyperfine interaction in the 6s6s and 7s7s states of Cs, including the off-diagonal matrix element. The calculations were used to determine the accuracy of the semi-empirical formula for the electromagnetic transition amplitude induced by the hyperfine interaction. We have found that even though the contribution of the many-body effects into the matrix elements is very large, the square root formula = = \sqrt{ } remains valid to the accuracy of a fraction of 10−310^{-3}. The result for the M1-amplitude is used in the interpretation of the parity-violation measurement in the 6s−7s6s-7s transition in Cs which claims a possible deviation from the Standard model.Comment: 13 pages, 4 figures, LaTeX, Submitted to Phys. Rev.

    Measurement of the 6s - 7p transition probabilities in atomic cesium and a revised value for the weak charge Q_W

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    We have measured the 6s - 7p_{1/2,3/2} transition probabilities in atomic cesium using a direct absorption technique. We use our result plus other previously measured transition rates to derive an accurate value of the vector transition polarizability \beta and, consequently, re-evaluate the weak charge Q_W. Our derived value Q_W=-72.65(49) agrees with the prediction of the standard model to within one standard deviation.Comment: 4 pages, 2 figure

    Calculations of parity nonconserving s-d transitions in Cs, Fr, Ba II, and Ra II

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    We have performed ab initio mixed-states and sum-over-states calculations of parity nonconserving (PNC) electric dipole (E1) transition amplitudes between s-d electron states of Cs, Fr, Ba II, and Ra II. For the lower states of these atoms we have also calculated energies, E1 transition amplitudes, and lifetimes. We have shown that PNC E1 transition amplitudes between s-d states can be calculated to high accuracy. Contrary to the Cs 6s-7s transition, in these transitions there are no strong cancelations between different terms in the sum-over-states approach. In fact, there is one dominating term which deviates from the sum by less than 20%. This term corresponds to an s-p_{1/2} weak matrix element, which can be calculated to better than 1%, and a p_{1/2}-d_{3/2} E1 transition amplitude, which can be measured. Also, the s-d amplitudes are about four times larger than the corresponding s-s transitions. We have shown that by using a hybrid mixed-states/sum-over-states approach the accuracy of the calculations of PNC s-d amplitudes could compete with that of Cs 6s-7s if p_{1/2}-d_{3/2} E1 amplitudes are measured to high accuracy.Comment: 15 pages, 8 figures, submitted to Phys. Rev.

    Calculation of parity and time invariance violation in the radium atom

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    Parity (P) and time (T) invariance violating effects in the Ra atom are strongly enhanced due to close states of opposite parity, the large nuclear charge Z and the collective nature of P,T-odd nuclear moments. We have performed calculations of the atomic electric dipole moments (EDM) produced by the electron EDM and the nuclear magnetic quadrupole and Schiff moments. We have also calculated the effects of parity non-conservation produced by the nuclear anapole moment and the weak charge. Our results show that as a rule the values of these effects are much larger than those considered so far in other atoms (enhancement is up to 10^5 times).Comment: 18 pages; LaTeX; Submitted to Phys. Rev.

    Light-induced structural changes in photosynthetic reaction centres studied by ESEEM of spin-correlated D+QA− radical pairs

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    AbstractZn-substituted Rhodobacter sphaeroides R26 reaction centres (RCs) frozen in the dark and under illumination exhibit quite different recombination kinetics of the D+QA− radical pairs [Kleinfeld et al., Biochemistry, 23 (1984) 5780]. We have applied electron spin echo envelope modulation (ESEEM) of the spin-correlated D+QA− radical pairs to assess a possible light-induced change in the distance between the D and QA cofactors. The recombination kinetics and the field-swept spin-polarized EPR signal for the two preparations have been monitored by time-resolved EPR spectroscopy. For the samples frozen under illumination, a slight increase in the distance, 0.4±0.2 Å, has been detected

    Parity nonconservation in heavy atoms: The radiative correction enhanced by the strong electric field of the nucleus

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    Parity nonconservation due to the nuclear weak charge is considered. We demonstrate that the radiative corrections to this effect due to the vacuum fluctuations of the characteristic size larger than the nuclear radius r0r_0 and smaller than the electron Compton wave-length λC\lambda_C are enhanced because of the strong electric field of the nucleus. The parameter that allows one to classify the corrections is the large logarithm ln⁥(λC/r0)\ln(\lambda_C/r_0). The vacuum polarization contribution is enhanced by the second power of the logarithm. Although the self-energy and the vertex corrections do not vanish, they contain only the first power of the logarithm. The value of the radiative correction is 0.4% for Cs and 0.9% for Tl, Pb, and Bi. We discuss also how the correction affects the interpretation of the experimental data on parity nonconservation in atoms.Comment: 4 pages, 3 figures, RevTe

    Precise calculation of parity nonconservation in cesium and test of the standard model

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    We have calculated the 6s-7s parity nonconserving (PNC) E1 transition amplitude, E_{PNC}, in cesium. We have used an improved all-order technique in the calculation of the correlations and have included all significant contributions to E_{PNC}. Our final value E_{PNC} = 0.904 (1 +/- 0.5 %) \times 10^{-11}iea_{B}(-Q_{W}/N) has half the uncertainty claimed in old calculations used for the interpretation of Cs PNC experiments. The resulting nuclear weak charge Q_{W} for Cs deviates by about 2 standard deviations from the value predicted by the standard model.Comment: 24 pages, 8 figure

    E1 amplitudes, lifetimes, and polarizabilities of the low-lying levels of atomic ytterbium

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    The results of ab initio calculation of E1 amplitudes, lifetimes,and polarizabilities for several low-lying levels of ytterbium are reported. The effective Hamiltonian for the valence electrons has been constructed in the frame of CI+MBPT method and solutions of many electron equation are found.Comment: 11 pages, submitted to Phys.Rev.

    Isotope shift calculations for atoms with one valence electron

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    This work presents a method for the ab initio calculation of isotope shift in atoms and ions with one valence electron above closed shells. As a zero approximation we use relativistic Hartree-Fock and then calculate correlation corrections. The main motivation for developing the method comes from the need to analyse whether different isotope abundances in early universe can contribute to the observed anomalies in quasar absorption spectra. The current best explanation for these anomalies is the assumption that the fine structure constant, alpha, was smaller at early epoch. We test the isotope shift method by comparing the calculated and experimental isotope shift for the alkali and alkali-like atoms Na, MgII, K, CaII and BaII. The agreement is found to be good. We then calculate the isotope shift for some astronomically relevant transitions in SiII and SiIV, MgII, ZnII and GeII.Comment: 11 page
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