14,921 research outputs found
Signatures of Electronic Correlations in Optical Properties of LaFeAsOF
Spectroscopic ellipsometry is used to determine the dielectric function of
the superconducting LaFeAsOF ( = 27 K) and undoped LaFeAsO
polycrystalline samples in the wide range 0.01-6.5 eV at temperatures 10 350 K. The free charge carrier response in both samples is heavily
damped with the effective carrier density as low as 0.0400.005 electrons
per unit cell. The spectral weight transfer in the undoped LaFeAsO associated
with opening of the pseudogap at about 0.65 eV is restricted at energies below
2 eV. The spectra of superconducting LaFeAsOF reveal a
significant transfer of the spectral weight to a broad optical band above 4 eV
with increasing temperature. Our data may imply that the electronic states near
the Fermi surface are strongly renormalized due to electron-phonon and/or
electron-electron interactions.Comment: 4 pages, 4 figures, units in Fig.2 adde
Dielectric constants of Ir, Ru, Pt, and IrO2: Contributions from bound charges
We investigated the dielectric functions () of Ir, Ru, Pt,
and IrO, which are commonly used as electrodes in ferroelectric thin film
applications. In particular, we investigated the contributions from bound
charges (), since these are important scientifically as
well as technologically: the (0) of a metal electrode is one of
the major factors determining the depolarization field inside a ferroelectric
capacitor. To obtain (0), we measured reflectivity spectra of
sputtered Pt, Ir, Ru, and IrO2 films in a wide photon energy range between 3.7
meV and 20 eV. We used a Kramers-Kronig transformation to obtain real and
imaginary dielectric functions, and then used Drude-Lorentz oscillator fittings
to extract (0) values. Ir, Ru, Pt, and IrO produced
experimental (0) values of 4810, 8210, 5810, and
295, respectively, which are in good agreement with values obtained using
first-principles calculations. These values are much higher than those for
noble metals such as Cu, Ag, and Au because transition metals and IrO have
such strong d-d transitions below 2.0 eV. High (0) values will
reduce the depolarization field in ferroelectric capacitors, making these
materials good candidates for use as electrodes in ferroelectric applications.Comment: 26 pages, 6 figures, 2 table
Towards an Optimal Reconstruction of Baryon Oscillations
The Baryon Acoustic Oscillations (BAO) in the large-scale structure of the
universe leave a distinct peak in the two-point correlation function of the
matter distribution. That acoustic peak is smeared and shifted by bulk flows
and non-linear evolution. However, it has been shown that it is still possible
to sharpen the peak and remove its shift by undoing the effects of the bulk
flows. We propose an improvement to the standard acoustic peak reconstruction.
Contrary to the standard approach, the new scheme has no free parameters,
treats the large-scale modes consistently, and uses optimal filters to extract
the BAO information. At redshift of zero, the reconstructed linear matter power
spectrum leads to a markedly improved sharpening of the reconstructed acoustic
peak compared to standard reconstruction.Comment: 20 pages, 5 figures; footnote adde
First-Principles Study of Electronic Structure in -(BEDT-TTF)I at Ambient Pressure and with Uniaxial Strain
Within the framework of the density functional theory, we calculate the
electronic structure of -(BEDT-TTF)I at 8K and room temperature
at ambient pressure and with uniaxial strain along the - and -axes. We
confirm the existence of anisotropic Dirac cone dispersion near the chemical
potential. We also extract the orthogonal tight-binding parameters to analyze
physical properties. An investigation of the electronic structure near the
chemical potential clarifies that effects of uniaxial strain along the a-axis
is different from that along the b-axis. The carrier densities show
dependence at low temperatures, which may explain the experimental findings not
only qualitatively but also quantitatively.Comment: 10 pages, 7 figure
Optical Study of the Free Carrier Response of LaTiO3/SrTiO3 Superlattices
We used infrared spectroscopic ellipsometry to investigate the electronic
properties of LaTiO3/SrTiO3 superlattices (SLs). Our results indicated that,
independent of the SL periodicity and individual layer-thickness, the SLs
exhibited a Drude metallic response with sheet carrier density per interface
~3x10^14 cm^-2. This is probably due to the leakage of d-electrons at
interfaces from the Mott insulator LaTiO3 to the band insulator SrTiO3. We
observed a carrier relaxation time ~ 35 fs and mobility ~ 35 cm^2V^-1s^-1 at 10
K, and an unusual temperature dependence of carrier density that was attributed
to the dielectric screening of quantum paraelectric SrTiO3.Comment: 4 pages, 4 figure
Electronic properties of correlated metals in the vicinity of a charge order transition: optical spectroscopy of -(BEDT-TTF)Hg(SCN) ( = NH, Rb, Tl)
The infrared spectra of the quasi-two-dimensional organic conductors
-(BEDT-TTF)Hg(SCN) ( = NH, Rb, Tl) were measured in
the range from 50 to 7000 \cm down to low temperatures in order to explore the
influence of electronic correlations in quarter-filled metals. The
interpretation of electronic spectra was confirmed by measurements of pressure
dependant reflectance of -(BEDT-TTF)KHg(SCN) at T=300 K. The
signatures of charge order fluctuations become more pronounced when going from
the NH salt to Rb and further to Tl compounds. On reducing the temperature,
the metallic character of the optical response in the NH and Rb salts
increases, and the effective mass diminishes. For the Tl compound, clear
signatures of charge order are found albeit the metallic properties still
dominate. From the temperature dependence of the electronic scattering rate the
crossover temperature is estimated below which the coherent charge-carriers
response sets in. The observations are in excellent agreement with recent
theoretical predictions for a quarter-filled metallic system close to charge
order
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