20 research outputs found
Diffusion and Creep of a Particle in a Random Potential
We investigate the diffusive motion of an overdamped classical particle in a
1D random potential using the mean first-passage time formalism and demonstrate
the efficiency of this method in the investigation of the large-time dynamics
of the particle. We determine the -time diffusion {<{<
x^{2}(t)>}_{th}>}_{dis}=A\ln^{\beta} \left ({t}/{t_{r}}) and relate the
prefactor the relaxation time and the exponent to the
details of the (generally non-gaussian) long-range correlated potential.
Calculating the moments {}_{th}>}_{dis} of the first-passage time
distribution we reconstruct the large time distribution function itself
and draw attention to the phenomenon of intermittency. The results can be
easily interpreted in terms of the decay of metastable trapped states. In
addition, we present a simple derivation of the mean velocity of a particle
moving in a random potential in the presence of a constant external force.Comment: 6 page
Analysis of self--averaging properties in the transport of particles through random media
We investigate self-averaging properties in the transport of particles
through random media. We show rigorously that in the subdiffusive anomalous
regime transport coefficients are not self--averaging quantities. These
quantities are exactly calculated in the case of directed random walks. In the
case of general symmetric random walks a perturbative analysis around the
Effective Medium Approximation (EMA) is performed.Comment: 4 pages, RevTeX , No figures, submitted to Physical Review E (Rapid
Communication
Particle displacements in the elastic deformation of amorphous materials: local fluctuations vs. non-affine field
We study the local disorder in the deformation of amorphous materials by
decomposing the particle displacements into a continuous, inhomogeneous field
and the corresponding fluctuations. We compare these fields to the commonly
used non-affine displacements in an elastically deformed 2D Lennard-Jones
glass. Unlike the non-affine field, the fluctuations are very localized, and
exhibit a much smaller (and system size independent) correlation length, on the
order of a particle diameter, supporting the applicability of the notion of
local "defects" to such materials. We propose a scalar "noise" field to
characterize the fluctuations, as an additional field for extended continuum
models, e.g., to describe the localized irreversible events observed during
plastic deformation.Comment: Minor corrections to match the published versio
A note on the violation of the Einstein relation in a driven moderately dense granular gas
The Einstein relation for a driven moderately dense granular gas in
-dimensions is analyzed in the context of the Enskog kinetic equation. The
Enskog equation neglects velocity correlations but retains spatial correlations
arising from volume exclusion effects. As expected, there is a breakdown of the
Einstein relation relating diffusion and
mobility , being the temperature of the impurity. The kinetic theory
results also show that the violation of the Einstein relation is only due to
the strong non-Maxwellian behavior of the reference state of the impurity
particles. The deviation of from unity becomes more significant as
the solid volume fraction and the inelasticity increase, especially when the
system is driven by the action of a Gaussian thermostat. This conclusion
qualitatively agrees with some recent simulations of dense gases [Puglisi {\em
et al.}, 2007 {\em J. Stat. Mech.} P08016], although the deviations observed in
computer simulations are more important than those obtained here from the
Enskog kinetic theory. Possible reasons for the quantitative discrepancies
between theory and simulations are discussed.Comment: 6 figure
Disorder and Funneling Effects on Exciton Migration in Tree-Like Dendrimers
The center-bound excitonic diffusion on dendrimers subjected to several types
of non-homogeneous funneling potentials, is considered. We first study the
mean-first passage time (MFPT) for diffusion in a linear potential with
different types of correlated and uncorrelated random perturbations. Increasing
the funneling force, there is a transition from a phase in which the MFPT grows
exponentially with the number of generations , to one in which it does so
linearly. Overall the disorder slows down the diffusion, but the effect is much
more pronounced in the exponential compared to the linear phase. When the
disorder gives rise to uncorrelated random forces there is, in addition, a
transition as the temperature is lowered. This is a transition from a
high- regime in which all paths contribute to the MFPT to a low- regime
in which only a few of them do. We further explore the funneling within a
realistic non-linear potential for extended dendrimers in which the dependence
of the lowest excitonic energy level on the segment length was derived using
the Time-Dependent Hatree-Fock approximation. Under this potential the MFPT
grows initially linearly with but crosses-over, beyond a molecular-specific
and -dependent optimal size, to an exponential increase. Finally we consider
geometrical disorder in the form of a small concentration of long connections
as in the {\it small world} model. Beyond a critical concentration of
connections the MFPT decreases significantly and it changes to a power-law or
to a logarithmic scaling with , depending on the strength of the funneling
force.Comment: 13 pages, 9 figure
Multifractals of Normalized First Passage Time in Sierpinski Gasket
The multifractal behavior of the normalized first passage time is
investigated on the two dimensional Sierpinski gasket with both absorbing and
reflecting barriers. The normalized first passage time for Sinai model and the
logistic model to arrive at the absorbing barrier after starting from an
arbitrary site, especially obtained by the calculation via the Monte Carlo
simulation, is discussed numerically. The generalized dimension and the
spectrum are also estimated from the distribution of the normalized first
passage time, and compared with the results on the finitely square lattice.Comment: 10 pages, Latex, with 3 figures and 1 table. to be published in J.
Phys. Soc. Jpn. Vol.67(1998
Excitonic Funneling in Extended Dendrimers with Non-Linear and Random Potentials
The mean first passage time (MFPT) for photoexcitations diffusion in a
funneling potential of artificial tree-like light-harvesting antennae
(phenylacetylene dendrimers with generation-dependent segment lengths) is
computed. Effects of the non-linearity of the realistic funneling potential and
slow random solvent fluctuations considerably slow down the center-bound
diffusion beyond a temperature-dependent optimal size. Diffusion on a
disordered Cayley tree with a linear potential is investigated analytically. At
low temperatures we predict a phase in which the MFPT is dominated by a few
paths.Comment: 4 pages, 4 figures, To be published in Phys. Rev. Let
Theory of Dilute Binary Granular Gas Mixtures
A computer-aided method for accurately carrying out the Chapman-Enskog expansion of the Boltzmann equation, including its inelastic variant, is presented and employed to derive a hydrodynamic description of a dilute binary mixture of smooth inelastic spheres. Constitutive relations, formally valid for all physical values of the coefficients of restitution, are calculated by carrying out the pertinent Chapman-Enskog expansion to sufficient high orders in the Sonine polynomials to ensure numerical convergence. The resulting hydrodynamic description is applied to the analysis of a vertically vibrated binary mixture of particles (under gravity) differing only in their respective coefficients of restitution. It is shown that even with this “minor”difference the mixture partly segregates, its steady state exhibiting a sandwich-like configuration